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材料导报  2023, Vol. 37 Issue (S1): 23020009-12    https://doi.org/10.11896/cldb.23020009
  无机非金属及其复合材料 |
多孔炭基复合材料用作碱金属离子电池负极的研究进展
毛晓璇1, 冯柳2,*, 吴立清1, 辛伍红2, 牛金叶2
1 山东理工大学材料科学与工程学院,山东 淄博 255000
2 山东理工大学分析测试中心,山东 淄博 255000
Research Progress of Porous Carbon Matrix Composites Used as Anodes of Alkali Metal Ion Batteries
MAO Xiaoxuan1, FENG Liu2,*, WU Liqing1, XIN Wuhong2, NIU Jinye2
1 School of Materials Science and Engineering, Shandong University of Technology, Zibo 255000, Shandong, China
2 Analysis and Testing Center, Shandong University of Technology, Zibo 255000, Shandong, China
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摘要 碱金属离子(Li+、Na+和K+为主)电池功率密度高,使用寿命长,可实现大规模、持续性的电能存储和释放,是极具前景的储能设备之一。现有大规模使用的商业石墨负极容量已经接近理论值,限制了电池的发展,开发和优化高性能负极材料是推进碱金属离子电池商业化发展的关键因素。多孔炭材料具有丰富的孔道结构、较大的比表面积和优异的导电性,用作碱金属离子电池负极可提升其导电能力和电化学性能,但仍存在容量偏低的问题。因此,多孔炭材料的改性策略被广泛研究,并取得了一系列重要突破。本文主要综述了多孔炭基复合材料在碱金属离子电池负极应用的最新研究进展,首先概述了多孔炭材料的合成方法,然后分别梳理了近年来多孔炭材料用作锂离子电池、钠离子电池及钾离子电池负极性能提升的三种改性策略(杂原子掺杂、与金属化合物复合、多元材料共复合/掺杂),最后对多孔炭基负极材料的应用挑战和前景进行了分析与展望。
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毛晓璇
冯柳
吴立清
辛伍红
牛金叶
关键词:  碱金属离子电池  负极  多孔炭  掺杂  复合    
Abstract: As one of the most promising energy storage devices, alkali metal ion batteries (Li+, Na+ and K+ as main ions) characterized by high power density and long service life, can realize large-scale, continuous storage and release of electric energy. However, the capacity of large-scale commercial graphite in service has approached the theoretical value, thus restricting the development of batteries. Therefore, it is particularly important to develop anode materials with high capacity, good stability, long cycle life, and excellent rate performance. Porous carbon materials, with abundant pore structure, large specific surface area and excellent electrical conductivity, can be used as the anode of alkali metal ion batte-ries to improve the conductivity and electrochemical stability of batteries, as long as the low capacity problem is solved. Accordingly, the modification strategies have been studied extensively, and a series of significant breakthroughs have been achieved. In this paper, the research progress on the application of porous carbon composite materials in lithium-ion batteries, sodium-ion batteries and potassium-ion batteries anode is reviewed. The synthesis methods of porous carbon materials are summarized at first, and then three modification strategies (doping heteroatom, compositing with metal compounds, and co-compositing/doping multi-materials) widely used in recent years are reviewed. Furthermore, the prospects of porous carbon on alkali metal ion batteries are prospected.
Key words:  alkali metal ion battery    anode    porous carbon    doping    composite
发布日期:  2023-09-06
ZTFLH:  TQ127.2  
  TM912  
基金资助: 国家自然科学基金(22002074);山东省自然科学基金青年基金(ZR2020QE145)
通讯作者:  *冯柳,山东理工大学分析测试中心教授、硕士研究生导师。2001年河北理工大学本科毕业,2004年兰州理工大学硕士研究生毕业,后到山东理工大学工作至今,2014年上海大学博士研究生毕业。主要从事能源材料,微纳米尺度材料的制备、结构与机理研究。获发明专利7项,发表论文30余篇。willow-feng@163.com   
作者简介:  毛晓璇,2021年6月于山东理工大学获得工学学士学位。现为山东理工大学材料科学与工程学院硕士研究生,在冯柳教授的指导下进行研究。目前主要研究方向为碱金属离子电池电极材料的改性及性能的提升。
引用本文:    
毛晓璇, 冯柳, 吴立清, 辛伍红, 牛金叶. 多孔炭基复合材料用作碱金属离子电池负极的研究进展[J]. 材料导报, 2023, 37(S1): 23020009-12.
MAO Xiaoxuan, FENG Liu, WU Liqing, XIN Wuhong, NIU Jinye. Research Progress of Porous Carbon Matrix Composites Used as Anodes of Alkali Metal Ion Batteries. Materials Reports, 2023, 37(S1): 23020009-12.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.23020009  或          http://www.mater-rep.com/CN/Y2023/V37/IS1/23020009
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