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材料导报  2023, Vol. 37 Issue (3): 22090241-10    https://doi.org/10.11896/cldb.22090241
  多尺度稀土晶体材料及其应用 |
基于稀土层状氢氧化物的荧光材料研究进展
陈露, 朱琦*, 孙旭东*
东北大学材料科学与工程学院,材料各向异性与织构工程教育部重点实验室,沈阳 110819
Recent Research on Luminescent Materials Derived from Layered Rare-earth Hydroxides
CHEN Lu, ZHU Qi*, SUN Xudong*
Key Laboratory for Anisotropy and Texture of Materials (Ministry of Education),School of Materials Science and Engineering, Northeastern University, Shenyang 110819, China
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摘要 稀土层状氢氧化物(LRHs)结合了层状化合物的结构特性和稀土离子的功能特性,代表了一类新的功能材料,在光电、催化以及生物医学等领域具有巨大的应用潜力。本文主要综述了LRHs的研究进展,包括Ln2(OH)5(Ax-)1/x·nH2O (251-LRHs)和Ln2(OH)4SO4·nH2O (241-LRHs)的可控合成、结构特征、阴离子交换、纳米片剥离,以及在发光领域的应用,重点关注251-LRHs晶体的尺寸和形貌调控及纳米片剥离,总结了LRHs及其煅烧衍生物(氧化物、含氧硫酸盐和硫氧化物)荧光粉、高取向透明薄膜、光学温度传感器的发光特性,展望了LRHs功能化设计的研究方向,以期为今后进一步开发LRHs新型功能材料提供参考。
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陈露
朱琦
孙旭东
关键词:  稀土层状氢氧化物(LRHs)  阴离子交换  纳米片剥离  荧光粉  薄膜  光学温度传感器    
Abstract: Layered rare-earth hydroxides (LRHs), having a unique combination of a layered structure and the functional properties of rare-earth elements, are a new family of functional materials. The compounds have potential applications in electro-optic, catalytic, biomedical fields and so forth. This review summarizes the recent research on LRHs, including controlled synthesis, structural features, anion exchange, nanosheet exfoliation, and application in the field of luminescence for both the Ln2(OH)5(Ax-)1/x·nH2O (251-LRHs) and Ln2(OH)4SO4·nH2O (241-LRHs). Particular attention is paid to the size and morphology control and nano sheets exfoliation in 251-LRHs. The luminescent behaviors of LRHs themselves and calcined derivatives of the oxide, oxysulfate, and oxysulfide for phosphors, highly oriented transparent films, and optical temperature sensors are the main content. Finally, the prospects of LRHs on novel functional materials are proposed, which provides a new way for future functional design.
Key words:  layered rare-earth hydroxides (LRHs)    anion exchange    nanosheets exfoliation    phosphor    film    optical temperature sensor
出版日期:  2023-02-10      发布日期:  2023-02-23
ZTFLH:  TB34  
基金资助: 国家自然科学基金(51302032);辽宁省自然科学基金(2020-MS-081)
通讯作者:  *zhuq@smm.neu.edu.cn;xdsun@mail.neu.edu.cn，朱琦,东北大学材料科学与工程学院研究员、博士研究生导师,主要从事光功能陶瓷材料的合成、晶体结构解析及光学性能的研究。2006年7月、2008年7月分别于哈尔滨工程大学、东北大学获得工学学士学位和硕士学位,2012年于东北大学获得博士学位,博士期间在日本国立材料科学研究所(NIMS)联合培养两年。毕业工作后又再次留学日本在NIMS从事光功能陶瓷材料研究一年(访问学者)。在Chemistry of Materials、Chemical Enginee-ring Journal、Nanoscale、Journal of Materials Chemistry等期刊发表SCI收录论文140余篇,研究成果被引用4 000余次,授权国家发明专利23项。
孙旭东,东北大学材料科学与工程学院教授、博士研究生导师,国家杰出青年科学基金获得者(2004年)、俄罗斯自然科学院外籍院士。1982年7月获得东北大学金属学及热处理专业学士学位;1984年12月获得东北大学金属材料及热处理专业硕士学位;1993年11月获得英国 Surrey大学材料科学与工程专业博士学位。入选国家首届新世纪百千万人才工程(第一层次)计划、教育部创新团队发展计划、国家教育部跨世纪优秀人才培养计划等。曾任中国材料研究学会青委会理事、中国复合材料学会理事、美国陶瓷学会会员,现任中国颗粒学会理事。获得中国冶金青年科技奖等。主要研究方向为陶瓷材料、纳米粉体合成、贵金属材料。承担和完成国家自然科学基金(国家杰出青年科学基金,国家自然科学基金重大项目子课题、重点、面上项目等12项)、国家“863”计划、国家教育部创新团队发展计划、国防科工委军工项目等30余项科研课题。在Acta Mater.、Chem. Mater.等国内外刊物上发表论文300余篇,获得国家发明专利授权38项。   
作者简介:  陈露,东北大学材料科学与工程学院博士研究生,2017年6月、2021年6月分别于东北大学、上海大学(中国科学院上海硅酸盐研究所联合培养)获得工学学士学位和硕士学位,在朱琦研究员的指导下进行研究,目前主要研究领域为尖晶石型近红外长余辉荧光粉。
引用本文:    
陈露, 朱琦, 孙旭东. 基于稀土层状氢氧化物的荧光材料研究进展[J]. 材料导报, 2023, 37(3): 22090241-10.
CHEN Lu, ZHU Qi, SUN Xudong. Recent Research on Luminescent Materials Derived from Layered Rare-earth Hydroxides. Materials Reports, 2023, 37(3): 22090241-10.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.22090241  或          http://www.mater-rep.com/CN/Y2023/V37/I3/22090241
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