全无机CsPbBr3钙钛矿太阳电池的研究进展

doi:10.11896/cldb.20060145

材料导报

2021, Vol. 35

Issue (11): 11039-11056 https://doi.org/10.11896/cldb.20060145

无机非金属及其复合材料

全无机CsPbBr₃钙钛矿太阳电池的研究进展

刘壮, 陈建林^*, 黄才友, 彭卓寅^*, 何建军, 陈荐

长沙理工大学能源与动力工程学院,能源高效清洁利用湖南省高校重点实验室,长沙 410114

Progress of All-inorganic CsPbBr₃ Perovskite Solar Cells

LIU Zhuang, CHEN Jianlin^*, HUANG Caiyou, PENG Zhuoyin^*, HE Jianjun, CHEN Jian

Key Laboratory of Efficient and Clean Energy Utilization, Colleges of Hunan Province, School of Energy Science & Engineering, Changsha University of Science and Technology, Changsha 410114, China

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摘要自2009年第一次报道以来,有机-无机杂化钙钛矿太阳电池(PSCs)的光电转换效率(PCE)从3.8%提升至25.5%,已可以与商业化的晶体硅太阳电池相媲美,引起全世界研究者的极大关注。然而,由于杂化物晶体结构中有机成分弱的化学键,器件长期稳定性受到很大的影响。近年来,用无机Cs⁺完全取代有机基团构成全无机卤化物钙钛矿被认为是解决太阳电池稳定性问题的有效途径。在Cs基钙钛矿之中,CsPbBr₃具有最优异的耐热、耐光、耐湿性能,作为顶电池具有与晶体硅太阳电池组成长寿命叠层太阳电池的潜力。本文系统地综述了CsPbBr₃ PSCs领域的研究进展,首先介绍了CsPbBr₃ PSCs的发展历史及CsPbBr₃的晶体结构和基本特性,随后阐述了CsPbBr₃薄膜的制备方法、CsPbBr₃的元素掺杂改性、器件的界面工程等方面的研究进展;最后,讨论了当前存在的问题和提高CsPbBr₃ PSCs性能的未来方向,为进一步推动钙钛矿太阳电池的实用化进程提供参考。

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	刘壮
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关键词: 全无机钙钛矿太阳电池 CsPbBr₃ 长期稳定性

Abstract: Since the first report in 2009, organic-inorganic hybrid perovskite solar cells (PSCs) have seen the improved power conversion efficiency (PCE) from 3.8% to 25.5%, which can be comparable to the commercial crystalline silicon solar cells. They have attracted tremendous attention of researchers all over the world. However, due to the weak-bonded organic components in the hybrid crystal structure, the long-term stability of devices is greatly affected. In recent years, using inorganic Cs⁺ ion to completely replace organic groups to form all-inorganic perovskites is considered to be an effective way to solve the problem of instability. Among Cs-based perovskites, CsPbBr₃ perovskite has the most excellent heat, ultraviolet light and moisture resistance, which is potentially expected to form the top cell of tandem solar cells with long-life crystalline silicon solar cells. In this paper, we systematically reviewed the research progress of CsPbBr₃ PSCs. Firstly, the history of CsPbBr₃ PSCs, and the crystal structure and basic properties of CsPbBr₃ are briefly introduced, and then the preparation methods of CsPbBr₃ thin films, element doping modification of CsPbBr₃, interface engineering of devices, and other aspects of the research progress to promote the PCE are elaborated. Finally, the current issues and the future prospect of improving the performance of CsPbBr₃ PSCs are discussed, which will provide a feasible reference to further promote the practical process of perovskite solar cells.

Key words: all-inorganic perovskite solar cells CsPbBr₃ long-term stability

发布日期: 2021-06-25

ZTFLH:

TB34

基金资助: 湖南省自然科学基金(2020JJ4097); 国家留学基金委留金发2017(3059); 长沙理工大学“双一流”科学研究国际合作拓展项目(2018IC15)

通讯作者: *cjlinhunu@csust.edu.cn;383904268@C.qq.com

作者简介: 刘壮,2018年6月毕业于长沙理工大学,获得工学学士学位。现为长沙理工大学能源与动力工程学院硕士研究生,在陈建林副教授的指导下进行研究。目前主要研究领域为柔性钙钛矿太阳电池。陈建林,长沙理工大学能源与动力工程学院副教授、硕士研究生导师、湖南省可再生能源学会副会长。1999年6月本科毕业于桂林工学院,2009年9月博士毕业于湖南大学材料科学与工程专业, 2017年12月—2018年12月国家公派美国明尼苏达大学作访问学者。主要从事太阳能转换与利用的表界面工程研究,主持国家自然科学基金项目1项,发表学术论文40余篇,其中SCI收录25篇、EI收录6篇。彭卓寅,长沙理工大学能源与动力工程学院副教授、硕士研究生导师。2008年6月本科毕业于武汉理工大学材料科学与工程专业,2014年6月博士毕业于武汉理工大学材料物理与化学专业。主要从事新型太阳电池方面的研究,在金属氧化物纳米材料、量子点材料和各种纳米薄膜太阳电池(量子点敏化太阳电池、染料敏化太阳电池、钙钛矿太阳电池等)的可控制备、表征、性能及机理方面开展了大量的研究工作,主持国家自然科学基金项目1项,发表学术论文40余篇,其中SCI收录30余篇。

引用本文:

刘壮, 陈建林, 黄才友, 彭卓寅, 何建军, 陈荐. 全无机CsPbBr₃钙钛矿太阳电池的研究进展[J]. 材料导报, 2021, 35(11): 11039-11056.
LIU Zhuang, CHEN Jianlin, HUANG Caiyou, PENG Zhuoyin, HE Jianjun, CHEN Jian. Progress of All-inorganic CsPbBr₃ Perovskite Solar Cells. Materials Reports, 2021, 35(11): 11039-11056.

链接本文:

http://www.mater-rep.com/CN/10.11896/cldb.20060145 或 http://www.mater-rep.com/CN/Y2021/V35/I11/11039

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