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材料导报  2023, Vol. 37 Issue (24): 22040242-6    https://doi.org/10.11896/cldb.22040242
  无机非金属及其复合材料 |
稀土氧化物掺杂对YSZ热障涂层热物理性能影响的研究进展
刘电超, 金国*, 井勇智, 崔秀芳, 房永超, 陈卓, 王薪贺
哈尔滨工程大学材料科学与化学工程学院,超轻材料与表面技术教育部重点实验室,哈尔滨 150001
Research Progress on the Effects of Rare Earth Oxides Doping on Thermophysical Properties of YSZ Thermal Barrier Coatings
LIU Dianchao, JIN Guo*, JING Yongzhi, CUI Xiufang, FANG Yongchao, CHEN Zhuo, WANG Xinhe
Key Laboratory of Superlight Material and Surface Technology of Ministry of Education, College of Material Science and Chemical Engineering, Harbin Enginee-ring University, Harbin 150001, China
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摘要 随着航空发动机和燃气轮机(简称“两机”)服役温度的升高,目前,在两机热端部件表面防护方面应用最为广泛的热障涂层(Thermal barrier coatings,TBCs)存在陶瓷层材料氧化钇稳定氧化锆(Yttria-stabilized zirconia,YSZ)在高温下会发生相转变、热膨胀系数与金属基底不匹配以及烧结导致涂层的热导率升高等问题,严重影响TBCs的服役寿命。新一代TBCs陶瓷面层材料分为以下几类:(1)稀土氧化物稳定YSZ;(2)钙钛矿结构陶瓷材料;(3)稀土六铝酸盐或稀土钽酸盐;(4)烧绿石或萤石结构稀土锆酸盐。其中,稀土氧化物掺杂可有效降低YSZ热障涂层的热导率,提高其热膨胀系数、高温相稳定性及耐烧结性能,被认为是提高YSZ热障涂层高温稳定性的有效方法。基于此,本文重点阐述了单元或多元稀土氧化物掺杂YSZ热障涂层材料的研究进展,讨论了稀土氧化物掺杂对YSZ陶瓷面层高温相稳定性、热导率和热膨胀系数的影响机理。基于耦合作用机理为未来稀土氧化物掺杂YSZ热障涂层的研发提供一定的借鉴。
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刘电超
金国
井勇智
崔秀芳
房永超
陈卓
王薪贺
关键词:  热障涂层  掺杂机理  热导率  热膨胀系数  相转变行为    
Abstract: With the increase in the service temperature of aero engines and gas turbines, thermal barrier coatings (TBCs) are most widely used in the surface protection of hot section components of two engines. There are some problems with yttria stabilized zirconia (YSZ) of ceramic layer material such as phase transformation at elevated temperature, mismatch between the thermal expansion coefficient and metal substrates, and increase in the thermal conductivity of coatings caused by sintering, which seriously affects the service life of TBCs. The new generation of TBCs materials are divided into the following categories:(i) rare earth oxides to stabilize YSZ; (ii) ceramic materials of perovskite structure; (iii) rare-earth hexaaluminates or rare-earth tantalates; (iv) pyrochlore or fluorite structured rare earth zirconates. Among them, rare earth oxides doping can effectively reduce the thermal conductivity of YSZ thermal barrier coatings and improve their thermal expansion coefficient, high temperature phase stability and sintering resistance, which is an effective method to improve the high temperature stability of YSZ thermal barrier coatings. Therefore, the main purpose of this paper is to focus on the research progress of unit or multi-element rare earth oxides doped YSZ thermal barrier coatings, the mechanism of the effect of rare earth oxides doping on the properties of high temperature phase stability, thermal conductivity and thermal expansion coefficient of YSZ top coatings is discussed. The coupling-based mechanism provides some implications for the future development of rare earth oxides doped YSZ thermal barrier coatings.
Key words:  thermal barrier coating    doping mechanism    thermal conductivity    thermal expansion coefficient    phase transition behavior
发布日期:  2023-12-19
ZTFLH:  TG148  
基金资助: 国家自然科学基金(52175163)
通讯作者:  *金国,博士,哈尔滨工程大学材料科学与化学工程学院教授、博士研究生导师,龙江学者特聘教授。目前的主要研究方向为表面工程、再制造、摩擦学等。作为项目负责人先后承担完成各类基金项目40余项,在国内外著名刊物发表论文100余篇。jinjg721@163.com   
作者简介:  刘电超,现为哈尔滨工程大学材料科学与化学工程学院硕士研究生,在金国教授和崔秀芳教授的指导下进行研究。目前主要研究领域为表面工程。
引用本文:    
刘电超, 金国, 井勇智, 崔秀芳, 房永超, 陈卓, 王薪贺. 稀土氧化物掺杂对YSZ热障涂层热物理性能影响的研究进展[J]. 材料导报, 2023, 37(24): 22040242-6.
LIU Dianchao, JIN Guo, JING Yongzhi, CUI Xiufang, FANG Yongchao, CHEN Zhuo, WANG Xinhe. Research Progress on the Effects of Rare Earth Oxides Doping on Thermophysical Properties of YSZ Thermal Barrier Coatings. Materials Reports, 2023, 37(24): 22040242-6.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.22040242  或          http://www.mater-rep.com/CN/Y2023/V37/I24/22040242
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