铅炭电池负极添加剂研究进展

doi:10.11896/cldb.22030203

材料导报

2023, Vol. 37

Issue (22): 22030203-8 https://doi.org/10.11896/cldb.22030203

无机非金属及其复合材料

铅炭电池负极添加剂研究进展

谢发之^1,*, 宋恒帅¹, 张道德¹, 杨少华², 张梦¹, 方亮², 邵永刚²

1 安徽建筑大学材料与化学工程学院,合肥 230601
2 安徽艾克瑞德科技有限公司,安徽黄山 242700

Research Progress of Additives for Lead-Carbon Battery Anodes

XIE Fazhi^1,*, SONG Hengshuai¹, ZHANG Daode¹, YANG Shaohua², ZHANG Meng¹, FANG Liang², SHAO Yonggang²

1 School of Materials and Chemical Engineering, Anhui Jianzhu University, Hefei 230601, China
2 Anhui Accord Science and Technology Co., Ltd., Huangshan 242700, Anhui, China

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摘要铅炭电池是在铅酸电池研究的基础上,选取具有多孔、高比表面积的碳材料作为负极材料添加剂来进一步提高性能的电池。碳材料为电池放电过程中产生的硫酸铅 (PbSO₄) 提供更多反应界面,从而抑制硫酸盐化,使电池循环寿命得以延长,但碳较低的析氢过电位会带来析氢速率过快的问题。目前,铅炭电池负极添加剂开始由不同结构碳材料及析氢抑制剂的研究转向复合型材料研究,如碳与铅型复合材料、碳与导电聚合物型复合材料以及碳与析氢抑制剂型复合材料等,其主要目的是在延长电池循环使用寿命的同时,能够有效解决碳材料带来的析氢速率过快及铅与添加剂相容性差的问题。本文主要综述了近年来铅炭电池负极添加剂的研究进展,分别对碳添加剂、析氢抑制剂以及复合材料添加剂进行归纳分析,并结合目前实际发展情况分析了未来铅炭电池发展可能遇到的问题及研究方向。

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	谢发之
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	方亮
	邵永刚

关键词: 铅炭电池硫酸盐化碳材料析氢抑制剂复合材料循环寿命

Abstract: High performance lead-carbon batteries are developed from lead-acid batteries; carbon materials, which are porous with a high specific surface area, are selected as negative additives. Carbon materials provide reaction surfaces for lead sulfate (PbSO₄) produced during battery discharge, which can inhibit sulfation and prolong the cycle life of the batteries. However, the low hydrogen evolution potential of carbon results in an excessive hydrogen evolution rate. Recently, the focus of research on anode additives of lead-carbon batteries was moved from carbon materials with different structures and hydrogen evolution inhibitors to various carbon composite materials (e.g., C/Pb, C/conductive polymer, and C/H evolution inhibitor). The primary reason is that the addition of carbon composite materials can effectively solve the problems of rapid hydrogen evolution caused by carbon materials and poor compatibility between lead and additives, while prolonging the cycle life of batteries. This paper mainly reviews the research progress of negative electrode additives for lead-carbon batteries in recent years and analyses carbon additives, hydrogen evolution inhibitors, and composite additives. Further, the problems that may be encountered in the future are detailed and possible research directions are outlined.

Key words: lead-carbon battery sulfation carbon materials hydrogen evolution inhibitors composites cycle life

出版日期: 2023-11-25 发布日期: 2023-11-21

ZTFLH:

TM912

基金资助: 安徽省教育厅高校自然科学研究项目 (KJ2018ZD049)

通讯作者: * 谢发之,安徽建筑大学材料与化学工程学院教授、硕士研究生导师。目前主要从事功能材料与储能技术研究以及水污染控制、污染物监测等研究工作。发表学术论文62篇,其中SCI、EI 39篇;获国家发明专利6项。fzxie@ahjzu.edu.cn

引用本文:

谢发之, 宋恒帅, 张道德, 杨少华, 张梦, 方亮, 邵永刚. 铅炭电池负极添加剂研究进展[J]. 材料导报, 2023, 37(22): 22030203-8.
XIE Fazhi, SONG Hengshuai, ZHANG Daode, YANG Shaohua, ZHANG Meng, FANG Liang, SHAO Yonggang. Research Progress of Additives for Lead-Carbon Battery Anodes. Materials Reports, 2023, 37(22): 22030203-8.

链接本文:

http://www.mater-rep.com/CN/10.11896/cldb.22030203 或 http://www.mater-rep.com/CN/Y2023/V37/I22/22030203

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