锂离子电池钒系电极材料的研究进展

doi:10.11896/cldb.20060110

材料导报

2021, Vol. 35

Issue (21): 21127-21142 https://doi.org/10.11896/cldb.20060110

无机非金属及其复合材料

锂离子电池钒系电极材料的研究进展

王皓¹, 李峻峰¹, 马悦¹, 杨亚楠¹, 张佩聪¹, 赖雪飞², 岳波³

1 成都理工大学材料与化学化工学院,成都 610059
2 四川大学化学工程学院,成都 610065
3 四川新锂想能源科技有限责任公司,射洪 629200

Review of Vanadium-based Electrode Materials for Lithium Ion Batteries

WANG Hao¹, LI Junfeng¹, MA Yue¹, YANG Yanan¹, ZHANG Peicong¹, LAI Xuefei², YUE Bo³

1 College of Materials and Chemical Engineering, Chengdu University of Technology, Chengdu 610059, China
2 School of Chemical Engineering, Sichuan University, Chengdu 610065, China
3 Sichuan Xinlixiang Energy Technology Co., Ltd., Shehong 629200, China

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摘要锂离子电池电极材料对锂离子电池性能提升起着关键作用。钒的价态较多,构成的钒系电极材料具有层状、尖晶石型、反尖晶石型等多种结构。该系列材料通常具有较高的理论比容量,且合成方式多样,性价比高,因此钒系化合物在锂离子电池电极材料的应用上受到了广泛关注,但目前尚缺少对钒系电极材料的系统性总结。本文综述了以钒的氧化物、无锂型金属离子钒酸盐、含锂型钒酸盐及钒磷酸根聚阴离子材料为主要体系的锂离子电池钒系电极材料,并对各体系的结构及电化学性能进行了总结,针对合成锂离子电池钒系电极材料的主要方法(如固相合成法、溶胶-凝胶法、水热法、碳热还原法、液相沉淀法等)进行概述及分析,还对通过纳米化、特殊形貌控制、复合改性等其他改性方式优化的钒系电极材料的性能进行了介绍,最后对钒系锂离子电池电极材料的研究方向和发展前景进行展望,希望对促进该类材料的研究与产业化应用能有所助益。

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	王皓
	李峻峰
	马悦
	杨亚楠
	张佩聪
	赖雪飞
	岳波

关键词: 锂钒化合物锂离子电池正极材料负极材料

Abstract: To improve the performance of lithium ion batteries, the electrode materials are a key point. Vanadium has rich variable valence state, and the vanadium-based electrode materials are under a variety of structures with layered-structure, spinel and anti-spinel structure. Vanadium-based electrode materials have the properties of higher theoretical specific capacity, various synthesis methods and cost-effective. The application of vanadium-based compounds have attracted extensive attention in lithium ion battery electrode materials. However, it is still lack of a systematic summary of vanadium-based electrode materials. This paper reviews the structure and electrochemical performance of promising electrode mate-rials for lithium ion batteries of vanadium-based electrode materials, which mainly include vanadium oxide, lithium-free vanadate, lithium-containing vanadate and lithium vanadium phosphate. Methods for synthesis of vanadium-based electrode materials are summarized, including solid phase synthesis, sol-gel synthesis, hydrothermal synthesis, carbothermal reduction synthesis, and liquid phase precipitation synthesis. The methods to optimize the defects of vanadium electrode materials by controlling of nano-crystallization, morphology and composite are also concluded. Finally, an outlook on potential breakthroughs for vanadium-based electrode materials will be provided.

Key words: lithium vanadium compound lithium-ion battery cathode material anode material

出版日期: 2021-11-10 发布日期: 2021-11-30

ZTFLH:

TM912

基金资助: 四川钒钛产业发展研究中心开放项目(2018VTCY-Z-01);四川省教育厅自然科学重点项目(18ZA0062);四川省科技厅重大科技专项(2019ZDZX0025)

通讯作者: lijunfeng@cdut.cn

作者简介: 王皓,2018年6月毕业于成都理工大学工程技术学院,获得工学学士学位。现为成都理工大学材料与化学化工学院硕士研究生,在李峻峰教授的指导下进行研究。目前主要研究领域为锂离子电池非晶态正极材料。
李峻峰,成都理工大学材料与化学化工学院教授、硕士研究生导师。2000年6月本科毕业于四川大学材料学院无机非金属材料专业,2005年6月在成都理工大学材料学专业获硕士学位,2009年6月在四川大学医学工程专业取得博士学位。主要从事新材料开发与应用相关的研究工作,具体包括稀土发光及催化材料、锂离子电池电极材料、骨修复材料。近年来,发表科研学术论文100篇,申请国家发明专利30项。

引用本文:

王皓, 李峻峰, 马悦, 杨亚楠, 张佩聪, 赖雪飞, 岳波. 锂离子电池钒系电极材料的研究进展[J]. 材料导报, 2021, 35(21): 21127-21142.
WANG Hao, LI Junfeng, MA Yue, YANG Yanan, ZHANG Peicong, LAI Xuefei, YUE Bo. Review of Vanadium-based Electrode Materials for Lithium Ion Batteries. Materials Reports, 2021, 35(21): 21127-21142.

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http://www.mater-rep.com/CN/10.11896/cldb.20060110 或 http://www.mater-rep.com/CN/Y2021/V35/I21/21127

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