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材料导报  2023, Vol. 37 Issue (17): 21120161-12    https://doi.org/10.11896/cldb.21120161
  无机非金属及其复合材料 |
纳米粒子自组装超结构的制备及基于构效关系的性能
秦肖雲1,*, 邵文龙1, 田宽1, 姜利英2, 罗聃3,4,*
1 郑州轻工业大学材料与化学工程学院,郑州 450002
2 郑州轻工业大学电气信息工程学院,郑州 450002
3 北京纳米能源与系统研究所,北京 101400
4 中国科学院大学纳米科学与技术学院,北京 100049
Preparation of Self-assembled Nanoparticles Superstructures and Their Properties Based on Structure-Activity Principle
QIN Xiaoyun1,*, SHAO Wenlong1, TIAN Kuan1, JIANG Liying2, LUO Dan3,4,*
1 School of Materials and Chemical Engineering, Zhengzhou University of Light Industry, Zhengzhou 450002, China
2 School of Electrical and Information Engineering, Zhengzhou University of Light Industry, Zhengzhou 450002, China
3 Beijing Institute of Nanoenergy and Nanosystems, Beijing 101400, China
4 School of Nanoscience and Technology, University of Chinese Academy of Sciences, Beijing 100049, China
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摘要 随着对纳米粒子形貌和尺寸的控制越来越成熟,由高度单分散的纳米粒子(粒径偏差不大于5%)自组装而成具有规则晶格结构的超结构成为可能,并受到越来越多的关注。纳米材料学家通过“人造块体”的概念来构建纳米粒子自组装超结构,以纳米粒子为“人造原子”,通过粒子间的相互作用力搭建具有不同堆积模式的超晶结构。作为一种“自下而上”构建材料的制备方法,纳米粒子的自组装技术可以实现材料器件的大面积制备。构效关系是自然界中广泛存在的一项基本原则,指的是物质的组成结构与其物理化学性能之间的关系。基于不同组装结构基元、不同堆积模式下的纳米粒子自组装超结构展现出区别于单分散纳米粒子和块体材料的特殊集体性能,在光学、电学、催化、生物医药等领域展现出广阔的应用前景。基于纳米粒子间的相互作用并充分利用外界环境,科研工作者们发展了一系列实现纳米粒子自组装的方法,从材料性能角度出发设计组装基元和堆积结构,构筑自组装超结构以实现功能定制化的集体性能。
本文总结了纳米粒子自组装超结构的组装机理以及组装方法,并从构效关系入手,讨论了纳米粒子自组装超结构与材料的光学、电学、磁学、力学集体性能之间的联系,对近年来纳米粒子自组装超结构方面的研究进展进行了综述,重点论述了构效关系在纳米粒子自组装超结构中的体现。通过改变纳米粒子自组装超结构的组成元素和搭建结构,各类纳米制造技术可以调节纳米材料的物理化学性能,以适应各个应用领域的不同需求。
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秦肖雲
邵文龙
田宽
姜利英
罗聃
关键词:  纳米粒子  自组装  超结构  构效关系  集体性能    
Abstract: With the mature control of morphology and size of nanoparticles, the superstructure can be self-assembled with regular lattice structure from highly monodispersed nanoparticles (size deviation ≤5%). Nanomaterials scientists use the concept of ‘artificial solids’ to construct self-assembled superstructures, by exploiting nanoparticles as ‘artificial atoms’ in building supercrystals with different stacking modes through interactions between the adjacent particles. As a ‘bottom-up’ fabrication approach, the self-assembly method can achieve fabrication of material devices in large area. Structure-activity relationship is a basic principle that widely exists in nature. It refers to the relationship between the composition and structure of a substance and its physical and chemical properties. The self-assembled superstructures of nanoparticles based on different constructed bricks and stacking modes show special collective properties different fromboth individual nanoparticles and their bulk materials, and show broad application prospects in optics, electricity, catalysis, biomedicine and other fields. Based on the interaction between nanoparticles and taking full advantage of the external environment, researchers have developed a series of self-assembly methods to construct superstructures with customized performance, which is realized by designing the building blocks and stacking structures from the point of view of desired material properties.
This review offers a retrospection of the self-assembled mechanism, methods, and research progress in this area, and provides elaborate descriptions about how the assembled superstructures take effects on their optical, electric, magnetic, and mechanical properties. It is focused on the embodiment of properties arising from the structure-activity principle in the self-assembled superstructures. By changing the components and structures of the self-assembled nanoparticles superstructures, different physical and chemical properties can be obtained to adapt to different application fields.
Key words:  nanoparticle    self-assembly    superstructure    structure-activity    collective property
出版日期:  2023-09-10      发布日期:  2023-09-05
ZTFLH:  O648  
基金资助: 国家自然科学基金(21904120;62073299;51902344);河南省重点研发与推广专项(科技攻关)项目(212102310858);中原科技创新领军人才项目(224200510026);郑州轻工业大学博士启动资金(2018BSJJ022)
通讯作者:  *秦肖雲,郑州轻工业大学讲师、硕士研究生导师。2010年唐山师范学院应用化学专业本科毕业,2013年西华师范大学物理化学专业硕士毕业,2017年中国科学院化学研究所分析化学专业博士毕业。2018年3月入职郑州轻工业大学工作至今,目前主要从事纳米粒子自组装及电化学传感方面的研究工作。发表SCI论文20余篇,包括Adv.Mater.、Adv.Funct.Mater.、Nano Today、Anal.Chem.、Electrochem.Commun.等。xyqin@zzuli.edu.cn
罗聃,青年研究员,博士研究生导师。2008年毕业于北京大学药学院,获理学学士学位,2013年毕业于北京大学生物物理系,获理学博士学位。2013年8月—2015年3月在中国科学院化学研究所工作担任助理研究员;2015年3月—2021年3月就职于中国石油大学(北京),先后担任助理研究员、副研究员、新能源科学与工程系副主任、生物质能源党支部书记;2021年3月入职中国科学院北京纳米能源与系统研究所。主要从事高性能纳米材料的设计与合成、仿生纳米界面的开发、纳米材料在生物调控及能源转化应用的研究,并开展纳米发电机在药物递送及组织修复领域的研究。已在Nat.Commun.、J.Am.Chem.Soc.、Adv.Mater.、Adv.Funct.Mater.、Nano Energy、ACS Nano、Small、J.Mater.Chem.A、Adv.Healthc.Mater.等国际权威学术期刊发表SCI论文30余篇。luodan@binn.cas.cn   
引用本文:    
秦肖雲, 邵文龙, 田宽, 姜利英, 罗聃. 纳米粒子自组装超结构的制备及基于构效关系的性能[J]. 材料导报, 2023, 37(17): 21120161-12.
QIN Xiaoyun, SHAO Wenlong, TIAN Kuan, JIANG Liying, LUO Dan. Preparation of Self-assembled Nanoparticles Superstructures and Their Properties Based on Structure-Activity Principle. Materials Reports, 2023, 37(17): 21120161-12.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.21120161  或          http://www.mater-rep.com/CN/Y2023/V37/I17/21120161
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