尖晶石型铁氧体异质结的构建及用于有机污染物光催化降解的研究进展

doi:10.11896/cldb.21110278

材料导报

2023, Vol. 37

Issue (16): 21110278-10 https://doi.org/10.11896/cldb.21110278

无机非金属及其复合材料

尖晶石型铁氧体异质结的构建及用于有机污染物光催化降解的研究进展

陈丹丹, 李燕^*, 王爱国

安徽建筑大学先进建筑材料安徽省重点实验室,合肥 230601

Research Progress on Fabrication and Application in Photocatalytic Degradation of Organic Pollutants of Spinel Ferrite Heterojunction

CHEN Dandan, LI Yan^*, WANG Aiguo

Anhui Key Laboratory of Advanced Building Materials, Anhui Jianzhu University, Hefei 230601, China

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摘要随着工业生产的快速发展,有机废水的排放对环境造成了严重的污染。光催化技术利用太阳能降解有机污染物,被视为极具前途的污水处理技术之一。然而传统光催化剂(TiO₂、ZnO、ZnS等)对可见光的利用率低、光生载流子复合率高和回收困难等问题限制了其在光催化领域的实际应用。研究者提出将传统半导体与尖晶石型铁氧体材料复合制备尖晶石型铁氧体异质结光催化剂,通过异质结的界面作用抑制光催化剂中光生电荷的复合。同时,尖晶石型铁氧体优异的磁学性能为异质结光催化剂在废水处理中的回收和再利用提供了保证。目前,大量的尖晶石型铁氧体在合成异质结光催化剂领域已经取得了显著的研究成果,例如Fe₃O₄、CoFe₂O₄、CuFe₂O₄、ZnFe₂O₄和NiFe₂O₄等。本文将尖晶石型铁氧体异质结分为 Ⅱ 型、肖特基型、Z型 (传统Z型、全固态Z型、直接Z型) 和S型,并具体介绍了各类尖晶石型铁氧体异质结材料光生电荷的分离途径、各类晶石型铁氧体异质结材料目前存在的缺陷以及尖晶石型铁氧体异质结光催化剂在水体治理领域应用的现状,为构建出高载流子分离率的尖晶石型铁氧体异质结光催化剂提供能带匹配理论参考。

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	陈丹丹
	李燕
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关键词: 尖晶石型铁氧体异质结光催化降解载流子迁移

Abstract: Discharge of organic wastewater into the environment following the rapid development of industrial production has led to serious pollution. Photocatalytic technology using solar energy to degrade organic pollutants is considered one of the most valuable strategies for water treatment. However, traditional photocatalysts (e.g., TiO₂, ZnO, and ZnS) suffer from the inefficient use of visible light, high recombination rate of photon-generated carriers, and poor recycling performance, which hinder their widespread application. Researchers have proposed the preparation of the spinel ferrite heterojunction photocatalyst by combining a traditional semiconductor and spinel ferrite. Photocarrier recombination is inhibited by the interface of the heterojunction, and the excellent magnetic properties of the ferrite guarantee the recovery and reuse of the photocatalyst in wastewater treatment. At present, a large number of spinel ferrites such as Fe₃O₄, CoFe₂O₄, CuFe₂O₄, ZnFe₂O₄ and NiFe₂O₄ have led to remarkable research results in the field of heterojunction photocatalysts. In this paper, the spinel ferrite heterojunctions are divided into type-Ⅱ, Schottky, Z-scheme (traditional, all-solid-state, and direct), and step-scheme heterojunctions. The separation strategies of the photogenerated charges, defects in various spinel ferrite heterojunction materials, as well as their applications in the field of water treatment are discussed, providing a theoretical reference for the construction of spinel ferrite heterojunction photocatalysts with high carrier separation rates.

Key words: spinel ferrite heterojunction photocatalytic degradation carrier transfer

出版日期: 2023-08-25 发布日期: 2023-08-14

ZTFLH:

O649

基金资助: 安徽省高校自然科学基金重点项目 (KJ2020A0476);安徽省重点研究与开发计划项目(202004b11020033)

通讯作者: ^*李燕,1985年曲阜师范学院本科毕业,1991年中国科学技术大学硕士毕业;2008年合肥工业大学材料学院材料学专业博士毕业。1995年迄今在安徽建筑大学工作,现为教授。目前主要从事无机功能材料、纳米材料合成与制备化学等方面的研究工作。近年来,在新型无机功能材料领域发表论文30余篇,包括International Journal of Refractory Metals & Hard Materials、Asian Journal of Chemistry、Advanced Materials Research、Journal of Materials Processing Technology、《复合材料学报》《人工晶体学报》和《硅酸盐通报》等。lyc171805@163.com

作者简介: 陈丹丹,2020年6月毕业于安徽建筑大学,获得理学学士学位。现为安徽建筑大学材料与化学工程学院硕士研究生,在李燕教授的指导下进行研究。目前主要研究领域为光催化复合材料。

引用本文:

陈丹丹, 李燕, 王爱国. 尖晶石型铁氧体异质结的构建及用于有机污染物光催化降解的研究进展[J]. 材料导报, 2023, 37(16): 21110278-10.
CHEN Dandan, LI Yan, WANG Aiguo. Research Progress on Fabrication and Application in Photocatalytic Degradation of Organic Pollutants of Spinel Ferrite Heterojunction. Materials Reports, 2023, 37(16): 21110278-10.

链接本文:

http://www.mater-rep.com/CN/10.11896/cldb.21110278 或 http://www.mater-rep.com/CN/Y2023/V37/I16/21110278

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