过硫酸盐高级氧化技术在土壤和地下水修复中的研究进展

材料导报

2020, Vol. 34

Issue (Z1): 107-110

无机非金属及其复合材料

过硫酸盐高级氧化技术在土壤和地下水修复中的研究进展

代朝猛¹, 王泽雨¹, 段艳平², 刘曙光¹, 涂耀仁², 李彦¹

1 同济大学土木工程学院,上海 200092;
2 上海师范大学环境与地理科学学院,上海 200234

Persulfate-based Advanced Oxidation Processes for Soil and GroundwaterRemediation: a Review

DAI Chaomeng¹, WANG Zeyu¹, DUAN Yanping², LIU Shuguang¹, TU Yaoren², LI Yan¹

1 College of Civil Engineering, Tongji University, Shanghai 200092, China;
2 School of Environmental and Geographical Sciences, Shanghai Normal University, Shanghai 200234, China

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摘要过硫酸盐由于卓越的特性,被广泛应用于土壤和地下水修复。在前期的研究中,学者们发现在不同活化条件下,过硫酸盐分解产生的自由基种类不同,降解有机污染物的效果也不同。本文综述了国内外过硫酸盐在土壤和地下水修复中几种活化技术的研究进展,包括热活化、UV活化、过渡金属离子活化、碱活化、超声活化以及含碳物质活化;详细介绍了不同类型的过渡金属离子活化过硫酸盐降解有机污染物的效果,包括零价铁、金属氧化物、双金属、铁与螯合剂的络合物以及搭载纳米级金属的复合材料;简述了有关过硫酸盐的组合技术的研究现状,包括过硫酸盐多种活化方式的结合使用以及过硫酸盐与电化学技术、微生物、表面活性剂的组合使用;最后总结了过硫酸盐研究中目前存在的问题,并对其未来的发展提出了建议。

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关键词: 过硫酸盐活化土壤地下水修复有机污染物

Abstract: Persulfate is widely used in soil and groundwater remediation due to its excellent properties. In the previous research, scholars found that under different activation conditions, the types of free radicals produced by persulfate decomposition are different, and the effects of degrading organic pollutants are also different. This paper reviews the research progress of several activation techniques of persulfate in soil and groundwater remediation at home and abroad, including thermal activation, UV activation, transition metal ion activation, alkali activation, ultrasonic activation and activation of carbonaceous materials. The effects of different types of transition metal ions on the activation of persulfate to degrade organic pollutants are described in detail, including zero-valent iron, metal oxides, bimetals, complexes of iron and chelating agents, and composites with nano-scale metals. The research status of the combined technology of persulfate is briefly described, including the combination of various activation modes of persulfate and the combination of persulfate with electrochemical technology, microorganisms and surfactants. Finally, the problems existing in the persulfate research are summarized, and suggestions for its future development are put forward.

Key words: persulfate activation soil groundwater remediation organic contaminant

发布日期: 2020-07-01

ZTFLH:	X52
	X53

基金资助: 国家自然科学基金(41601514);上海市自然科学基金(19ZR1459300);上海市教育委员会重点学科交叉基金(0200121005/053;2019010202)

作者简介: 代朝猛,同济大学土木学院副教授、硕士生导师。2007年在郑州大学获得硕士学位,2011年获得同济大学和德国柏林工业大学博士学位。主要研究方向为地下水污染治理与修复、地下水数值模拟计算。近年来发表学术论文将近70篇,其中SCI收录论文40多篇,ESI高被引论文2篇;段艳平,助理研究员,主要关注新兴污染物(药物与个人护理品、持久性有机污染物和环境激素类物质等)的分析方法、迁移转化及污染控制技术。主持国家自然科学基金、上海市自然科学基金等多项科研项目。近年来在国内外核心学术刊物上发表论文20余篇,申请专利6项,主编专著1部,参编教材2部。

引用本文:

代朝猛, 王泽雨, 段艳平, 刘曙光, 涂耀仁, 李彦. 过硫酸盐高级氧化技术在土壤和地下水修复中的研究进展[J]. 材料导报, 2020, 34(Z1): 107-110.
DAI Chaomeng, WANG Zeyu, DUAN Yanping, LIU Shuguang, TU Yaoren, LI Yan. Persulfate-based Advanced Oxidation Processes for Soil and GroundwaterRemediation: a Review. Materials Reports, 2020, 34(Z1): 107-110.

链接本文:

http://www.mater-rep.com/CN/ 或 http://www.mater-rep.com/CN/Y2020/V34/IZ1/107

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