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材料导报  2023, Vol. 37 Issue (5): 21050074-11    https://doi.org/10.11896/cldb.21050074
  无机非金属及其复合材料 |
基于定向冷冻技术构建的多孔材料及其应用
俞彦飞1, 王暄1,2, 高鑫3,*, 宁锋3, 张浩鹏3, 岳红彦3
1 哈尔滨理工大学电气与电子工程学院,哈尔滨 150080
2 哈尔滨理工大学电介质及其应用重点实验室,哈尔滨 150080
3 哈尔滨理工大学材料科学与化学工程学院,哈尔滨 150040
Review of Porous Materials Derived from Using the Directional Freeze-casting Technique and Their Applications
YU Yanfei1, WANG Xuan1,2, GAO Xin3,*, NING Feng3, ZHANG Haopeng3, YUE Hongyan3
1 School of Electrical and Electronic Engineering, Harbin University of Science and Technology, Harbin 150080, China
2 Key Laboratory of Engineering Dielectrics and Its Application, Harbin University of Science and Technology, Harbin 150080, China
3 School of Materials Science and Chemical Engineering, Harbin University of Science and Technology, Harbin 150040, China
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摘要 定向冷冻技术是将原材料、溶剂及添加剂均匀混合,利用溶剂的“液-固-气”相转变获得多孔材料的一种方法,具有操作简便和绿色环保等优点。与通常的造孔技术不同,定向冷冻技术可实现对物理、化学和力学性能的高度控制,所制备的材料具有定向排列的孔隙和不同层面上的分级结构。这种技术被广泛应用于制备具有各向异性的无机、有机、杂化和碳质多孔材料。此外,该方法还可以扩展到模拟天然结构的仿生材料中,以组装具有优异力学和物理特征的多孔复合材料,在环境、能源、热管理和生物医学等领域具有广阔的应用前景。
本文从定向冷冻技术的来源以及原理出发,根据单颗粒及多颗粒的受力模型揭示了定向结构的形成机理,分析了溶质、溶剂、温度梯度和添加剂等对材料结构以及性能的影响。另外,根据前驱体材料掺杂改性的不同手段,介绍了一步法与两步法制备定向结构的特点。同时,总结了定向冷冻技术在污染物吸附、能量储存与转换、结构材料、热管理和生物材料等方面的研究进展,最后指出了当前研究中亟需解决的问题,并展望了其未来的发展方向。
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俞彦飞
王暄
高鑫
宁锋
张浩鹏
岳红彦
关键词:  多孔材料  定向冷冻  冰模板  各向异性    
Abstract: Directional freeze casting is a method that uses the "liquid-solid-gas" phase transformation of solvents to obtain porous materials by uniformly mixing raw materials, solvents and additives. It has the advantages of simple operation and green environmental protection. Different from the usual pore-making technology, it offers a high degree of control over the physical, chemical and mechanical properties of materials, where the materials prepared by this technology have oriented pores and hierarchical structures at different levels. Because of these characteristics, this technique is widely used in anisotropic porous inorganic, organic, hybrid and carbonaceous materials. This method can also be extended to simulate the structures of natural materials to assemble porous composites with excellent mechanical and physical properties. Finally, the method offers wide application prospects in fields such as environmental science, energy, thermal management and biology.
In this paper, based on the origins and principles of directional freezing technology, the formation mechanism of a directional structure is revealed based on the force model of single and multiple particles. The effects of the solute, solvent, temperature gradient, and additives on a structure and on the properties of the materials are analyzed. In addition, according to the different means of doping modification of precursor materials, the characteristics of directional structures prepared by one-step and two-step methods are introduced. Simultaneously, the research progress of directional freezing technology in pollutant adsorption, energy storage and conversion, structural materials, thermal management, and biomaterials are summarized. Finally, the problems that must be solved in the current research are briefly described, and future developmental directions are proposed.
Key words:  porous material    directional freeze-casting    ice template    anisotropy
出版日期:  2023-03-10      发布日期:  2023-03-14
ZTFLH:  TB333  
基金资助: 教育部“春晖计划”(HLJ2019007);哈尔滨理工大学杰出青年项目(LGYC2018JQ012);黑龙江省普通高校基本科研业务费专项资金(2019-KYYWF-0239)
通讯作者:  *高鑫,博士,哈尔滨理工大学材料科学与化学工程学院讲师、硕士研究生导师。2012年在哈尔滨理工大学毕业,获学士学位。2015年在哈尔滨理工大学毕业,获硕士学位。2019年在哈尔滨理工大学毕业,获博士学位。主要从事金属基复合材料和新型纳米材料等方面的研究工作,近年来在相关领域发表SCI论文12篇,授权发明专利4项。gaoxin6825@126.com
岳红彦,博士,哈尔滨理工大学材料科学与化学工程学院教授、博士研究生导师。2002年在哈尔滨理工大学毕业,获学士学位。2005年在哈尔滨理工大学毕业,获硕士学位。2009年在哈尔滨工业大学材料物理与化学专业博士毕业,获工学博士学位。2012—2013年和2016—2018年,分别在韩国成均馆大学和美国凯斯西储大学作为访问学者。主要从事石墨烯增强金属基复合材料、纳米生物传感器、纳米材料在生物医学中的应用和新型能源存储材料(超级电容器)等方面的研究工作。近年来,在ACS Nano、Advanced Functional Materials、Biosensors and Bioelectronics、Carbon、Sensors and Actuators B:Chemical和Materials and Design等期刊发表论文70余篇,授权国家发明专利22项。hyyue@hrbust.edu.cn   
作者简介:  俞彦飞,2016年6月毕业于哈尔滨理工大学,获得工学学士学位。2022年3月毕业于哈尔滨理工大学,获得工学硕士学位,主要研究领域为新型能源存储材料。
引用本文:    
俞彦飞, 王暄, 高鑫, 宁锋, 张浩鹏, 岳红彦. 基于定向冷冻技术构建的多孔材料及其应用[J]. 材料导报, 2023, 37(5): 21050074-11.
YU Yanfei, WANG Xuan, GAO Xin, NING Feng, ZHANG Haopeng, YUE Hongyan. Review of Porous Materials Derived from Using the Directional Freeze-casting Technique and Their Applications. Materials Reports, 2023, 37(5): 21050074-11.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.21050074  或          http://www.mater-rep.com/CN/Y2023/V37/I5/21050074
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