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材料导报  2020, Vol. 34 Issue (18): 18177-18182    https://doi.org/10.11896/cldb.19120179
  高分子与聚合物基复合材料 |
三种取代度不同的含辣素衍生结构功能单体对PSf/PES超滤膜性能的影响
张丽丽1, 唐媛媛1, 徐丽1, 单超越1, 于良民1,2
1 中国海洋大学海洋化学理论与工程技术教育部重点实验室, 青岛 266100
2 中国海洋大学海洋高等研究院,青岛 266100
Effects of Three Capsaicin Derivatives with Different Degrees on the Performance of PSf/PES Ultrafiltration Membranes
ZHANG Lili1, TANG Yuanyuan1, XU Li1, SHAN Chaoyue1, YU Liangmin1,2
1 Key Laboratory of Marine Chemistry Theory and Technology, Ministry of Education, Ocean University of China, Qingdao 266100, China
2 Institute for Advanced Ocean Study, Ocean University of China, Qingdao 266100, China
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摘要 以含辣素衍生结构功能单体为抗菌剂,以聚砜/聚醚砜为膜材料,以聚乙二醇400为致孔剂,以N, N-二甲基乙酰胺为溶剂,采用“微波原位聚合-相转化”法制备了含辣素衍生结构聚砜/聚醚砜抗菌超滤膜。考察了三种取代度不同的辣素单体对膜结构及性能的影响。研究结果表明,辣素单体的添加均使超滤膜的性能得到明显提升,且随着取代度的增加,改性超滤膜的力学性能逐渐增强,但单体取代度的不同对改性超滤膜的结构、渗透性、分离性能等并无明显影响。从研究结果可以看出,改性后的复合膜具有良好的抗菌性能,抑菌率高达89.5%。
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张丽丽
唐媛媛
徐丽
单超越
于良民
关键词:  辣素衍生结构  聚砜  聚醚砜  超滤  抗菌    
Abstract: The antibacterial ultrafiltration membranes were prepared via “MWA (microwave-assisted)-in situ polymerization-blending” method, using capsaicin derivatives as antibacterial additives, PSf/PES as membrane materials, polyethylene glycol 400 (PEG-400) as pore-forming agent and N, N-dimethyl acetamide (DMAc) as solvent. And the effects of functionality of different capsaicin derivatives on the structure and properties of the modified membranes were investigated. The results showed that the performance of the membranes modified with different capsaicin derivatives improved obviously. In addition, the mechanical properties of modified ultrafiltration membrane gradually strengthened with the functionality of capsaicin derivatives increased. However, the microstructure, permeability and separation performance had no apparent change as the change of the functionality. All the modified composite membrane had good antibacterial properties, up to 89.5%.
Key words:  capsaicin derivatives    polysulfone    polyethersulfone    ultrafiltration    antibacterial
                    发布日期:  2020-09-12
ZTFLH:  TQ326.55  
基金资助: 国家自然科学基金-山东联合基金(U1706225); 青岛海洋科学与技术国家实验室鳌山人才培养计划(2017ASTCP-OS02)
通讯作者:  yuyan@ouc.edu.cn   
作者简介:  张丽丽,2018年6月毕业于中国海洋大学,获得理学博士学位。同年加入中国海洋大学海洋化学理论与工程技术教育部重点实验室工作至今,主要从事防污超滤膜的制备及其在水处理中的应用研究。
于良民,中国海洋大学化学化工学院“长江学者”特聘教授,博士研究生导师,“环境友好型海洋功能材料与防护技术”科技部重点领域创新团队和教育部创新团队负责人,山东省暨青岛市腐蚀与防护学会监事长。研究方向/领域:环境友好型海洋防护材料与应用技术、先进高分子复合材料、类天然产物及其生态特性。
引用本文:    
张丽丽, 唐媛媛, 徐丽, 单超越, 于良民. 三种取代度不同的含辣素衍生结构功能单体对PSf/PES超滤膜性能的影响[J]. 材料导报, 2020, 34(18): 18177-18182.
ZHANG Lili, TANG Yuanyuan, XU Li, SHAN Chaoyue, YU Liangmin. Effects of Three Capsaicin Derivatives with Different Degrees on the Performance of PSf/PES Ultrafiltration Membranes. Materials Reports, 2020, 34(18): 18177-18182.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.19120179  或          http://www.mater-rep.com/CN/Y2020/V34/I18/18177
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