Recent Progress in Facets Regulation and Catalytic Antibacterial Activity of Low-dimensional ZnO Crystals
LI Dan, ZHANG Minhao, LIAO Peizi, XIE Yuan, ZHEN Hewei, XU Xiaoling, ZHOU Zuowan
Key Laboratory of Advanced Technologies of Materials (Ministry of Education), School of Materials Science and Engineering, Southwest Jiaotong University, Chengdu 610031
Abstract: As a kind of typical wide-band-gap semiconductor material, low dimensional zinc oxide (ZnO) has attracted increasing attention in long-term antibacterial, catalytic degradation and energy conversion, owing to its unique morphological adjustability, excellent catalytic activity and good biocompatibility. Sufficient research has indicated that, by changing the reaction conditions, the morphology and structure of ZnO can be easily tuned, which will further exert remarkable influence on properties and performance of ZnO. Therefore, the regulation of morphology and structure has been regarded as a crucial issue for the application of ZnO. The morphological diversification of ZnO originates from the anisotropic growth of its crystal. Many factors (like solvent, nucleating agent and additive agent etc.) may impact on this process and facilitate the growth of crystal along different crystal orientation. Therefore, the reaction condition determines both morphology and exposed crystal facet of ZnO. The atomic alignment, atomic density and surface dangling bonds vary consi-derably among different types of crystal facets. Hence, the performance of ZnO can be regulated by carefully control the morphology, structure, crystal orientation and exposed crystal surface. The continuous advancement of technology and simulation, the methodologies for facets regulation can be classified into crystal facets adsorption, seeding induction, solvent adjustment and crystal facets etching. The former three methods are bottom-up synthesis techniques, which achieve the control of crystal morphology and facets by either introducing adsorbents and/or seeds synthesis process, or carefully choosing appropriate solvent. On the other hand, crystal facets etching is a top-down process. The crystal facets of ZnO can be selectively etched because of the differences in reactive activity, which facilitates to obtain the required facets. These methods enable researchers to precisely regulate the crystal morphology and facet of the synthesized ZnO, and in consequence, to further study the relationship and mechanism between exposed crystal facets and catalytic antibacterial activity. In this review, we summarize the recent progress and the common methods, along with their action mechanisms, with respect to facets regulation of ZnO. The potential effects of crystal facets regulation on the catalytic antibacterial activity of ZnO with or without light irradiation are also explored. The paper ends with a discussion on the growing trends and emerging challenges in this field.
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2019, Vol. 33 
