Influence of Metal Organic Framework Materials Synthesis Method on the Adsorption Performance of Nitrogen Oxides
CUI Xinghui, WU Xiaopeng, QI Wenhao, XING Yiqiang, PAN Mengbo, DU Haoran, MA Chengliang
Henan Key Laboratory of High Temperature Functional Ceramics,School of Materials Science and Engineering, Zhengzhou University, Zhengzhou 450052, China
Abstract: Metal organic framework materials have good gas adsorption performance due to their high specific surface area and porosity. Compared with traditional NOx adsorption materials, MOFs have ultra-high specific surface area and porosity, rich and diverse structures and periodicity, and good thermal and chemical stability. The synthesis methods of MOFs have been studied a lot to get a high adsorption efficiency of NOx. The synthesis methods of MOFs mainly include hydrothermal method, solvothermal method, ultrasonic synthesis method and microwave synthesis method. The hydrothermal method has an easy operation and high crystal quality but a large crystal grains and small pore volume; The principles of the solvothermal method and the hydrothermal method are same. By adding organic solvents with different functional groups, the synthesized material can have a richer structure, larger specific surface area, and a better adsorption property on NOx than hydrothermal method. So it is also the most widely used method; the MOFs synthesized by ultrasonic synthesis method has small particle and uniform size,large specific surface area and pore volume, and good NOx adsorption property but high cost; the microwave synthesis method can accelerate the reaction process to get a smaller particle size, specific surface area and pore volume, and a high adsorption capacity for NOx, but it also has the disadvantage of high economic cost. Therefore, we summarize the synthesis methods and modification technologies of MOFs in this article, and analyze the effects of MOFs synthesized by different methods on the adsorption of NOx, and then prospecte the development trend of MOFs for adsorbing NOx.
1 王宗雄, 储荣邦. 表面工程资讯, 2011, 11(2), 3. 2 Matito-Martos I, Rahbari A, Martin-Calvo A, et al. Phyical Chemistry Chemical Physics, 2018, 20(6), 4189. 3 马现奇, 高旭东, 范永斌, 等. 中国水泥, 2019(5), 78. 4 Zengel D, Koch P, Torkashvand B, et al. Angewandte Chemie International Edition, 2020, 132(34), 11423. 5 Ye B, Kim J, Lee M J, et al. Microporous and Mesoporous Materials, 2021, 310, 110588. 6 Klose W, Rincon S. Fuel, 2007, 86(1-2), 203. 7 Perdana I, Creaser D, Hrman O, et al. Journal of Catalysis, 2005, 234(1), 219. 8 李娟娟. 吸附脱除低浓度一氧化氮的研究. 硕士学位论文, 大连理工大学, 2017. 9 Li H L, Eddaoudi M, O'Keeffe M, et al. Academic Journal, 1999, 402(6759), 4. 10 郭大为, 李倩, 陈西岩, 等.石油炼制与化工, 2012, 42(2), 9. 11 Xu Q, Fang L, Fu Y, et al. Materials Letters, 2020, 264, 127402. 12 Zhao X, Wang Y, Li D S, et al. Advanced Materials, 2018, 30(37), 1705189.1. 13 Kim K C. Journal of Organometallic Chemistry, 2018, 854, 94. 14 Chavan S, Vitillo J G, Gianolio D, et al. Physical Chemistry Chemical Physics, 2012, 14(5), 1614. 15 王丽苹, 赵粒成, 兰开顺, 等. 化学通报, 2017, 80(7) , 14. 16 Glomb S, Woschko D, Makhloufi G, et al. Acs Applied Materials & Interfaces, 2017, 9(42), 37419. 17 Petit C, Levasseur B, Mendoza B, et al. Microporous and Mesoporous Materials, 2012, 154, 107. 18 Yu J. Computational evaluation of metal-organic frameworks for CO2 capture. Ph.D.Thesis, Texas A&M University, USA, 2013. 19 Tan K, Zuluaga S, Gong Q, et al. Chemistry of Materials, 2015, 27(6), 2203. 20 Levasseur B, Petit C, Bandosz T J. ACS Applied Materials and Interfaces, 2010, 2(12), 3606. 21 Breedon M, Spencer M J S, Miura N. The Journal of Physical Chemistry C, 2013, 117(24), 12472. 22 Breedon M, Spencer M J S, Miura N. Chemical Physics Letters, 2014, 593, 61. 23 Liu Z S. Waste Management, 2008, 28(11), 2329. 24 Khan A H, Peikert K, Fröba M, et al. Microporous and Mesoporous Materials, 2015, 216, 111. 25 Meek S T, Greathouse J A, Allendorf M D. Advanced Materials, 2011, 23(2), 249. 26 Zheng N, Masel R I. Journal of the American Chemical Society, 2006, 128(38), 12394. 27 Seo Y K, Hundal G, Jang I T, et al. Microporous and Mesoporous Mate-rials, 2009, 119(1), 331. 28 Vaitsis C, Sourkouni G, Argirusis C. Ultrasonics sonochemistry, 2019, 52, 106. 29 Klimakow M, Klobes P, Thu Nemann A F, et al. Chemistry of Materials, 2010, 22(18), 5216. 30 乔萌, 牛建瑞, 钟为章, 等. 河北工业科技, 2018, 167(1), 74. 31 Chui S S Y, Lo S M F, Charmant J P H, et al. Science, 1999, 283(5405), 1148. 32 Yang S H, Sun J L, Ramirez-Cuesta A J, et al. Green Chemistry, 2012, 4(11), 887. 33 Ibarra I A, Bayliss P A, Pérez E, et al. Green Chemistry, 2012, 14(1), 117. 34 Han X, Godfrey H G W, Briggs L, et al. Nature Materials, 2018, 17(8), 691. 35 Nijem N, Bluhm H, Ng M L, et al. Chemical Communications Royal Society of Chemistry, 2014, 50(70), 10144. 36 Petit C, Bandosz T J. Dalton Transactions, 2012, 41(14), 4027. 37 Sava Gallis D F, Vogel D J, Vincent G A, et al. ACS Applied Materials and Interfaces, 2019, 11(46), 43270. 38 Gupta A, Kang S B, Harold M P. Catal. Today, 2021, 360, 411. 39 Bello E, Margarit V J, Gallego E M, et al. Microporous and Mesoporous Materials, 2020, 302, 110222. 40 Han X, Hong Y, Ma Y, et al. Journal of the American Chemical Society, 2020, 142(36), 15235. 41 Lu Z, Godfrey H G W, Da Silva I, et al. Nature Communications, 2017, 8, 14212. 42 Kyriakidou E A, Lee J, Choi J S, et al. Catal. Today, 2020, 360. 43 Li J, Han X, Zhang X, et al. Nature Chemistry, 2019, 11(12), 1085. 44 Xiang L, Blake A J, Wilson C, et al. Journal of the American Chemical Society, 2006, 128(33), 10745. 45 聂明, 陆顺, 李庆, 等.中国科学:化学, 2016, 46(4), 357. 46 Cavka J H, Jakobsen S R, Olsbye U, et al. Journal of the American Chemical Society, 2008, 130(42), 13850. 47 Ebrahim A M, Levasseur B, Bandosz T J. Langmuir, 2012, 29(1), 168. 48 Ebrahim A M, Bandosz T J. Microporous & Mesoporous Materials, 2014, 188, 149. 49 Wang Y, Ercan C, Khawajah A, et al. Aiche Journal, 2012, 58(3), 782. 50 Li B, Wen H-M, Wang H, et al. Energy & Environmental Science, 2015, 8(8), 2504. 51 Ebrahim A M, Bandosz T J. ACS Applied Materials and Interfaces, 2013, 5(21), 10565. 52 陈驰, 庞军, 韩爽, 等. 物理化学学报, 2012, 28(1), 189. 53 Wang L, Wang L, Zhao J, et al. Journal of Applied Physics, 2012, 111(11) , 112628. 54 Chae H K, Siberio-Pérez D Y, Kim J, et al. Nature, 2004, 427(6974), 523. 55 Caskey S R, Wong-Foy A G, Matzger A J. Journal of the American Che-mical Society, 2008, 130(33), 10870. 56 Tan K, Zuluaga S, Wang H, et al. Chemistry Materials, 2017, 29(10), 4227. 57 王玮, 吴云, 迟博伟. 化工设计通讯, 2016, 42(9), 32. 58 Bo X, Wheatley P S, Zhao X, et al. Journal of the American Chemical Society, 2007, 129(5), 1203. 59 侯吉聪.山东化工, 2019, 48(10), 81. 60 Petit C, Burress J, Bandosz T J. Carbon, 2011, 49(2), 563. 61 Seredych M, Bandosz T J. Journal of Physical Chemistry C, 2007, 111(43), 15596. 62 Decoste J B, Demasky T J, Katz M J, et al. New Journal of Chemistry, 2015, 39(4), 2396. 63 Katz M J, Brown Z J, Colon Y J, et al. Chemical Communications, 2013, 49(82), 9449. 64 张林建, 李芳芹, 任建兴, 等. 上海电力学院学报, 2019, 35(3), 267. 65 Thomas-Hillman I, Stevens L A, Lange M, et al. Green Chemistry, 2019, 21(18), 5039. 66 Peterson G W, Mahle J J, DeCoste J B, et al. Angewandte Chemie, 2016, 128 (21) , 6343.