稀土氟化物上转换纳米晶尺寸调控的研究进展

doi:10.11896/cldb.22110116

材料导报

2023, Vol. 37

Issue (3): 22110116-8 https://doi.org/10.11896/cldb.22110116

多尺度稀土晶体材料及其应用

稀土氟化物上转换纳米晶尺寸调控的研究进展

武素丽^*, 荀文斐, 张淑芬

大连理工大学智能材料化工前沿科学中心,精细化工国家重点实验室,辽宁大连 116024

Progress in Size-controlled Synthesis of Rare Earth Fluoride Upconversion Nanocrystals

WU Suli^*, XUN Wenfei, ZHANG Shufen

State Key Laboratory of Fine Chemicals, Frontier Science Center for Smart Materials, Dalian University of Technology, Dalian 116024, Liaoning, China

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摘要稀土掺杂的上转换发光材料是一类能够吸收低频率光子、发射高频率光子的反斯托克斯位移发光材料。镧系稀土氟化物NaREF₄是上转换效率最高的基质材料之一。该类材料由于具有荧光寿命长、背景干扰弱、组织穿透性强、化学稳定性高等优点,被广泛应用于显示与防伪、生物荧光标记、高性能传感器等领域。近年来,研究者发现通过尺寸控制可以有效改善NaREF₄材料的性能。本文详细介绍了可控地合成不同尺寸NaREF₄晶体的方法和影响因素,并概述了NaREF₄晶体尺寸对其发光性能的影响。

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	武素丽
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关键词: 上转换稀土纳米晶体尺寸调控

Abstract: Rare earth ions doped upconversion nanocrystals is a kind of material which can absorb low frequency photons and emit high frequency photons. Rare earth fluoride (NaREF₄) is considered to be a kind of most efficient matrix for rare earth doped upconversion material. Due to their long luminescence lifetime, low background interference, deep penetration and high stability, upconversion nanocrystals are widely used in the field of display and anticounterfeiting, biomarker, bioimaging and sensors. During recent years, researchers found that the performance of NaREF₄ based upconversion nanocrystals can be effectively improved by controlling their size. In this paper, the influence of the size of NaREF₄ crystals on its luminescent properties is summarized, and the size controllable synthesis methods of NaREF₄ are introduced in detail.

Key words: upconversion rare earth nanocrystal size control

出版日期: 2023-02-10 发布日期: 2023-02-23

ZTFLH:

基金资助: 国家自然科学基金(22178047;21878042);大连市科技创新基金(2020JJ26GX046)

通讯作者: ^*wusuli@dlut.edu.cn，武素丽,大连理工大学化工学院教授、博士研究生导师,1996年、1999年、2007年先后获大连理工大学学士、硕士、博士学位,曾在新加坡国立大学做访问学者一年。主要从事稀土掺杂上转换纳米材料、量子点、光子晶体及其在传感器、太阳能电池和显示设备中应用的研究。在Advanced Materials、ACS Nano、Advanced Functional Materials等期刊发表文章100余篇,撰写英文专著Long Afterglow Phosphorescent Materials一部,获得国际授权专利3项、国内授权专利10项。

引用本文:

武素丽, 荀文斐, 张淑芬. 稀土氟化物上转换纳米晶尺寸调控的研究进展[J]. 材料导报, 2023, 37(3): 22110116-8.
WU Suli, XUN Wenfei, ZHANG Shufen. Progress in Size-controlled Synthesis of Rare Earth Fluoride Upconversion Nanocrystals. Materials Reports, 2023, 37(3): 22110116-8.

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http://www.mater-rep.com/CN/10.11896/cldb.22110116 或 http://www.mater-rep.com/CN/Y2023/V37/I3/22110116

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