Recent Advances of Optical Tweezers and Its Prospect in Application of Cement-based Materials
ZHOU Yue1, ZHU Zheyu1, XU Linglin1,2, WANG Zhongping1,2, ZHOU Long1
1 School of Materials Science and Engineering, Tongji University, Shanghai 201804, China 2 Key Laboratory of Advanced Civil Engineering Materials, Ministry of Education, Tongji University, Shanghai 201804, China
Abstract: Calcium silicate hydrate (C-S-H), as the main hydration product of Portland cement, is limited by the ability of traditional characterization methods when establishing theoretical models. However, the information, which is used to establish the theoretical model like chemical composition and structural parameters, is based on the results of cement particle groups. Since the composition and structure of C-S-H are susceptible to the change of hydration condition, the average results need to be further optimized to accurately explain C-S-H. Optical tweezers technologyhave been used in single particle research of many fields, because it can capture small particles nondestructively. Introducing optical tweezers into the research of cement-based materials can manipulate the individual cement particle and observe its hydration, which is beneficial to achieving the precise control of cement hydration conditions and reducing the interaction effect between different particles. By using optical tweezers, morphological characteristics, composition and structure of C-S-H at the micro-nano scale can be directly explored under specific hydration conditions. This is of significance for establishing a theoretical model of C-S-H which is closer to the actual system.Optical tweezers have gone through three main development stages according to the difference of capture accuracy as follow: (i) Far-field optical tweezers are more suitable for capturing micron-sized particles. The capture objects mainly include microbial cells and gradually expand the field of organic and inorganic materials. (ii) Near-field optical tweezers are suitable for capturing micron and sub-micron particles. They break through the classical optical diffraction limit through the evanescent field of near field optics. (iii) Nano-aperture optical tweezers are based on the self-induced back-action (SIBA) effect, which increases the capture accuracy of optical tweezers to nanoscale. Nano-aperture optical tweezers can reduce the laser power, decrease the thermal damage and enrich the capture objects. At present, the capture medium of the three optical tweezers includes liquid, gas and vacuum, while the capture objects extend to organic particles, inorganic particles and metal particles, making it applied to the particles in various fields in theory. The parameters of optical tweezers to capture particles include many factors such as laser wavelength, beam power, capture medium and particle properties. For the particle, capture is mainly related to its refractive index. The larger the refractive index is, the more helpful it is to produce “pull force”(gradient force). This paper counts the properties of some particles that have been captured, and the refractive index ranges from 0.30 to 2.86. For cement particles, the refractive index is about 1.7. The capture medium of air will not affect cement hydration, and the laser power for capture is at milliwatt level which is not enough to damage the cement particles. Thus it is realizable to achieve the capture of cement particles stably. This paper reviews the research about optical tweezers. Their application objects, capture medium and capture accuracy are focused, and the application of optical tweezers in cement-based materials is explored.
作者简介: 周玥,2017年6月毕业于中国矿业大学,获得工学学士学位。现为同济大学材料科学与工程学院博士研究生,在王中平教授的指导下进行研究。目前主要研究领域为水泥基材料的组成与结构。 徐玲琳,同济大学材料科学与工程学院副教授。2013年6月博士毕业于同济大学材料科学与工程学院。2013年9月进入同济大学博士后流动站工作。2014年10月至2015年10月获中德博士后奖学金资助赴德国包豪斯大学开展博士后研究,2015年12月进入同济大学材料科学与工程学院工作。2015年入选同济大学青年优秀人才培养行动计划,先后主持国家自然科学基金项目、硅酸盐建筑材料国家重点实验室开放基金重点项目、先进土木工程材料教育部重点实验室项目等科研项目,并作为主要研究者参与“十一五”“十二五”科技支撑项目和国家自然科学基金等国家级项目的研究工作,在Cement and Concrete Research、Cement and Concrete Composites、Construction and Building Materials和《硅酸盐学报》等国内外学术期刊发表论文20余篇。
引用本文:
周玥, 朱哲誉, 徐玲琳, 王中平, 周龙. 光镊技术进展及其在水泥基材料中的应用展望[J]. 材料导报, 2022, 36(8): 20070147-7.
ZHOU Yue, ZHU Zheyu, XU Linglin, WANG Zhongping, ZHOU Long. Recent Advances of Optical Tweezers and Its Prospect in Application of Cement-based Materials. Materials Reports, 2022, 36(8): 20070147-7.
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2022, Vol. 36 
