应变工程对钙钛矿材料光电性质和稳定性的调制

doi:10.11896/cldb.20070095

材料导报

2022, Vol. 36

Issue (17): 20070095-9 https://doi.org/10.11896/cldb.20070095

无机非金属及其复合材料

应变工程对钙钛矿材料光电性质和稳定性的调制

王超, 严铮洸, 肖家文^*

北京工业大学材料与制造学部,固体微结构与性能研究所,固体微结构与性能北京市重点实验室,北京 100124

Modulating the Optoelectronic Properties and Stability of Perovskites by Strain Engineering

WANG Chao, YAN Zhengguang, XIAO Jiawen^*

Beijing Key Lab of Microstructure and Property of Advanced Materials, Institute of Microstructure and Property of Advanced Materials,Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing 100124, China

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摘要卤化物钙钛矿材料由于其优异的光电性质成为近几年的研究热点之一。钙钛矿太阳能电池的光电转换效率在短短几年内已超过25%,钙钛矿材料在光电二极管、光电探测器、激光器等光电器件中也表现出良好的应用前景。钙钛矿材料及器件性能和稳定性的进一步提高是研究人员重点关注的问题。各种改善钙钛矿材料的光电性质和稳定性的策略也被不断提出,如薄膜结晶控制、界面改性/缺陷钝化、组件工程、添加剂工程等。近年来,应变工程被发现可有效改善钙钛矿材料的光电性质和器件性能,为钙钛矿材料器件性能的优化提供了新的研究视角。本文从应力应变的基本概念入手,介绍了如何测量和评估钙钛矿材料的残余应力和应变、残余应力和应变如何影响钙钛矿材料的器件性能,以及总结了对钙钛矿材料施加应力和应变的策略,最后本文对应变工程改善钙钛矿材料的器件性能这一新的研究视角做出展望。

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	王超
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关键词: 卤化物钙钛矿应力-应变稳定性光电性质

Abstract: Halide perovskite materials have been one of the hottest topics in recent years due to their excellent optoelectronic properties. This upsurge was initially caused by perovskite solar cells, whose power conversion efficiency has exceeded 25% in just a few years. The halide perovskite materials also show huge potential in light-emitting devices, photodetectors, lasers and other optoelectronic devices. The further improvement of perovskite materials and device performance and stability is the key issue of researchers. Various strategies to improve the optoelectronic properties and stability of perovskite materials have also been proposed, such as film crystallization control, interface modification/defect passivation, component engineering, additive engineering, etc. In recent years, strain engineering has been found to be able to effectively improve the optoelectronic properties and device performance of halide perovskites, which provides a novel avenue for the optimization of device performance of perovskite materials. In this review, we start with the basic concept of stress and strain, then describe how to measure and evaluate the residual stress and strain of perovskite materials, as well as how residual stress and strain affect the device performance and the underlying mechanism, and summarize the strategy of applying stress and strain to perovskite material. Finally, the new research perspective of strain engineering to improve the device performance of perovskite materials is prospected.

Key words: halide perovskite stress-strain stability optoelectronic property

出版日期: 2022-09-10 发布日期: 2022-09-10

ZTFLH:

O472

基金资助: 国家自然科学基金(11674015;21701009);北京市卓越青年科学家项目(BJJWZYJH01201910005018)

通讯作者: ^*xiaojw@bjut.edu.cn

作者简介: 王超,硕士研究生。2019年本科毕业于北京化工大学材料科学与工程学院,2019年9月起于北京工业大学固体微结构与性能研究所攻读硕士学位。目前主要研究方向为卤化物钙钛矿器件的光电性能与稳定性研究。
肖家文,北京工业大学固体微结构与性能研究所,博士,副研究员。2010年7月本科毕业于北京师范大学化学学院,2015年7月在北京大学无机化学专业取得博士学位,2016—2019年在北京理工大学材料学院进行博士后研究工作。2019年5月入职北京工业大学固体微结构与性能研究所。长期从事贵金属、半导体纳米材料的溶液法合成及其光电性能、器件应用的研究。以第一作者在Advanced Energy Materials、Nano Energy、Nanoscale、Solar RRL、Chemistry-A European Journal等杂志上发表多篇论文,他引170余次。以合作者身份在JACS、ACS Nano、Small等杂志发表多篇论文。

引用本文:

王超, 严铮洸, 肖家文. 应变工程对钙钛矿材料光电性质和稳定性的调制[J]. 材料导报, 2022, 36(17): 20070095-9.
WANG Chao, YAN Zhengguang, XIAO Jiawen. Modulating the Optoelectronic Properties and Stability of Perovskites by Strain Engineering. Materials Reports, 2022, 36(17): 20070095-9.

链接本文:

http://www.mater-rep.com/CN/10.11896/cldb.20070095 或 http://www.mater-rep.com/CN/Y2022/V36/I17/20070095

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