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材料导报  2023, Vol. 37 Issue (17): 21110116-12    https://doi.org/10.11896/cldb.21110116
  无机非金属及其复合材料 |
氨硼烷水解制氢催化剂的研究进展
韦秋红, 褚海亮*, 夏永鹏, 邱树君, 温鑫, 徐芬, 孙立贤
桂林电子科技大学材料科学与工程学院,广西电子信息材料构效关系重点实验室,广西 桂林 541004
Progress in Catalysts for Hydrolytic Dehydrogenation of Ammonia Borane
WEI Qiuhong, CHU Hailiang*, XIA Yongpeng, QIU Shujun, WEN Xin, XU Fen, SUN Lixian
Guangxi Key Laboratory of Information Materials, School of Materials Science and Engineering, Guilin University of Electronic Technology, Guilin 541004, Guangxi, China
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摘要 近年来,氢能已成为全球公认的清洁能源之一,氢能的高效利用有利于缓解能源短缺和环境污染等问题。在适当的催化剂作用下可以实现氨硼烷(NH3BH3,AB)水解反应的可控放氢,其因具有反应条件温和、环境友好等特点而备受关注,选择高活性的催化剂是提高氨硼烷水解制氢效率的关键。本文介绍了氨硼烷的结构、性质及合成方法,综述了氨硼烷水解制氢催化剂的最新研究进展,介绍了催化剂的分类及特点,指出了该领域中面临的挑战和未来研发重点。
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韦秋红
褚海亮
夏永鹏
邱树君
温鑫
徐芬
孙立贤
关键词:  氨硼烷  水解  制氢  催化剂    
Abstract: Hydrogen has been recognized as the green energy source and the use of hydrogen energy technologies has gained considerable attention from worldwide researchers and industries. The efficient utilization of hydrogen can be beneficial to the alleviation of global issues such as energy crisis and environment pollution. The catalyzed hydrolytic dehydrogenation of ammonia borane (NH3BH3, AB) is a potential route to the controllable generation of hydrogen. This catalytic reaction also has the advantages of mild reaction conditions and environmental friendliness, which make it one of the research hotspots in the field of hydrogen energy. Catalyst is a crucial factor determining the hydrogen generation efficiency of ammonia borane. This review includes an introduction of the structure, properties and synthesis of ammonia borane, a comprehensive description of the recent progress in the research of relevant catalysts with high (or potentially high) activities, as well as a brief discussion on challenges and future development trends.
Key words:  ammonia borane    hydrolysis    dehydrogenation    catalysts
出版日期:  2023-09-10      发布日期:  2023-09-05
ZTFLH:  TB34  
基金资助: 广西自然科学基金(2020GXNSFAA297047);中央引导地方科技发展资金项目(桂科ZY21195038);国家自然科学基金(52101245; 22179026; 21965007; 52161035; U20A20237);桂林电子科技大学研究生教育创新计划资助项目(2022YCXS195);广西新能源材料结构与性能协同创新中心;广西八桂学者项目
通讯作者:  *褚海亮,桂林电子科技大学材料科学与工程学院教师、博士研究生导师,广西杰出青年基金获得者,中国仪表功能材料学会储能与动力电池及其材料专业委员会委员和全国材料与器件网理事会理事。2008年毕业于中国科学院大连化学物理研究所,获理学博士学位,随后留所工作,2012年调入桂林电子科技大学材料科学与工程学院,2014年在加拿大魁北克大学氢能研究所作访问学者。长期从事新能源材料领域的研究,以研发高容量氢气制备/储存材料与电化学储能材料为主要研究方向。已发表100余篇SCI收录论文,授权中国发明专利10余项。chuhailiang@guet.edu.cn   
作者简介:  韦秋红,2020年6月于桂林电子科技大学获得工学学士学位。现为桂林电子科技大学材料科学与工程学院硕士研究生,在褚海亮研究员的指导下进行研究。目前主要研究领域为新能源材料。
引用本文:    
韦秋红, 褚海亮, 夏永鹏, 邱树君, 温鑫, 徐芬, 孙立贤. 氨硼烷水解制氢催化剂的研究进展[J]. 材料导报, 2023, 37(17): 21110116-12.
WEI Qiuhong, CHU Hailiang, XIA Yongpeng, QIU Shujun, WEN Xin, XU Fen, SUN Lixian. Progress in Catalysts for Hydrolytic Dehydrogenation of Ammonia Borane. Materials Reports, 2023, 37(17): 21110116-12.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.21110116  或          http://www.mater-rep.com/CN/Y2023/V37/I17/21110116
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