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材料导报  2021, Vol. 35 Issue (21): 21085-21090    https://doi.org/10.11896/cldb.21060276
  环境催化材料 |
铁含量对Fe-P-C非晶合金降解亚甲基蓝性能的影响
马娅娅1,2, 李强1,2, 穆保霞1,2, 马旭1,2
1 新疆大学新疆固态物理与器件重点实验室,乌鲁木齐 830046
2 新疆大学物理科学与技术学院,乌鲁木齐 830046
Effect of Iron Content on the Degradation of Methylene Blue in Fe-P-C Amorphous Alloy
MA Yaya1,2, LI Qiang1,2, MU Baoxia1,2, MA Xu1,2
1 Xinjiang Key Laboratory of Solid State Physics and Devices, Xinjiang University, Urumqi, 830046, China
2 School of Physics Science and Technology, Xinjiang University, Urumqi 830046, China
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摘要 本文制备了四种不同铁含量的Fe80+2xP10-xC10-x(x=0, 1, 2, 3 (原子分数,%))非晶合金条带,通过类芬顿反应催化降解亚甲基蓝(Methylene blue,MB)溶液对它们性能的影响进行比较研究,探讨铁含量对铁基非晶合金降解性能的影响。结果表明,目前Fe-P-C非晶合金条带通过类芬顿反应降解MB表现出优异的性能,且铁含量越高,降解性能越好,但当铁含量超过82%后,铁含量对降解性能的影响不显著。由表面形貌观察可知,随着Fe含量的增加,反应后的Fe-P-C非晶条带表面呈现更加疏松多孔的结构,这有利于获得高的降解效率。循环降解测试显示,四种不同铁含量Fe-P-C非晶合金条带的降解性能差别不大,且均具有较长的使用寿命,这可能与降解过程中形成具有松散片层状结构和3D花状网格结构的表面形态有关。X射线电子能谱分析结果表明,Fe含量的不同并不影响Fe-P-C非晶合金的降解反应机理。
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马娅娅
李强
穆保霞
马旭
关键词:  铁基非晶合金  类芬顿反应  亚甲基蓝(MB)  降解    
Abstract: In this work, four kinds of Fe80+2xP10-xC10-x(x=0,1,2,3, at%) amorphous alloy ribbons with different Fe contents were prepared. The catalytic degradation of methylene blue (MB) solution by Fe80+2xP10-xC10-x(x=0,1,2,3, at%) amorphous alloy ribbons was studied by Fenton-like reaction. The results show that Fe-P-C amorphous alloy ribbons exhibit excellent degradation performance of MB solution by Fenton-like reaction, and the higher the iron content, the better the degradation performance. However, when the iron content exceeds 82at%, the effect of iron content on the degradation performance is not obvious.The surface morphology observation showed that with the increase of Fe content, the surface of the Fe-P-C amorphous ribbon after reaction showed a more porous structure, which was beneficial to obtain high degradation efficiency. The cyclic degradation test shows that the four Fe-P-C amorphous alloys with different iron contents have little difference and have long service life, which may be related to the formation of surface morphology with loose lamellar structure and 3D flower-like grid structure during the degradation process. The results of X-ray electron energy spectrum analysis showed that the different Fe content did not affect the degradation reaction mechanism of Fe-P-C amorphous alloy.
Key words:  Fe-based amorphous alloys    Fenton-like reaction    methylene blue(MB)    degradation
               出版日期:  2021-11-10      发布日期:  2021-11-30
ZTFLH:  TG139+.8  
基金资助: 国家自然科学基金(51771161)
通讯作者:  qli@xju.edu.cn   
作者简介:  马娅娅,2021年6月毕业于新疆大学,获得工学硕士学位。研究生期间主要从事铁基非晶合金催化性能的研究。
李强,新疆大学教授,博士研究生导师,享受国务院政府特殊津贴。2002年毕业于香港中文大学,获博士学位。2005年进入新疆大学物理科学与技术学院工作至今,主要研究方向包括大过冷态下的合金相变、块体非晶态合金和纳米合金的制备及其性能研究等。自入职新疆大学以来,共主持国家自然科学基金项目5项,在学术期刊发表SCI论文60余篇。
引用本文:    
马娅娅, 李强, 穆保霞, 马旭. 铁含量对Fe-P-C非晶合金降解亚甲基蓝性能的影响[J]. 材料导报, 2021, 35(21): 21085-21090.
MA Yaya, LI Qiang, MU Baoxia, MA Xu. Effect of Iron Content on the Degradation of Methylene Blue in Fe-P-C Amorphous Alloy. Materials Reports, 2021, 35(21): 21085-21090.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.21060276  或          http://www.mater-rep.com/CN/Y2021/V35/I21/21085
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