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材料导报  2023, Vol. 37 Issue (8): 21060242-9    https://doi.org/10.11896/cldb.21060242
  高分子与聚合物基复合材料 |
地聚物的耐高温性能研究进展
宋天诣1, 曲星宇1, 潘竹2,3,*
1 北京工业大学城市建设学部,北京 100124
2 河北工业大学土木与交通学院,天津 300401
3 天津市装配式建筑与智能建造重点实验室,天津 300401
Research Progress on High Temperature Performance of Geopolymers
SONG Tianyi1, QU Xingyu1, PAN Zhu2,3,*
1 Faculty of Architecture, Civil and Transportation Engineering, Beijing University of Technology, Beijing 100124, China
2 School of Civil Engineering and Transportation, Hebei University of Technology, Tianjin 300401, China
3 Tianjin Key Laboratory of Prefabricated Buildings and Smart Construction, Tianjin 300401, China
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摘要 地聚物是一种使用工业固废作为原料的新型绿色环保建筑材料。固废中含有的铝硅酸盐玻璃体在高碱性条件下经缩聚反应可形成无定型态的硅铝网状类沸石立体结构,从而使地聚物具有类陶瓷的特性,改善其耐高温性能。近年来,地聚物的耐高温性能成为绿色建材领域研究热点。
地聚物混凝土是一种多相复合材料,其原料来源多样且配制过程中需要控制的参数较为复杂,这些因素都导致地聚物混凝土在高温下(后)抗压强度变化的多样性。近年来,研究者们开展了大量试验和理论分析工作,发现影响地聚物混凝土高温下(后)抗压强度的三个主要影响因素是:(1)晶相转变;(2)微观结构变化;(3)地聚物和骨料的位移不相容性。地聚物混凝土在高温下(后)的抗压强度最终取决于三个主要因素中占主导的因素和混凝土延性。
本文着重探讨了硅铝原子比、碱溶液类型和骨料对地聚物混凝土高温下(后)抗压强度的影响规律,结合三种影响因素分析了地聚物混凝土的抗压强度劣化机理,同时对地聚物的热工性能和地聚物混凝土结构的耐火性能进行了综述。最后,对地聚物材料耐高温性能的未来研究前景进行了讨论。
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宋天诣
曲星宇
潘竹
关键词:  地聚物  地聚物混凝土结构  高温  热工性能  抗压强度    
Abstract: Geopolymers are a kind of emerging cementitious materials that provide an environmentally alternative to ordinary Portland cement (OPC) based concrete. Compared with OPC concrete, the benefits of geopolymers are mainly based on their ability to bring high volume ratio of industrial wastes into construction products. Generated via the dissolution and polycondensation reaction of aluminosilicate vitreous in industrial waste under high alkaline conditions, geopolymers possess the zeolite-like network structures in which aluminum and silica tetrahedrally interlink alternately by sharing all the oxygen atoms. The formation of this three-dimensional structure leads to ceramic-like properties. Therefore, geopolymers are generally considered to provide excellent fire resistance, and research in this field has been attracting increasing interest in recent years.
Geopolymeric concrete is a multiphase composite material, and its composition has wide variations. The orthotropic nature of the constituent materials results in the variation of high-temperature performance. Owing to the considerable research efforts, it has been recognized that there are mainly three factors which can affect compressive strength of geopolymeric concrete (exposed to high temperature): (Ⅰ) phase transition; (Ⅱ) microstructure changes; (Ⅲ) thermal incompatibility of geopolymer matrix and aggregates. The compressive strength of geopolymeric concrete under (or experienced) high temperatures depends on the dominant factor and the material's ductility.
In this paper, the influence of Si/Al ratio, type of alkali solution and aggregates on the compressive strength of geopolymeric concrete under (and after experiencing) high temperatures are discussed. Combined with three factors, the compressive strength degradation mechanisms of geopolymeric concrete is analyzed. The paper also summarizes the thermal performance of geopolymers and the fire resistance of geopolymeric concrete structures. Finally, the future research prospect of high temperature performance of geopolymers is discussed.
Key words:  geopolymer    geopolymeric concrete structure    high temperature    thermal property    compressive strength
出版日期:  2023-04-25      发布日期:  2023-04-24
ZTFLH:  TU528  
基金资助: 国家自然科学基金(U20A20313;51778018, 52178444);河北省自然科学基金重点项目(E2019202484)
通讯作者:  *潘竹,河北工业大学土木与交通学院教授、博士研究生导师。2012年6月在澳大利亚蒙纳什大学(Monash University)土木工程系取得结构工程专业博士学位,2014年7月至2018年12月在澳大利亚西悉尼大学(Western Sydney University)进行博士后研究工作。长期从事高性能绿色胶凝材料的形成机理和耐高温性能研究,主持澳大利亚国家级项目2项、国家自然科学基金联合基金重点项目1项(在研)。在Cement and Concrete Research、Cement and Concrete Compo-sites、Journal of Cleaner Production、Materials and Design、Applied Energy和Composites Part B: Engineering等SCI期刊上发表论文27篇。其中两篇为该领域ESI高被引文章。所发表成果被SCI论文引用超过1 400次,H因子17。zhu.pan@hebut.edu.cn   
作者简介:  宋天诣,北京工业大学城市建设学部副教授、博士研究生导师。2011年1月博士毕业于清华大学土木工程系结构工程专业,2016年入选北京市第十二批海外高层次人才“海聚工程青年项目”,目前兼任中国钢结构协会防火与防腐分会理事、中国土木工程学会工程防火技术分会理事、中国建筑学会抗震防灾分会结构抗火专业委员会委员。主要从事钢-混凝土组合结构和新型混凝土材料耐火性能等方面的研究。已发表中英文学术论文50余篇,出版专著1部,参编国家标准1部、建筑工业行业或地方标准7部。
引用本文:    
宋天诣, 曲星宇, 潘竹. 地聚物的耐高温性能研究进展[J]. 材料导报, 2023, 37(8): 21060242-9.
SONG Tianyi, QU Xingyu, PAN Zhu. Research Progress on High Temperature Performance of Geopolymers. Materials Reports, 2023, 37(8): 21060242-9.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.21060242  或          http://www.mater-rep.com/CN/Y2023/V37/I8/21060242
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