锂离子电池用纳米碳材料研究进展

doi:10.11896/cldb.21050286

材料导报

2022, Vol. 36

Issue (20): 21050286-13 https://doi.org/10.11896/cldb.21050286

无机非金属及其复合材料

锂离子电池用纳米碳材料研究进展

张佰伦¹, 王凯¹, 李嘉辉¹, 钟海长², 张文魁¹, 章文献², 梁初^1,2,*

1 浙江工业大学材料科学与工程学院&浙江碳中和创新研究院,杭州 310014
2 福建省功能材料及应用重点实验室,福建厦门 361024

Progress in Carbon Nanomaterials for Lithium-ion Batteries

ZHANG Bailun¹, WANG Kai¹, LI Jiahui¹, ZHONG Haichang², ZHANG Wenkui¹, ZHANG Wenxian², LIANG Chu^1,2,*

1 College of Materials Science and Engineering & Zhejiang Carbon Neutral Innovation Institute, Zhejiang University of Technology, Hangzhou 310014, China
2 Fujian Provincial Key Laboratory of Functional Materials and Applications, Xiamen 361024, Fujian, China

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摘要锂离子电池作为最有前景的储能器件之一,已经在便携式电子设备上广泛应用。然而使用传统电极材料,电池的能量密度和功率密度不够高、耐久性差、成本高,限制了其在电动汽车等方面的大规模应用。纳米碳材料的发展为设计适合锂离子电池的新型储能材料提供了机会。纳米碳材料作为一种新型碳材料具有许多独特的性能,包括独特的形貌结构、高比表面积、低扩散距离、高电导率和离子导电性能、可控的合成和掺杂等优点。因此,纳米碳材料在高可逆容量、高功率密度、长循环稳定性和高安全性锂离子电池中具有较大的应用前景。
然而,纳米碳材料普遍存在首次库仑效率低、电压滞后等缺点,且纳米碳材料的电化学性能取决于碳材料的形貌和微观结构。解决这一问题最常用的方法主要有:(1)通过对纳米碳材料的形貌和微结构调控来改善其电化学性能;(2)通过异质原子掺杂改善纳米碳材料的电化学性能;(3)将纳米碳与其他储锂材料复合形成复合电极材料。
本文主要综述了富勒烯、石墨烯、碳纳米管和多孔碳等四种具有代表性的纳米碳材料在锂离子电池中的最新研究进展,系统归纳了纳米结构和形貌对电化学性能的影响,讨论了纳米碳的合成、电化学储锂性能和电极反应机理。本文还对纳米碳材料未来在锂离子电池应用中需要解决的关键问题进行了总结与展望。

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关键词: 纳米碳锂离子电池富勒烯石墨烯碳纳米管多孔碳

Abstract: As one of the most promising energy storage devices, lithium-ion batteries have been widely used in portable electronic devices. However, the inadequate energy density and power density, poor durability and high cost, which are resulted from using traditional electrode materials, limit the large-scale applications of lithium-ion batteries in electric vehicles. The development of carbon nanomaterials provides an opportunity for the new energy storage materials applied in lithium-ion batteries. Nanocarbons have many unique characteristics, including unique morphology and microstructure, high specific surface area, low diffusion distance, high electronic and ionic conductivity, controllable synthesis and doping, etc. Therefore, nanocarbons have great application prospects in the field of lithium-ion batteries with high reversible capacity, high power density, good cycle stability and high safety.
However, nanocarbons as electrode materials exhibit low initial Coulombic efficiency and large voltage hysteresis during charging/discharging. Moreover, the electrochemical performance of nanocarbons is dependent on their morphology and microstructure. The following strategies are proposed to solve these problems: (Ⅰ) improving the electrochemical performance by adjusting the morphology and microstructure of nanocarbons; (Ⅱ) improving electrochemical performance by doping heteroatoms into nanocarbons; (Ⅲ) combining nanocarbons with other materials to form carbon-based composites for high-performance lithium storage.
The recent progress of nanocarbon materials in lithium-ion batteries, typically represented by fullerene, graphene, carbon nanotubes and po-rous carbon is reviewed in this paper. The influence of nano-size and morphology on the electrochemical performance of nanocarbons is also summarized. The synthesis of nano-carbon, lithium-ion battery performance and electrode reaction mechanism are emphasized. The purpose of this paper is to summarize the recent progress of carbon nanomaterials in the lithium-ion batteries and their key fundamental problems to be solved in the future.

Key words: nanocarbon lithium-ion battery fullerene graphene carbon nanotube porous carbon

发布日期: 2022-10-26

ZTFLH:

TM911

基金资助: 国家自然科学基金(52072342;51677170);浙江省自然科学基金(LY19E010007);福建省功能材料及应用重点实验室开放基金(fma2020003)

通讯作者: ^*cliang@zjut.edu.cn

作者简介: 张佰伦,2018年6月毕业于井冈山大学,获得工学学士学位。现为浙江工业大学材料科学与工程学院硕士研究生,在梁初教授指导下从事碳材料的合成机理和储能应用研究。
梁初,浙江工业大学材料科学与工程学院&浙江碳中和创新研究院教授。2011年6月在浙江大学材料科学与工程学系取得博士学位,2011—2013年在浙江大学材料科学与工程学系从事博士后研究工作。2014入职浙江工业大学,其中2018—2019年前往美国马里兰大学帕克分校材料科学与工程学系进行访问交流。近年来,主要从事碳中和技术与新材料的基础理论和应用开发研究工作,在Nature Communications、Advanced Energy Materials、Small、Journal of Materials Chemistry A等期刊发表SCI学术论文110余篇。

引用本文:

张佰伦, 王凯, 李嘉辉, 钟海长, 张文魁, 章文献, 梁初. 锂离子电池用纳米碳材料研究进展[J]. 材料导报, 2022, 36(20): 21050286-13.
ZHANG Bailun, WANG Kai, LI Jiahui, ZHONG Haichang, ZHANG Wenkui, ZHANG Wenxian, LIANG Chu. Progress in Carbon Nanomaterials for Lithium-ion Batteries. Materials Reports, 2022, 36(20): 21050286-13.

链接本文:

http://www.mater-rep.com/CN/10.11896/cldb.21050286 或 http://www.mater-rep.com/CN/Y2022/V36/I20/21050286

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