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材料导报  2022, Vol. 36 Issue (11): 21010142-5    https://doi.org/10.11896/cldb.21010142
  无机非金属及其复合材料 |
熔盐辅助制备钛酸锶钡纳米粉体及其介电性能
唐滋励1, 夏浚淞1, 尹航1, 傅光辉1, 艾细彤1, 唐海龙1,2
1 重庆理工大学材料科学与工程学院,重庆 400054
2 重庆市高校模具技术重点实验室,重庆 400054
Preparation of Barium Strontium Titanate Nanopowders Using Molten Salt Assisted and Its Dielectric Properties
TANG Zili1, XIA Junsong1, YIN Hang1, FU Guanghui1, AI Xitong1, TANG Hailong1,2
1 College of Materials Science and Engineering, Chongqing University of Technology, Chongqing 400054, China
2 Chongqing Key Laboratory of Mold Technology, Chongqing 400054, China
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摘要 采用溶胶沉淀法并结合熔盐辅助热处理,通过调节钡锶物质的量比制备了一系列纳米钛酸锶钡(Ba1-xSrxTiO3,x=0.1、0.33、0.5、0.74、0.8)粉体。通过X射线衍射仪(XRD)、扫描电子显微镜(SEM)、介电常数测试仪等测试手段,分析反应产物晶体结构,表征产物微观形貌并研究其介电性能。结果表明:钛酸锶钡纳米粉体具有钙钛矿型结构,且颗粒形貌为四方形或球形,平均粒径为70~100 nm,其中Ba0.9Sr0.1TiO3、Ba0.67Sr0.33-TiO3具有四方钙钛矿结构。1 kHz时Ba0.67Sr0.33TiO3样品的介电常数高达1 680,介电损耗为0.043,居里温度为27.3 ℃。
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唐滋励
夏浚淞
尹航
傅光辉
艾细彤
唐海龙
关键词:  钛酸锶钡  溶胶沉淀法  熔盐辅助  介电性能    
Abstract: Barium strontium titanate (Ba1-xSrxTiO3,x=0.1,0.33,0.5,0.74,0.8) nanopowders were synthesized by adjusting the molar ratio of barium to strontium via simple sol-precipitation method combined with heat treatment with molten salt. The morphology, structure and dielectric pro-perties of Ba1-xSrxTiO3 were characterized by scanning electron microscope (SEM), X-ray diffractometer (XRD) and dielectric constant tester. The results reveal that the Ba1-xSrxTiO3 nanopowders show a well-defined perovskite crystal structure and square or spherical morphology with average size of 70—100 nm. Moreover, Ba0.9Sr0.1TiO3 and Ba0.67Sr0.33TiO3 exhibit a tetragonal perovskite structure. The dielectric constant and dielectric loss of Ba0.67Sr0.33TiO3 at 1 kHz reach 1 680 and 0.043 respectively, and the curie temperature is 27.3 ℃.
Key words:  barium strontium titanate    sol-precipitation method    molten salt assisted    dielectric property
发布日期:  2022-06-09
ZTFLH:  TB34  
基金资助: 重庆市自然科学基金(cstc2018jcyjAX0565);重庆市留学人员回国创业创新支持计划(cx2018132);重庆市研究生科研创新项目(CYS20353);重庆市高校创新研究群体项目(CXQT19027)
通讯作者:  hailong.tang@cqut.edu.cn   
作者简介:  唐滋励,硕士。本科毕业于江苏理工学院功能材料专业,硕士毕业于重庆理工大学材料工程专业,主要从事纳米功能材料及聚芳醚腈基纳米复合材料的研究。
唐海龙,博士,重庆理工大学副教授、硕士研究生导师。本科毕业于电子科技大学应用化学专业,硕士及博士毕业于电子科技大学材料科学与工程专业(硕博连读)。主要研究方向为特种工程塑料及其先进复合材料、荧光功能材料及其传感检测应用、耐高温介电材料等,已发表SCI学术论文40余篇,并出版学术专著1部。
引用本文:    
唐滋励, 夏浚淞, 尹航, 傅光辉, 艾细彤, 唐海龙. 熔盐辅助制备钛酸锶钡纳米粉体及其介电性能[J]. 材料导报, 2022, 36(11): 21010142-5.
TANG Zili, XIA Junsong, YIN Hang, FU Guanghui, AI Xitong, TANG Hailong. Preparation of Barium Strontium Titanate Nanopowders Using Molten Salt Assisted and Its Dielectric Properties. Materials Reports, 2022, 36(11): 21010142-5.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.21010142  或          http://www.mater-rep.com/CN/Y2022/V36/I11/21010142
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