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材料导报  2023, Vol. 37 Issue (19): 22020093-15    https://doi.org/10.11896/cldb.22020093
  无机非金属及其复合材料 |
氧化物固体电解质的三维框架结构设计及在全固态锂离子电池中的应用
陈斐1,2,*, RannalterLeana Ziwen2, 宋尚斌1,2, 曹诗雨1,2, 沈强2
1 武汉理工大学深圳研究院,广东 深圳 518063
2 武汉理工大学材料复合新技术国家重点实验室,武汉 430070
Three-dimensional Structural Design in Oxide Solid Electrolytes and Its Application in All-Solid-State Lithium-ion Batteries
CHEN Fei1,2,*, Rannalter Leana Ziwen2, SONG Shangbin1,2, CAO Shiyu1,2, SHEN Qiang2
1 Shenzhen Research Institute of Wuhan University of Technology, Shenzhen 518063, Guangdong, China
2 State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China
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摘要 相比于传统锂离子电池,全固态锂电池在安全性、能量密度和工作温度范围等方面具有显著优势,研究并开发固体电解质是突破锂电池的技术瓶颈和进一步产业化发展的关键步骤。针对目前聚合物复合电解质中的颗粒填料团聚以及固体电解质/电极界面中存在的问题,该领域涌现了一批具有创新性的无机固体电解质结构设计。本文首先对基于三维氧化物固体电解质框架的复合电解质中的离子传输途径进行了概括性的讨论,阐述了电解质的结构可能对离子传输带来的影响。文章重点介绍了近年来对氧化物固体电解质的三维框架结构设计和应用及其制备方法,详述了不同的电解质框架结构对电池电化学性能方面的优化策略并对电池性能进行了比较。三维电解质框架除了可以作为复合电解质的基体外,也可以将电极材料填入其中,使其作为复合电极的基体,为电极与电解质之间提供了一种新的接触形式,以解决电极的体积变化和锂枝晶生长问题。文章在最后对设计思路以及仍面临的挑战进行了总结。
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陈斐
RannalterLeana Ziwen
宋尚斌
曹诗雨
沈强
关键词:  复合固体电解质  三维框架  锂离子电导率  全固态电池  多孔材料    
Abstract: Due to the advantages of all-solid-state lithium batteries in safety, energy density and working temperature range, the development of solid electrolytes is a crucial step to breaking through the technical bottleneck of lithium batteries and further industrialization. Because of the problems of filler particle agglomeration in composite electrolytes and electrolyte/electrode interfaces, several innovative inorganic electrolyte designs have recently been proposed. This review paper begins with a brief discussion of ion transport pathways in a composite electrolyte based on a three-dimensional oxide solid electrolyte framework, describing the effects that the electrolyte structure may have on ion transport. The designs and application of different types of 3D framework structures of oxide solid electrolyte reported in recent years, together with their preparation methods are then highlighted. We also detail the optimization strategies of the different designs of the structure for the electrochemical perfor-mance of the batteries and make a comparison between them. The 3D oxide solid electrolyte framework can not only be used as the matrix of composite electrolyte but also be filled with electrode materials to form a composite electrode, which provides a new contact form between the electrode and the electrolyte, aiming to solve the problems of volume change and lithium dendrite growth. At the end of this review, the design ideas and ongoing challenges are summarized.
Key words:  composite solid electrolyte    three-dimensional framework    Li+ conductivity    all-solid-state lithium battery    porous material
出版日期:  2023-10-10      发布日期:  2023-09-28
ZTFLH:  TM912  
基金资助: 广东省基础与应用基础研究重大项目(2021B0301030001);深圳市科技计划项目(JCYJ20190809153405505);国家自然科学基金项目(51972246;51521001);国家重点研发计划 (2018YFB0905600);中央高校基本科研业务费专项资金;“111” 工程 (B13035)
通讯作者:  *陈斐,武汉理工大学教授、博士研究生导师。2004年6月在武汉理工大学获得工学学士学位,2009年6月在武汉理工大学获得工学博士学位。长期从事功能梯度材料及其在能量转换与存储中的应用研究。主持国家重点研发计划、国家自然科学基金、中央军委科技委创新特区项目装备预研领域基金等10余项科研项目。获国家发明专利21项,发表研究论文150余篇,包括Nature Energy、Journal of Power Sources、ACS Applied Nano Mate-rials、ACS Applied Materials Interfaces、Journal of the American Ceramic Society等。chenfei027@whut.edu.cn   
引用本文:    
陈斐, RannalterLeana Ziwen, 宋尚斌, 曹诗雨, 沈强. 氧化物固体电解质的三维框架结构设计及在全固态锂离子电池中的应用[J]. 材料导报, 2023, 37(19): 22020093-15.
CHEN Fei, Rannalter Leana Ziwen, SONG Shangbin, CAO Shiyu, SHEN Qiang. Three-dimensional Structural Design in Oxide Solid Electrolytes and Its Application in All-Solid-State Lithium-ion Batteries. Materials Reports, 2023, 37(19): 22020093-15.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.22020093  或          http://www.mater-rep.com/CN/Y2023/V37/I19/22020093
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