固体表面液滴定向运动行为研究进展

doi:10.11896/cldb.19070008

材料导报

2020, Vol. 34

Issue (13): 13175-13193 https://doi.org/10.11896/cldb.19070008

高分子与聚合物基复合材料

固体表面液滴定向运动行为研究进展

胡海豹, 曹刚, 张梦卓, 杜鹏, 黄潇

西北工业大学航海学院, 西安 710072

Research Advance on Directional Motion Behavior of Solid Surface Droplets

HU Haibao, CAO Gang, ZHANG Mengzhuo, DU Peng, HUANG Xiao

School of Marine Science and Technology, Northwestern Polytechnical University, Xi’an 710072, China

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摘要液滴在固体表面定向运动极具研究价值,目前被广泛应用于水收集、油水分离、微流控、自清洁等领域,已成为表界面领域的研究热点。同时,液滴定向运动行为研究对理解液体与固体表面之间的作用机制具有重要意义。
然而,目前对液滴定向运动的研究主要集中在宏观尺度观测与分析方面,缺乏对基本原理的深入探索,并且对实现液滴定向运动的基本条件认识不足。同时,人造仿生材料存在工艺复杂、成本高昂,以及运动距离相对较短、运动速度相对较小等缺点,限制了其适用范围。另外,虽然广大学者在液滴定向运动行为研究方面已经取得了较多成果,比如制得微型混合器、流体二极管等,但这些研究仅局限在实验室阶段,如何将其广泛应用于日常生活仍有待进一步研究。
目前,学者们从液滴润湿性基本原理出发,发现仙人掌、猪笼草、瓶子草、蜘蛛丝、蝴蝶等天然材料表面可以实现液滴定向运动,其中,瓶子草绒毛表面液滴定向运动速度高达(1 1738±715) μm·s^-1。在此基础上,广大学者通过静电纺丝、电化学腐蚀、光刻法、浸涂法等方式对仙人掌刺、猪笼草口缘、瓶子草绒毛、蜘蛛丝等做了进一步的仿生研究,其中仿蜘蛛丝实现了液滴的可逆运动和高效水收集。此外,受天然材料表面液滴定向运动启发,有学者研制了可实现液滴快速、长距离、方向可控运动的拓扑流体二极管,而结构简单的箭头状微结构更是为实际应用提供了可能。
本文全面综述了近10年国内外学者在仙人掌、猪笼草、瓶子草、蜘蛛丝及蝴蝶等天然材料表面液滴定向运动行为方面的研究进展,从表面能梯度、Laplace压力梯度及毛细力等角度分析了固体表面液滴定向运动的基本原理,同时展示了国内外在仿生定向运动表面的典型研究实例。最后,对该领域未来的研究工作提出了一些建议。

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关键词: 液滴固体表面定向运动仿生

Abstract: The directional motion of droplets on solid surfaces is of great research value and has been widely used in water collection, oil-water separation, microfluidics, etc., which has become a research hotspot in the field of surface interface. At the same time, the study of droplet orientation motion behavior is of great significance for understanding the mechanism of action between liquid and solid surfaces.
However, the current research on the directional movement of droplets mainly focuses on macroscopic scale observation and analysis, lacks in-depth exploration of the basic principles and lacks understanding of the basic conditions for achieving droplet directional motion. At the same time, the current artificial biomimetic materials are complicated and costly, and their relatively short moving distance and relatively small moving speed limit their application range. In addition, although the majority of scholars have made great achievements in the research of droplet directional motion behavior, such as micro-mixers, fluid diodes, etc., these studies are only limited to the “laboratory” stage, applying it widely to daily life needs further research.
Fortunately, the current scholars have started from the basic principle of droplet wetting and found that the surface of natural materials such as cactus, Nepenthes alata, Sarracenia,spider silk and butterfly,etc. can realize the directional movement of droplets. And the directional movement speed of droplets on the surface of Sarracenia trichome is up to (1 1738±715) μm·s^-1. On this basis, the majority of scholars have made further biomimetic research on cactus spine, Nepenthes alata peristome, Sarracenia trichome,spider silk, etc. by electrospinning, electrochemical etching, photolithography, dip-coating, etc.,and the biomimetic spider silk achieves reversible movement of the droplets and efficient water collection. In addition, inspired by the directional movement of droplets on the surface of natural materials, some scholars have developed topological fluid diodes that realize rapid, long-distance and direction-controllable movement of droplets. The simple arrow-shaped microstructures provide a possibility for practical applications.
This paper comprehensively reviews the recent research progress of domestic and foreign scholars on the surface directional movement beha-vior of natural materials such as cactus, Nepenthes alata, Sarracenia, spider silk and butterfly. The basic principle of directional movement of so-lid surface droplets is analyzed from the angle of force, and a typical example of bionic self-orienting surface at home and abroad is demonstrated. Finally, some suggestions for future research work are presented.

Key words: droplet solid surface directional motion bionic

发布日期: 2020-06-24

ZTFLH:	O647.11
	O647.5

基金资助: 国家自然科学基金(51879218; 51679203);中央高校基本科研业务费专项资金(3102018gxc007);国防科技工业海洋防务技术创新中心创新基金;西北工业大学研究生创意创新种子基金(CX2020062)

通讯作者: huhaibao@nwpu.edu.cn

作者简介: 胡海豹, 教授, 博士研究生导师, 2005年 4 月在西北工业大学航海学院参加工作。西北工业大学学士 (2002)、硕士 (2005)、工学博士 (2009)。曾入选西工大“翱翔之星”、“优秀青年教师”、“优秀研究生指导教师”。长期致力于特种表面力学行为与机制研究工作,累计获得省部级科技奖2项,发表学术论文50余篇,授权发明专利10多项。

引用本文:

胡海豹, 曹刚, 张梦卓, 杜鹏, 黄潇. 固体表面液滴定向运动行为研究进展[J]. 材料导报, 2020, 34(13): 13175-13193.
HU Haibao, CAO Gang, ZHANG Mengzhuo, DU Peng, HUANG Xiao. Research Advance on Directional Motion Behavior of Solid Surface Droplets. Materials Reports, 2020, 34(13): 13175-13193.

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http://www.mater-rep.com/CN/10.11896/cldb.19070008 或 http://www.mater-rep.com/CN/Y2020/V34/I13/13175

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