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材料导报  2023, Vol. 37 Issue (23): 22080136-9    https://doi.org/10.11896/cldb.22080136
  无机非金属及其复合材料 |
电子束辐照改善材料表面润湿性能的研究进展
王力1,2, 王海斗1,3,*, 底月兰2,*, 何东昱2, 黄艳斐2
1 哈尔滨工程大学材料科学与化学工程学院,哈尔滨 150090
2 陆军装甲兵学院装备再制造技术国防科技重点实验室,北京 100072
3 陆军装甲兵学院机械产品再制造国家工程研究中心,北京 100072
A Technological Review of the Use of Electron Beam Irradiation for Modifying Materials Surface Wettability
WANG Li1,2, WANG Haidou1,3,*, DI Yuelan2,*, HE Dongyu2, HUANG Yanfei2
1 College of Materials Science and Chemical Engineering, Harbin Engineering University, Harbin 150090, China
2 Key Laboratory of National Defense Science and Technology for Equipment Remanufacturing Technology, Army Armored of Forces Academy, Beijing 100072, China
3 National Engineering Research Center for Remanufacturing, Army Armored of Forces Academy， Beijing 100072, China
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摘要 电子束辐照植入官能团具有均匀和可控修饰等优势,已经被广泛应用于改变表面能、改善材料表面润湿性能,但是关于电子束与材料表面相互作用以及改性表面润湿性能机制尚无明确的解释。因此本文主要针对电子束辐照改性材料表面性能进行研究,总结当前电子束与材料表面相互作用机制,发现电子束与材料表面相互作用主要有弹性相互作用和非弹性相互作用。当电子束能量超过材料损伤阈值时,电子束辐照会改变材料表面形貌,并且通过交联和接枝反应在聚合物之间产生新的化学键(如碳基、羟基和羧基等)或使材料表面形成氧化层,导致表面能的改变。电子束辐照改性表面的润湿性能与诸多因素有关,如电子能量、电子剂量、材料种类和复合工艺等。电子束辐照可以提高或者降低材料表面润湿性能,通过控制电子辐照参数,达到精确调整表面润湿性能的目的。电子束辐照作为一种简单、快速改善材料表面润湿性能的新工艺,复合其他工艺制备特殊功能的超疏水表面具有发展前景。
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王力
王海斗
底月兰
何东昱
黄艳斐
关键词:  电子束辐照  表面自由能  润湿性能  复合工艺    
Abstract: Electron beam irradiation offers the advantages of uniformity and controllability over implanted functional groups. It has been widely used to change the surface energy and modify the surface wetting properties of materials. However, the mechanisms of interaction between the electron beam and material surface and the modification of the wettability have not been clearly elucidated. Accordingly, this work primarily focuses on the surface properties under electron beam irradiation. The mechanism is explained by elastic and inelastic interactions. When the electron beam energy exceeds the damage threshold of a material, electron beam irradiation changes the surface morphology of the material. The generation of new polar groups such as carbon, hydroxyl, and carboxyl groups between polymers or the formation of oxide layers on modified surfaces by cross-linking and grafting reactions leads to changes in the surface energy. The wettability modification of the surface under electron beam irradiation is attributed to many factors, such as the electron energy, electron dose, material type, and composite process. Electron beam irradiation can increase or decrease the surface wettability of the material, and can be precisely adjusted by controlling the electron irradiation parameters. Electron irradiation, as a novel process for the simple and rapid modification of the surface wettability, has a promising future in the preparation of hydrophobic surfaces with specific functions by an electron beam irradiation composite process.
Key words:  electron beam irradiation    surface free energy    wetting property    composite process
出版日期:  2023-12-10      发布日期:  2023-12-08
ZTFLH:  V261.6+2  
基金资助: 国家自然科学基金(52175207);国防科技领域基金项目
通讯作者:  * 王海斗,陆军装甲兵学院机械产品再制造国家工程研究中心主任,2003年博士毕业于清华大学机械工程系。目前的研究领域包括表面工程、再制造和摩擦学。已发500余篇论文。whaidou2021@163.com;底月兰,陆军装甲兵学院装备再制造技术国防科技重点实验室助理研究员,2013年博士毕业于陆军装甲兵学院,研究领域为表面工程与再制造工程,功能涂层表面改性方向。已发30余篇论文。dylxinjic031@163.com   
作者简介:  王力,2021年毕业于江西理工大学,获得硕士学位。现为哈尔滨工程大学博士研究生,主要研究方向为金属材料功能表面改性。
引用本文:    
王力, 王海斗, 底月兰, 何东昱, 黄艳斐. 电子束辐照改善材料表面润湿性能的研究进展[J]. 材料导报, 2023, 37(23): 22080136-9.
WANG Li, WANG Haidou, DI Yuelan, HE Dongyu, HUANG Yanfei. A Technological Review of the Use of Electron Beam Irradiation for Modifying Materials Surface Wettability. Materials Reports, 2023, 37(23): 22080136-9.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.22080136  或          http://www.mater-rep.com/CN/Y2023/V37/I23/22080136
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