MOFs基核壳结构电磁波吸收材料研究进展

doi:10.11896/cldb.21030206

材料导报

2022, Vol. 36

Issue (16): 21030206-10 https://doi.org/10.11896/cldb.21030206

金属与金属基复合材料

MOFs基核壳结构电磁波吸收材料研究进展

姜超, 华楚侨, 温变英^*

北京工商大学化学与材料工程学院,北京 100048

Overview of Electromagnetic Wave Absorbing Materials with Core-Shell Structure Based on MOFs

JIANG Chao, HUA Chuqiao, WEN Bianying^*

College of Chemistry and Materials Engineering, Beijing Technology and Business University, Beijing 100048, China

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摘要电子设备的广泛应用在给人们生活带来方便的同时也造成了严重的电磁干扰和电磁辐射污染问题。开发更轻、更薄、吸收频率更宽的高效电磁波吸收材料,对维持设备的正常运行和保障人们的身体健康具有重要意义。
金属-有机骨架(Metal-organic frameworks,MOFs)材料是由金属离子或金属团簇与有机配体结合形成的一维或多维结构的一类化合物。MOFs具有超大的比表面积、有序的可进入空腔以及可调的组成和结构等特点,通过对其进行高温煅烧可以制备出具有特殊微观结构的轻质多孔碳材料,其中包含了因煅烧而产生的金属和金属氧化物纳米粒子。此种多孔碳材料因具有丰富的电磁损耗机制而拥有了优异的吸波性能和吸收带宽,因而受到了研究者的关注。
本文从结构、性能和制备方法等方面综述了MOFs基核壳结构吸波材料在电磁波吸收领域的研究进展。首先介绍了不同MOFs基核壳结构吸波材料的微观结构及其吸波性能和机理,然后归纳了不同类型MOFs基核壳结构吸波材料的制备方法,最后对目前MOFs基核壳结构吸波材料制备和应用中亟待解决的问题进行了总结,以期为MOFs在电磁波吸收领域的研究和应用提供参考。

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	姜超
	华楚侨
	温变英

关键词: 金属有机骨架核壳结构吸波材料制备方法

Abstract: The wide application of electronic equipment brings convenience to people's life but also causes serious problems of electromagnetic interfe-rence and electromagnetic radiation pollution. Therefore, the development of lighter, thinner and more efficient electromagnetic wave absorbing materials with a wider absorption frequency is of great significance to maintain the normal operation of the equipment and protect the health of the people.
The metal-organic frameworks (MOFs) are a kind of compound that combine metal ions or metal clusters with organic ligands to form one-dimensional or multi-dimensional structures. MOFs are characterized by extra large specific surface area, ordered accessible cavities, tunability of composition and structure. By calcining MOFs at high temperature, light porous carbon-based materials with unique microstructure can be prepared, which contain metal and metal oxide nanoparticles produced by calcination. Such porous carbon-based materials possess excellent wave absorption performance and absorption bandwidth due to their rich electromagnetic loss mechanism, which has attracted the attention of researchers.
In this paper, the research progress of MOFs-based core-shell structure absorbing materials used in the field of electromagnetic wave absorption is reviewed from the perspectives of structure, performance and preparation methods. Firstly, the microstructures, electromagnetic wave absorption performances and the corresponding absorbing mechanism of different MOFs-based composites are introduced. And then, their preparation methods are summarized. Finally, the current problems that need to be solved of the electromagnetic wave absorbing materials with core-shell structures based on MOFs are overviewed. It is expected to provide a reference for the research and application of such composites in the field of electromagnetic wave absorption.

Key words: metal-organic frameworks core-shell structure wave-absorbing material preparation method

出版日期: 2022-08-25 发布日期: 2022-08-29

ZTFLH:

TB34

基金资助: 北京市自然科学基金暨北京市教委科技计划重点项目(KZ202110011018)

通讯作者: ^*wenbianying@tsinghua.org.cn

作者简介: 姜超,2018年毕业于北京工商大学高分子材料与工程专业,获得工学学士学位。现为北京工商大学化学材料与工程学院硕士研究生,在温变英教授的指导下进行研究。目前主要研究领域为MOFs基吸波材料。温变英,北京工商大学化学与材料工程学院教授,北京市高等学校教学名师。1984年和1998年在中北大学分别获得学士和硕士学位,2003年博士毕业于北京化工大学,2003—2005年在清华大学进行博士后研究。主要从事高分子材料与功能复合材料研究。已在国内外重要学术期刊发表学术论文140余篇。21030206-21030206-

引用本文:

姜超, 华楚侨, 温变英. MOFs基核壳结构电磁波吸收材料研究进展[J]. 材料导报, 2022, 36(16): 21030206-10.
JIANG Chao, HUA Chuqiao, WEN Bianying. Overview of Electromagnetic Wave Absorbing Materials with Core-Shell Structure Based on MOFs. Materials Reports, 2022, 36(16): 21030206-10.

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http://www.mater-rep.com/CN/10.11896/cldb.21030206 或 http://www.mater-rep.com/CN/Y2022/V36/I16/21030206

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