Review on CO2 Mineralization, Sequestration and Utilization of Cement-based Materials
LI Linkun1,2, LIU Qi1, HUANG Tianyong3, LI Yang3, PENG Bo1
1 Beijing Key Laboratory for Greenhouse Gas Storage and CO2-EOR, the Unconventional Petroleum Research Institute, China University of Petroleum-Beijing, Beijing 102249, China 2 CNOOC Energy Conservation & Pollution Reduction Monitoring Center Co., Ltd., Tianjin 300457, China 3 State Key Laboratory of Green Building Materials, Beijing Building Materials Academy of Sciences Research, Beijing 100041, China
Abstract: In order to mitigate the negative impact of CO2 emissions from cement production on the global climate change, CO2 was sequestered in cement-based materials in the form of inorganic carbonate by utilizing the mineralization reaction between CO2 and cementitious materials containing Ca2+ and Mg2+ and their hydration products based on carbon capture, storage and utilization (CCUS) technology. Meanwhile, due to the good stability, filling effect and nucleation effect of its mineralized products (mainly calcium carbonate and amorphous SiO2), the mechanical properties and durability of cement-based materials after CO2 mineralization were effectively improved, and the cement-based materials with high performance were obtained in a short time. This paper reviews currently primary methodologies for the mineralization of CO2 in cement-based material. First, we discuss the reaction characteristics of different cementitious materials and CO2 in the maintenance process of concrete. Second is property improvement of recycled concrete aggregate by mineral carbonation. The CO2 mineralization and utilization technology to improve the mechanical performance of concrete and the quality of recycled concrete aggregate in detail in the perspectives of micro-mechanisms, factors influencing reaction kinetics and CO2 absorption are introduced emphatically. Finally, based on current research status and existing problems, the future development and research direction for CO2 mineralization of cement-based material are also proposed.
作者简介: 李林坤,2019年5月毕业于长春工业大学,获得工学学士学位。现为中国石油大学(北京)非常规油气科学技术研究院硕士研究生,在刘琦副教授的指导下进行研究。目前主要研究领域为低碳能源工程。 刘琦,中国石油大学(北京)非常规油气科学技术研究院副教授、博士研究生导师。2007年7月本科毕业于中国矿业大学(北京),2012年7月在英国诺丁汉大学化学工程专业取得博士学位,2012—2015年在英国赫瑞瓦特大学进行博士后研究工作。主要从事油气田化学工程和低碳能源工程的研究工作。近年来,在该领域发表论文20余篇,包括Chemical Engineering Science、Journal of cleaner production、Journal of Petroleum Science and Engineering和Journal of CO2 Utilization等。
引用本文:
李林坤, 刘琦, 黄天勇, 李扬, 彭勃. 基于水泥基材料的CO2矿化封存利用技术综述[J]. 材料导报, 2022, 36(19): 20100295-9.
LI Linkun, LIU Qi, HUANG Tianyong, LI Yang, PENG Bo. Review on CO2 Mineralization, Sequestration and Utilization of Cement-based Materials. Materials Reports, 2022, 36(19): 20100295-9.
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2022, Vol. 36 
