事故容错锆包壳表面FeCrAl合金涂层的研究进展

doi:10.11896/cldb.22110325

材料导报

2024, Vol. 38

Issue (12): 22110325-11 https://doi.org/10.11896/cldb.22110325

金属与金属基复合材料

事故容错锆包壳表面FeCrAl合金涂层的研究进展

王亚恒, 左家栋, 王亚强^*, 张金钰, 吴凯, 刘刚, 孙军

西安交通大学金属材料强度国家重点实验室,西安 710049

Research Progress of FeCrAl Coatings on Accident-Tolerant Zircaloy Cladding Surface

WANG Yaheng, ZUO Jiadong, WANG Yaqiang^*, ZHANG Jinyu, WU Kai, LIU Gang, SUN Jun

State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an 710049, China

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摘要日本福岛核事故暴露出了核燃料包壳锆合金在失水事故工况下的致命缺陷,即锆水反应,同时也引发了高安全事故容错燃料(ATF)包壳材料的研究热点。表面涂层技术是一种有效提升现役锆合金包壳事故容错能力的重要途径,其中FeCrAl合金涂层由于具有优异的抗高温氧化性能和高温力学性能,是极具发展潜力的ATF包壳涂层候选材料之一。本文主要综述了FeCrAl合金涂层的制备工艺、成分组织、服役性能(力学、氧化、腐蚀、辐照)及失效机制,并对锆合金包壳/FeCrAl涂层体系在工程应用中存在的问题和未来的发展方向进行了分析与展望。

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关键词: 锆合金包壳表面技术 FeCrAl涂层微观组织服役性能失效机制

Abstract: The Fukushima nuclear accident in Japan exposed the fatal deficiency of zircaloy fuel cladding under loss of coolant accident (LOCA) conditions, i.e., the reaction of zirconium with high-temperature steam. As a result, a research focus on the accident tolerant fuel (ATF) cladding materials with high security was triggered rapidly. Surface coating technologies provide a promising avenue for effectively improving the accident tolerance of zircaloy cladding in service. FeCrAl alloy, due to its excellent oxidation resistance and mechanical properties at high temperatures, becomes one of the candidate coating materials with great development potential for ATF claddings. This paper mainly reviewed the preparation technologies, composition and microstructure, service performances (including mechanical properties, oxidation resistance, corrosion resistance and anti-irradiation), and the relevant failure mechanisms of FeCrAl alloy coating. Moreover, the existed problems of FeCrAl coating/zircaloy cladding system in the engineering applications were also discussed, with prospecting the future direction of development.

Key words: zircaloy cladding surface technology FeCrAl coatings microstructure service performances failure mechanisms

出版日期: 2024-06-25 发布日期: 2024-07-17

ZTFLH:

TG178

基金资助: 国家自然科学基金(U2067219;U20B2027;52001247;92163201);博士后创新人才支持计划项目 (BX20190266)

通讯作者: *王亚强,西安交通大学材料科学与工程学院副教授、硕士研究生导师。分别于2012年和2019年获得西安交通大学材料科学与工程专业学士学位与博士学位,毕业后留校工作至今。目前主要从事高性能核燃料包壳金属涂层材料的研发及应用、金属纳米薄膜材料的变形断裂与强韧化等研究工作。发表论文60余篇,包括Acta Materialia、Advanced Materials、Scripta Materialia等。yaqiangwang@xjtu.edu.cn

作者简介: 王亚恒,2020年6月于河南科技大学获得工学学士学位。现为西安交通大学材料科学与工程学院硕士研究生。目前主要研究领域为包壳涂层的界面特性和高温氧化性能。

引用本文:

王亚恒, 左家栋, 王亚强, 张金钰, 吴凯, 刘刚, 孙军. 事故容错锆包壳表面FeCrAl合金涂层的研究进展[J]. 材料导报, 2024, 38(12): 22110325-11.
WANG Yaheng, ZUO Jiadong, WANG Yaqiang, ZHANG Jinyu, WU Kai, LIU Gang, SUN Jun. Research Progress of FeCrAl Coatings on Accident-Tolerant Zircaloy Cladding Surface. Materials Reports, 2024, 38(12): 22110325-11.

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http://www.mater-rep.com/CN/10.11896/cldb.22110325 或 http://www.mater-rep.com/CN/Y2024/V38/I12/22110325

1 Lei Y M. Design, synthesis and properties of protective coatings for accident tolerant fuels. Ph. D. Thesis, University of Science and Technology of China, China, 2021(in Chinese).
雷一明. 几种事故容错燃料包壳涂层的设计、制备与性能研究. 博士学位论文, 中国科学技术大学, 2021.
2 Rickover H G, Geiger L D, Lustman B. Energy Research and Development Administration, DOI:10.2172/4240391.
3 Gadiyar H. In: Proceedings of Symposium on Zirconium Alloys For Reactor Components. Bhabha Atomic Research Centre:Bombay, 1992, pp.149.
4 Cox B. Journal of Nuclear Materials, 2005, 336(2), 331.
5 Kashkarov E, Afornu B, Sidelev D, et al. Coatings, 2021, 11(5), 557.
6 Bischoff J, Delafoy C, Vauglin C, et al. Nuclear Engineering and Technology, 2018, 50(2), 223.
7 Kim H G, Yang J H, Kim W J. Nuclear Engineering and Technology, 2016, 48(1), 1.
8 Cheng B, Chou P, Kim Y J. EPJ Nuclear Sciences & Technologies, 2016, 2, 1.
9 Terrani K A, Zinkle S J, Snead L L. Journal of Nuclear Materials, 2014, 448(1), 420.
10 Yueh K, Terrani K A. Journal of Nuclear Materials, 2014, 448(1), 380.
11 Liu J K, Zhang X H, Yun D. Materials Reports, 2018, 32(11), 1757. (in Chinese)
刘俊凯, 张新虎, 恽迪. 材料导报, 2018, 32(11), 1757.
12 Baek J H, Jeong Y H. Journal of Nuclear Materials, 2008, 372(2), 152.
13 Kim H G, Hwan J Y. Nuclear Engineering and Technology, 2010, 42(2), 193.
14 Duan Z G, Yang H L, Satoh Y, et al. Nuclear Engineering and Design, 2017, 316, 131.
15 Maier B R, Garcia-Diaz B L, Hauch B, et al. Journal of Nuclear Mate-rials, 2015, 466, 712.
16 Usui T, Sawada A, Amaya M, et al. Journal of Nuclear Science and Technology, 2015, 52(10), 1318.
17 Xiao W W, Deng H, Zou S L, et al. Journal of Nuclear Materials, 2018, 509, 542.
18 Wang X J, Liu Y H, Feng S, et al. Chinese Journal of Vacuum Science and Technology, 2018, 38(4), 332. (in Chinese)
王晓婧, 刘艳红, 冯硕, 等. 真空科学与技术学报, 2018, 38(4), 332.
19 Tang C C, Steinbrueck M, Stueber M, et al. Corrosion Science, 2018, 135, 87.
20 Dong Y, Ge F F, Meng F P, et al. Surface & Coatings Technology, 2018, 350, 841.
21 Dong Y. Preparation and oxidation in high-temperature steam of Cr-AI-Si(-N) protective coatings coated on Zr alloys. Master's Thesis, Chengdu University of Technology, China, 2018 (in Chinese).
董悦. Zr合金表面Cr-Al-Si(-N)防护涂层的制备及其抗高温水蒸气氧化研究. 硕士学位论文, 成都理工大学, 2018.
22 Xiao X, Wang Y Q, Zhang J Y, et al. Materials China, 2022, 41(6), 445(in Chinese).
肖珣, 王亚强, 张金钰, 等. 中国材料进展, 2022, 41(6), 445.
23 Kim H G, Kim I H, Jung Y I, et al. Journal of Nuclear Materials, 2015, 465, 531.
24 Zhong W C, Mouche P A, Heuser B J. Journal of Nuclear Materials, 2018, 498, 137.
25 Yeom H, Maier B, Johnson G, et al. Journal of Nuclear Materials, 2018, 507, 306.
26 Yeom H, Maier B, Johnson G, et al. Journal of Nuclear Materials, 2019, 526, 151737.
27 Yang H Y, Zhang R Q, Peng X M, et al. Surface Technology, 2017, 46(1), 69(in Chinese).
杨红艳, 张瑞谦, 彭小明, 等. 表面技术, 2017, 46(1), 69.
28 He L X, Liu C H, Lin J H, et al. Journal of Nuclear Materials, 2021, 551, 152966.
29 Yang H Y, Chen Q S, Zhang R Q, et al. Nuclear Power Engineering, 2020, 41(S1), 200(in Chinese).
杨红艳, 陈青松, 张瑞谦, 等. 核动力工程, 2020, 41(S1), 200.
30 Wang Y D, Zhou W C, Wen Q L, et al. Surface & Coatings Technology, 2018, 344, 141.
31 Li T, Liu T. Nuclear Power Engineering, 2019, 40(4), 65(in Chinese).
李锐, 刘彤. 核动力工程, 2019, 40(4), 65.
32 Jr C V K, Dennis H, Phillip L, et al. Journal of Thermal Spray Techno-logy, 2005, 14(3), 330.
33 Shang C. China Steel Focus, 2021(5), 35(in Chinese).
尚灿. 冶金管理, 2021(5), 35.
34 Chen Q S. Investigation of the preparation and accident-tolerant properties of metal coating on zirconium alloy. Master's Thesis, Chengdu University of Technology, China, 2020(in Chinese).
陈青松. 锆合金表面事故容错金属涂层的制备及相关性能研究. 硕士学位论文, 成都理工大学, 2020.
35 Yamamoto Y, Field K G, Snead L L. Iaea Tecdoc Series, 2016, 47(29), 47080117.
36 Zhang Y Y, Sun H Y, Wang H, et al. Materials Science & Engineering A, 2021, 826, 142003.
37 Yamamoto Y, Pint B A, Terrani K A, et al. Journal of Nuclear Mate-rials, 2015, 467, 703.
38 Huang X, Li X Y, Fang X D, et al. Journal of Materials Engineering, 2020, 48(3), 19(in Chinese).
黄希, 李小燕, 方晓东, 等. 材料工程, 2020, 48(3), 19.
39 Satoru K, Takayuki T. Scripta Materialia, 2010, 63(11), 1104.
40 Kim I H, Jung Y I, Kim H G, et al. Surface & Coatings Technology, 2021, 411, 126915.
41 Zhong W C, Mouche P A, Han X C, et al. Journal of Nuclear Materials, 2016, 470, 327.
42 Gigax J G, Kennas M, Kim H, et al. Journal of Nuclear Materials, 2019, 519, 57.
43 Josefsson H, Liu R, Svensson J E, et al. Materials and Corrosion, 2005, 56(11), 801.
44 Badini C, Laurella F. Surface & Coatings Technology, 2001, 135(2), 291.
45 Yin L, Jurewicz T. B, Larsen M, et al. Journal of Nuclear Materials, 2021, 554, 153090.
46 Zhou J, Qiu S Y, Du P N, et al. Materials Reports, 2017, 31(S2), 47(in Chinese).
周军, 邱绍宇, 杜沛南, 等. 材料导报, 2017, 31(S2), 47.
47 Field K G, Hu X X, Littrell K C, et al. Journal of Nuclear Materials, 2015, 465, 746.
48 Field K G, Briggs S A, Sridharan K, et al. Journal of Nuclear Materials, 2017, 489, 118.
49 Lei Y, Zhang H S, Mao J J, et al. Nuclear Power Engineering, 2022, 43(1), 97(in Chinese).
雷阳, 张海生, 毛建军, 等. 核动力工程, 2022, 43(1), 97.
50 Deng P, Peng Q J, Han E H, et al. Corrosion Science, 2017, 127, 91.
51 Wang P, Grdanovska S, Bartels D M, et al. Journal of Nuclear Mate-rials, 2020, 533, 152108.
52 Hao S Z, Zhao L M, He D Y. Nuclear Instruments and Methods in Physics Research Section B, 2013, 312, 97.
53 Haley J C, Briggs S A, Edmondson P D, et al. Acta Materialia, 2017, 136, 390.
54 Jiang G Y, Xu D H, Feng P, et al. Journal of Alloys and Compounds, 2021, 869, 159235.
55 Ackland G. Science, 2010, 327(5973), 1587.
56 Yutani K, Kishimoto H, Kasada R, et al. Journal of Nuclear Materials, 2007, 367, 423.
57 Rebak R B. EPJ Nuclear Sciences & Technologies, 2017, 3, 34.
58 Alat E, Motta A T, Comstock R J, et al. Surface & Coatings Technology, 2015, 281, 133.
59 Zhang W, Tang R, Yang Z B, et al. Surface & Coatings Technology, 2018, 347, 13.
60 Pint B A, Terrani K A, Brady M P, et al. Journal of Nuclear Materials, 2013, 440(1), 420.

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