负载型贵金属催化剂氧化分解甲醛的研究进展

材料导报

2020, Vol. 34

Issue (Z1): 400-407

金属与金属基复合材料

负载型贵金属催化剂氧化分解甲醛的研究进展

李世杰, 黄慧娟, 文世涛, 马建锋, 刘杏娥

国际竹藤中心竹藤科学与技术重点实验室,北京 100102

Research Progress of Supported Noble Metal Catalysts in Catalytic Oxidation of Formaldehyde

LI Shijie, HUANG Huijuan, WEN Shitao, MA Jianfeng, LIU Xing'e

International Centre for Bamboo and Rattan, Key Laboratory of Bamboo and Rattan Science and Technology, Beijing 100102,China

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摘要甲醛(HCHO)是主要的室内污染气体之一,长期处于含甲醛的环境会对人体健康产生不利影响。因此,从室内空气中去除甲醛至关重要。室温下,采用贵金属催化剂将甲醛氧化为无毒的二氧化碳和水,是目前最有前景的去除甲醛的方法之一。本文介绍了近年来铂(Pt)、金(Au)、钯(Pd)和银(Ag)四种负载型贵金属催化剂在室温下去除甲醛的研究进展,讨论了负载型贵金属催化剂影响甲醛去除的因素,分析了催化氧化甲醛的机理,并对负载型贵金属催化剂在室温下催化氧化甲醛提出了展望。

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关键词: 甲醛贵金属催化剂催化氧化

Abstract: Formaldehyde (HCHO) is one of the major pollutants in indoor air, and long-term exposure to the environment containing formaldehyde is harmful and may cause health problems. Therefore, it is necessary to eliminate HCHO from indoor air. Supported noble metal catalysts can completely oxidized HCHO into harmless H₂O and CO₂ at ambient temperature, which is regarded as the most promising strategy for the removal of HCHO. In this review, we summarize the recent advances in room-temperature HCHO oxidation over noble metal-based catalysts, which contain platinum (Pt), gold (Au), palladium (Pd), and silver (Ag). In particular, the factors affecting the removal efficiency of formaldehyde, the mechanisms for catalytic oxidation of HCHO over supported noble metal catalysts at room temperature and perspectives for future research in this area are also reviewed.

Key words: formaldehyde noble metal catalyst catalytic oxidation

发布日期: 2020-07-01

ZTFLH:

TG1

基金资助: “十三五”国家重点研发计划资助(2017YFD0600804)

作者简介: 李世杰,2019年6月毕业于福建农林大学,获得工学学士学位。现为国际竹藤中心硕士研究生,在刘杏娥教授的指导下进行研究。目前主要研究领域为生物质基功能性炭材料;刘杏娥,博士,研究员,博士研究生导师。主要从事竹藤材结构与性能、竹藤等生物质基炭材料方面的研究工作。主持和参加了国家级、省部级科研课题多项,在Wood and Fiber Science、Holzforschung、Carbohydrates Polymer和Electrochimica Acta等多种刊物发表论文40余篇,参与编写专著3部,获“梁希”林业科学技术奖一等奖、二等奖及茅以升木材科学技术奖各1项,入选“国家林业和草原局百千万人才工程”第五批人选和国家林业局“全国生态建设突出贡献先进个人”。

引用本文:

李世杰, 黄慧娟, 文世涛, 马建锋, 刘杏娥. 负载型贵金属催化剂氧化分解甲醛的研究进展[J]. 材料导报, 2020, 34(Z1): 400-407.
LI Shijie, HUANG Huijuan, WEN Shitao, MA Jianfeng, LIU Xing'e. Research Progress of Supported Noble Metal Catalysts in Catalytic Oxidation of Formaldehyde. Materials Reports, 2020, 34(Z1): 400-407.

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http://www.mater-rep.com/CN/ 或 http://www.mater-rep.com/CN/Y2020/V34/IZ1/400

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