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材料导报  2023, Vol. 37 Issue (15): 21110075-14    https://doi.org/10.11896/cldb.21110075
  无机非金属及其复合材料 |
石墨烯改性导热复合材料研究进展
颜睿1, 沃虓野1, 王豫2, 黄健1, 张齐贤1,*
1 上海大学材料科学与工程学院,上海 200436
2 吉林农业大学园艺学院,长春 130022
Research Progress of Graphene-modified Thermo-conductive Composites
YAN Rui1, WO Xiaoye1, WANG Yu2, HUANG Jian1, ZHANG Qixian1,*
1 School of Materials Science and Engineering, Shanghai University, Shanghai 200436, China
2 School of Horticulture, Jilin Agricultural University, Changchun 130022, China
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输出:  BibTeX | EndNote (RIS)      
摘要 石墨烯具有极佳的热学与电学性能,是目前十分热门的炭材料之一,在导热领域应用价值显著。石墨烯与聚合物复合后制得的石墨烯改性导热复合材料(GTCCs)具有优异的力学性能、热学性能和化学稳定性。对电子设备日益严重的发热问题而言,GTCCs是一种有效的解决方案,其具有替代商用导热硅脂的潜力,梳理相关研究的核心思路并提炼关键信息有助于把握切合实际的发展导向,推动GTCCs大规模产业化应用。本文简要分析了当代电子设备的散热需求与GTCCs的导热机理;将GTCCs的改性手段分为填料杂化、填料改性和主动构建导热骨架三类,介绍了与各类改性手段相适应的生产工艺和国内外研究进展;列举了GTCCs在传感器、涂层等方面的实际应用,展示了其巨大的工业价值;最后,在展望GTCCs未来的同时,对GTCCs研究中存在的问题进行了探讨,从实际出发总结了一些有前景的发展方向。
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颜睿
沃虓野
王豫
黄健
张齐贤
关键词:  导热材料  石墨烯  环氧树脂  热界面材料    
Abstract: Graphene is one of the most widely known carbon materials owing to its excellent thermal and electrical properties. It has significant potential for application in thermal conductivity. Graphene-modified thermo-conductive composites (GTCCs), fabricated using graphene and a polymer, have excellent mechanical and thermal properties, and chemical stability. GTCCs is an effective solution for the heating issues commonly experienced by electronic equipment, with the potential to replace commercial thermally-conductive silicone grease. Combining the fundamental concepts derived from GTCC-related research and refining the key information will facilitate the practical development and promote the large-scale industrial application of the technology. In this review, the heat dissipation requirements of modern electronic equipment and the heat conduction mechanism of GTCCs are briefly examined. Subsequently, the modification methods of GTCCs are divided into three categories: filler hybrids, filler modification, and active fabrication of heat-conductive skeletons. The adaption of the production process to various modification methods and the local and international research progress are introduced. The practical applications of GTCCs in sensors and coatings are presented, demonstrating its significant industrial importance. Finally, the existing problems facing GTCC research are discussed, while summarizing and predicting the future prospects of the GTCC technology, concluding with guidelines for some promising developments.
Key words:  thermal conductive material    graphene    epoxy resin    thermal interfacial material
出版日期:  2023-08-10      发布日期:  2023-08-07
ZTFLH:  TB33  
基金资助: 国家自然科学基金(21375124)
通讯作者:  * 张齐贤,上海大学材料科学与工程学院研究员、博士研究生导师。2000年吉林大学材料化学专业本科毕业,2003年吉林大学高分子化学与物理专业硕士毕业,2011年东北师范大学物理化学专业博士毕业。主要研究方向为电子信息材料、石墨烯导热材料、特种复合材料、纳米材料电化学等。已发表SCI收录的署名文章40余篇,获得授权或正在申请的发明专利20项。qxzhangshu@shu.edu.cn   
作者简介:  颜睿,2020年6月毕业于南京邮电大学,获得工学学士学位。现为上海大学材料科学与工程学院硕士研究生,在张齐贤研究员的指导下进行研究。目前主要研究领域为石墨烯导热材料。
引用本文:    
颜睿, 沃虓野, 王豫, 黄健, 张齐贤. 石墨烯改性导热复合材料研究进展[J]. 材料导报, 2023, 37(15): 21110075-14.
YAN Rui, WO Xiaoye, WANG Yu, HUANG Jian, ZHANG Qixian. Research Progress of Graphene-modified Thermo-conductive Composites. Materials Reports, 2023, 37(15): 21110075-14.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.21110075  或          http://www.mater-rep.com/CN/Y2023/V37/I15/21110075
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