质子交换膜水电解制氢反应:铱基催化剂设计研究进展

doi:10.11896/cldb.24110228

材料导报

2025, Vol. 39

Issue (23): 24110228-13 https://doi.org/10.11896/cldb.24110228

无机非金属及其复合材料

质子交换膜水电解制氢反应:铱基催化剂设计研究进展

李赢华^1,2, 皮晓琳³, 李鸿鹏³, 田乙然³, 王钰锟³, 张毅², 张振强³, 唐振艳³, 徐超⁴, 姚苌^3,*

1 昆明贵金属研究所稀贵金属综合利用新技术国家重点实验室,昆明 650106
2 昆明学院化学化工学院,昆明 650106
3 云南贵金属实验室有限公司,昆明 650106
4 华东理工大学化工学院,上海 200237

Research Progress on Iridium-based Catalyst Design for Hydrogen Production via Proton Exchange Membrane Water Electrolysis

LI Yinghua^1,2, PI Xiaolin³, LI Hongpeng³, TIAN Yiran³, WANG Yukun³, ZHANG Yi², ZHANG Zhenqiang³,TANG Zhenyan³, XU Chao⁴, YAO Chang^3,*

1 Kunming Institute of Precious Metals, State Key Laboratory of New Technologies for Comprehensive Utilization of Rare and Precious Metals, Kunming 650106, China
2 School of Chemistry and Chemical Engineering, Kunming University, Kunming 650106, China
3 State Key Laboratory of New Technology for Comprehensive Utilization of Rare and Precious Metals, Kunming Institute of Precious Metals, Kunming 650106, China
4 School of Chemical Engineering, East China University of Science and Technology, Shanghai 200237, China

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摘要质子交换膜(PEM)水电解制氢技术在克服间歇性可再生能源利用障碍以及在减少碳排放方面具有重要意义。由于反应条件苛刻和析氧反应(OER)中的缓慢四电子转移过程,贵金属铱(Ir)凭借其卓越的耐腐蚀性,成为酸性电解水的理想选择。然而,Ir资源的稀缺性和高昂成本严重制约了其商业化和大规模应用。因此,如何合理设计和高效制备Ir基催化剂对电解水制氢至关重要。本文综述了近年来Ir基催化剂在酸性介质中电解水制氢领域的研究进展,重点讨论了三种催化剂的合成策略:特殊形貌的Ir基催化剂合成策略、Ir与其他金属的合金化策略以及氧化铱的改性策略。此外,还展望了PEM水电解OER Ir基催化剂在材料改性方面的发展方向。通过对现有研究成果的综合分析,本文可为未来的研究提供理论基础和实践指导。

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	李赢华
	皮晓琳
	李鸿鹏
	田乙然
	王钰锟
	张毅
	张振强
	唐振艳
	徐超
	姚苌

关键词: 质子交换膜析氧反应电解水铱催化剂催化剂设计

Abstract: Proton exchange membrane (PEM) water electrolysis technology plays a significant role in overcoming the challenges of intermittent rene-wable energy utilization and reducing carbon emissions. Due to the harsh reaction conditions and the slow four-electron transfer process involved in the oxygen evolution reaction (OER), precious metal iridium (Ir), with its exceptional corrosion resistance, has become an ideal choice for acidic water electrolysis. However, the scarcityand high cost of Ir resources severely restrict their commercialization and large-scale application. Therefore, rational design and efficient preparation of Ir-based catalysts are crucial for hydrogen production via water electrolysis. This review introduced recent advances in Ir-based catalysts for hydrogen production in acidic media, focusing on three synthesis strategies:the synthesis of Ir-based catalysts with special morphologies, the alloying strategy of Ir with other metals, and the modification strategy of iridium oxide. Additionally, it outlined future directions for the development of PEM water electrolysis OER Ir-based catalysts in terms of material modification. Through a comprehensive analysis of existing research findings, this work can provide a theoretical foundation and practical guidance for future investigations.

Key words: proton exchange membrane oxygen evolution reaction water electrolysis iridium catalyst catalyst design

出版日期: 2025-12-10 发布日期: 2025-12-03

ZTFLH:

TB34

基金资助: 云南贵金属实验室科技计划(YPML-20240502078;YPML-20240502093;YPML-2023050215)

通讯作者: ^*姚苌,博士,云南贵金属实验室有限公司助理研究员。目前研究主要聚焦于高性能聚合物、高端化学品合成中以及电解水反应的催化加氢体系,致力于基于反应机理与数据驱动方法的选择性加氢催化剂设计与优化。yaoc@ipm.com.cn

作者简介: 李赢华,昆明学院化学化工学院与昆明贵金属研究所联合培养硕士研究生,在唐振艳副研究员和姚苌助理研究员的指导下研究电解水制氢的催化剂设计与性能调控。

引用本文:

李赢华, 皮晓琳, 李鸿鹏, 田乙然, 王钰锟, 张毅, 张振强, 唐振艳, 徐超, 姚苌. 质子交换膜水电解制氢反应:铱基催化剂设计研究进展[J]. 材料导报, 2025, 39(23): 24110228-13.
LI Yinghua, PI Xiaolin, LI Hongpeng, TIAN Yiran, WANG Yukun, ZHANG Yi, ZHANG Zhenqiang,TANG Zhenyan, XU Chao, YAO Chang. Research Progress on Iridium-based Catalyst Design for Hydrogen Production via Proton Exchange Membrane Water Electrolysis. Materials Reports, 2025, 39(23): 24110228-13.

链接本文:

https://www.mater-rep.com/CN/10.11896/cldb.24110228 或 https://www.mater-rep.com/CN/Y2025/V39/I23/24110228

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