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材料导报  2024, Vol. 38 Issue (11): 22120169-13    https://doi.org/10.11896/cldb.22120169
  无机非金属及其复合材料 |
二维材料用于电化学法制备过氧化氢的研究进展
盛雄1,2, 李邦兴1,*, 陆顺2, 陆文强2, 李晓锋3, 康帅2,*
1 重庆理工大学理学院,重庆 400054
2 中国科学院重庆绿色智能技术研究院,重庆 400714
3 重庆市计量质量检测研究院,重庆 401123
Research Progress on Electrochemically Producing Hydrogen Peroxide Using Two-dimensional Materials as Catalysts
SHENG Xiong1,2, LI Bangxing1,*, LU Shun2, LU Wenqiang2, LI Xiaofeng3, KANG Shuai2,*
1 Faculty of Science, Chongqing University of Technology, Chongqing 400054, China
2 Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 400714, China
3 Chongqing Academy of Metrology and Quality Inspection, Chongqing 401123, China
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摘要 用电化学的方法通过氧还原反应生产过氧化氢更为环保和有效,而实现这一途径的关键在于制备高活性、高选择性和高稳定性的电催化剂。贵金属催化剂是首选,其催化活性好且稳定性高。但是,贵金属成本高,不利于过氧化氢的规模化制备。因此,减少贵金属用量或者寻找低成本的可替代品一直是近年来的研究热点。很多非贵金属材料已被用作氧还原反应的电催化剂,其中部分材料和贵金属的催化性能相当,甚至更加优异。二维材料相比于本体材料更利于电子传递且更加容易进行化学修饰,二维材料的原子利用率高,可以给电化学反应提供较大的反应场所和更多的裸露活性位点。本文根据已报道的大量实验和理论计算研究,讨论了用二电子氧还原反应法制备过氧化氢的反应机理,然后列举了近年来石墨烯类催化材料、二维过渡金属硫族化合物、二维共价有机骨架和二维金属有机骨架、石墨相氮化碳、二维过渡金属碳/氮化物在电催化氧还原反应中的研究进展,重点分析了其电化学反应机理。最后,指出了二维材料在二电子氧还原反应中的研究挑战和趋势。
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盛雄
李邦兴
陆顺
陆文强
李晓锋
康帅
关键词:  电催化  氧还原反应  过氧化氢  二维材料    
Abstract: The electrochemical production of hydrogen peroxide via the two-electron oxygen reduction reaction (ORR) is a green, mild, and on-demand strategy. The key to this process is highly active, selective, and stable electrocatalysts. Noble metal catalysts are the most effective catalysts for the electrochemical production of hydrogen peroxide due to their unique physical and chemical properties. However, low-cost catalysts are essential for achieving the large-scale production of hydrogen peroxide. Therefore, reducing the dosage of precious metals or finding affor-dable and readily available alternatives has been a topic of considerable research interest in recent years. Numerous non-precious metals or non-metallic materials have been used in oxygen reduction electrocatalysts, some of which have comparable or even superior electrochemical perfor-mances compared to noble metal catalysts. Furthermore, the band structures and surface structures of two-dimensional materials are easier to adjust than those of bulk materials. Two-dimensional materials exhibit faster electron transportation, achieve higher atomic utilization, and possess more exposed active sites. This review discusses the reaction mechanisms of the two-electron ORR for hydrogen peroxide production based on reported experimental results and theoretical calculations, and collates recent reports on the use of graphene, two-dimensional transition metal chalcogenide compounds, two-dimensional MOFs/COFs, g-C3N4, and MXenes as electrocatalysts for the ORR. Finally, the remaining challenges of the application of two-dimensional materials as oxygen reduction electrocatalysts are briefly summarized.
Key words:  electrocatalysis    two-electron oxygen reduction    hydrogen peroxide    two-dimensional materials
出版日期:  2024-06-25      发布日期:  2024-06-25
ZTFLH:  O64  
基金资助: 中国科学院青年创新促进会(2019374);重庆自然科学基金项目(cstc2021jcyj-msxmX0923)
通讯作者:  *李邦兴,重庆理工大学理学院副教授、硕士研究生导师。2013年四川大学电子信息学院光学工程专业博士毕业后到重庆理工大学工作至今,2015年到2016年期间在中国香港教育大学资源与环境学院做高级研究助理,2018年到2020年在美国威斯康辛大学密尔沃基分校做访问学者。目前主要从事新能源材料与器件等方面的研究。发表论文20余篇,包括Optics Materials、Physic B等。libx@cqut.edu.cn;
康帅,中国科学院重庆绿色智能技术研究院副研究员、硕士研究生导师。2015年中山大学物理科学与工程技术学院凝聚态物理专业博士毕业,2015年到2017年在美国威斯康辛大学密尔沃基分校做博士后、研究助理,随后到中国科学院重庆绿色智能技术研究院工作至今。目前主要从事电催化剂、电化学电池等方面的研究工作。发表论文30余篇,包括Nano Letters、Journal of Power Sources、Electrochimica Acta、Chemical Communications等。kangshuai@cigit.ac.cn   
作者简介:  盛雄,2021年6月于重庆理工大学获得工学学士学位。现为重庆理工大学理学院和中国科学院重庆绿色智能技术研究院联合培养的硕士研究生,在李邦兴副教授和康帅副研究员的指导下进行研究。目前主要研究领域为电催化制备过氧化氢。
引用本文:    
盛雄, 李邦兴, 陆顺, 陆文强, 李晓锋, 康帅. 二维材料用于电化学法制备过氧化氢的研究进展[J]. 材料导报, 2024, 38(11): 22120169-13.
SHENG Xiong, LI Bangxing, LU Shun, LU Wenqiang, LI Xiaofeng, KANG Shuai. Research Progress on Electrochemically Producing Hydrogen Peroxide Using Two-dimensional Materials as Catalysts. Materials Reports, 2024, 38(11): 22120169-13.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.22120169  或          http://www.mater-rep.com/CN/Y2024/V38/I11/22120169
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