农林废弃生物质资源精深加工技术进展

doi:10.11896/cldb.20090140

材料导报

2021, Vol. 35

Issue (19): 19001-19014 https://doi.org/10.11896/cldb.20090140

材料与可持续发展(四)——材料再制造与废弃物料资源化利用^*

农林废弃生物质资源精深加工技术进展

李涛¹, 何松¹, 林晓莹¹, 郝世吉¹, 檀付瑞¹, 杨震宇¹, 陈德良^1,2, 杨华明³

1 东莞理工学院材料科学与工程学院科技创新研究院,东莞 523808
2 郑州大学材料科学与工程学院,郑州 450001
3 中南大学资源加工与生物工程学院,长沙 410083

Recent Advances on Deep Processing Technologies for Resourcing Utilization of Agricultural and Forestry Biomass Wastes

LI Tao¹, HE Song¹, LIN Xiaoying¹, HAO Shiji¹, TAN Furui¹, YANG Zhengyu¹, CHEN Deliang^1,2, YANG Huaming³

1 Institute of Science & Technology Innovation, School of Materials Science and Engineering, Dongguan University of Technology, Dongguan 523808, China
2 School of Materials Science and Engineering, Zhengzhou University, Zhengzhou 450001, China
3 School of Minerals Processing and Bioengineering, Central South University, Changsha 410083, China

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摘要农林废弃生物质主要由木质素、纤维素等组成,来源广泛、可再生,通过对其进行精深加工,可获得具有高附加值的产品,是一种潜在的化石资源替代品,对绿色可持续发展具有重大意义。在生物质资源化产品中,生物质炭材料可通过热解和水热两种炭化方法获得,功能性炭材料的设计与制备是近年来的研究重点。生物质合成气可通过气化、热解、水热气化等方法获得,主要含有H₂、CO等气体,可直接作为燃料,或者作为合成生物质油及其他化学品的原料,目前的研究主要致力于提高生物质合成气的产率和质量。生物质油则可通过热解、水热液化等方法得到,或以生物质合成气为原料经费托合成获得,生物质油主要含有烷烃、烯烃、芳香族化合物等,通过精炼可作为汽油、柴油的替代品,提高生物油的产率及选择性是近年来的研究重点。
本文根据生物质深加工产物形态的不同,将生物质精深加工技术分为固相、气相、液相等三类,从生物质利用技术的原理、工艺条件、最新进展等角度,对农林废弃生物质资源的精深加工研究进展进行了梳理和系统总结,列举了部分代表性研究成果,旨在进一步理解生物质农林废弃物资源化精深加工技术发展的前沿动态、前景与潜力,为探求绿色可持续发展提供新的工程化思路与方法。

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	李涛
	何松
	林晓莹
	郝世吉
	檀付瑞
	杨震宇
	陈德良
	杨华明

关键词: 农林废弃物生物质热解水热生物质炭生物质合成气生物质油资源化

Abstract: Biomass, mainly composed of lignin and cellulose, is abundant and renewable. Through physical and chemical methods, these agricultural and forestry waste biomasses can be processed to be high value-added products, such as carbon materials, bio-oil, organic chemicals and so on, and this is of great significance for green and sustainable development. Biomass carbon materials can be obtained by pyrolysis and hydrothermal carbonization methods, and the research on biochar is extensively focused on the design and preparation of functional carbon materials in recent years. Biomass syngas can be obtained by gasification, pyrolysis, hydrothermal gasification and other methods. Biomass syngas mainly contains H₂, CO and other gases, and can be directly used as fuel or as raw materials for the synthesis of biomass oil and other chemicals. The yields and quality of biomass syngas are usually low, and different catalysts are developed to improve them. Biomass oils can be obtained by pyrolysis, hydrothermal liquefaction and biomass syngas as raw materials. Biomass oils mainly contain alkanes, olefins, aromatic compounds and so on. They can be used as the substitute for gasoline and diesel oil after refining. The compositions of bio-oils are complex and contain a variety of organic compounds, and the separation and purification of these components and enhancing yields of target oils are the research focus in recent years.
In this review, the deep processing technologies of biomass are divided into the solid-phase, gas-phase and liquid-phase utilization ones according to the different forms of target products prepared by deep-processing biomass. From the perspective of the principle, process conditions and the latest progress of typical utilization technology of biomass, the fine-processing technologies of agricultural and forestry biomass are systematically summarized, and some representative research examples are introduced. In order to further understand the developing trend, prospect and potential of agricultural and forestry biomass, the intensive processing technologies provide new engineering ideas and technical support for exploring green and sustainable development.

Key words: biomass wastes deep processing pyrolysis carbonization biomass carbon bio-syngas bio-oil resource utilization

出版日期: 2021-10-10 发布日期: 2021-11-03

ZTFLH:

TQ91

基金资助: 国家自然科学基金(51574205);广东省自然科学基金(2018B030311022);广东高等教育创新团队(2017KCXTD030);广东省高等学校非粮生物质高效热解与利用技术工程研究中心(2016GCZX009);东莞理工学院高层次人才项目(KCYKYQD2017017);河南省高校科技创新团队(19IRTSTHN028);东莞理工学院大学生创新创业计划立项项目(201911819038)

通讯作者: dlchen@dgut.edu.cn; hmyang@csu.edu.cn

作者简介: 李涛,2012年毕业于郑州大学,获工学硕士学位,现为东莞理工学院研究助理,主要从事能源转换与存储功能材料的研究。
陈德良,博士,郑州大学教授,博士研究生导师,2005年博士毕业于中国科学院上海硅酸盐研究所,河南省学术技术带头人、河南省科技创新杰出青年、河南省高校创新人才、郑州市青年科技奖获得者、东莞理工学院学科领军人才,现任东莞理工学院材料科学与工程学院副院长。主要从事生物质与矿物等天然资源材料、功能精细陶瓷、环境净化与催化材料、纳米结构材料、光电功能复合材料的设计、制备与应用研究,对先进无机材料的制备、生物质及矿物材料的精细加工及高效利用方法与思路以及高附加值化有一定基础和经验。
杨华明,工学博士,中南大学教授、博士研究生导师,中组部国家“万人计划”领军人才、国家杰出青年科学基金获得者、国家中青年科技创新领军人才、湖南省科技领军人才、教育部新世纪优秀人才,享受国务院政府特殊津贴。现任中国建筑材料行业黏土矿物功能材料重点实验室主任、矿物材料及其应用湖南省重点实验室主任、湖南省矿物材料国际联合实验室(国际科技创新合作基地)主任。在中南工业大学获学士、硕士和博士学位,先后在英国布里斯托大学、澳大利亚昆士兰大学、俄罗斯科学院固态化学研究所任访问学者。长期从事矿物材料、能源与环境材料、生物医学材料、材料计算、固废资源化等研究,致力于材料、矿物、化学、物理、生物医学等多学科交叉,主持国家自然科学基金、国家科技支撑计划、863课题、973专题、博士点基金、教育部重点项目等多项基金项目。

引用本文:

李涛, 何松, 林晓莹, 郝世吉, 檀付瑞, 杨震宇, 陈德良, 杨华明. 农林废弃生物质资源精深加工技术进展[J]. 材料导报, 2021, 35(19): 19001-19014.
LI Tao, HE Song, LIN Xiaoying, HAO Shiji, TAN Furui, YANG Zhengyu, CHEN Deliang, YANG Huaming. Recent Advances on Deep Processing Technologies for Resourcing Utilization of Agricultural and Forestry Biomass Wastes. Materials Reports, 2021, 35(19): 19001-19014.

链接本文:

http://www.mater-rep.com/CN/10.11896/cldb.20090140 或 http://www.mater-rep.com/CN/Y2021/V35/I19/19001

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