光/电催化废塑料升级再造高附加值化学品研究进展

doi:10.11896/cldb.23060226

材料导报

2024, Vol. 38

Issue (20): 23060226-7 https://doi.org/10.11896/cldb.23060226

高分子与聚合物基复合材料

光/电催化废塑料升级再造高附加值化学品研究进展

刘睿琦, 孙善富^*, 程鹏飞, 王莹麟, 郝熙冬

西安电子科技大学空间科学与技术学院,西安 710126

Recent Progresses in Photocatalytic and Electrocatalytic Upcycling of Plastic Wastes to High Value-added Chemicals

LIU Ruiqi, SUN Shanfu^*, CHENG Pengfei, WANG Yinglin, HAO Xidong

School of Aerospace Science and Technology, Xidian University, Xi’an 710126, China

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摘要废塑料的回收利用是降低环境污染和减少资源浪费的有效途径之一,与传统的机械循环和化学循环回收相比,近年来新兴的光催化和电催化废塑料升级再造高附加值化学品技术因其反应条件温和、效率高,且能够利用可再生能源(太阳能、风能等)驱动反应发生,有望实现能源和化学品的脱石化资源、低碳绿色和分布式发展,符合“双碳”发展理念,迅速得到学者们的广泛关注和探讨。综述了近年来有关光催化和电催化废塑料升级再造高附加值化学品的最新研究进展,重点讨论了催化剂类型对产物类型和产率的影响以及不同催化剂的光催化和电催化反应路径和机理,最后针对目前技术存在的问题提出开发高效光/电催化剂以提升高附加值产物选择性和产率、理论模拟结合原位表征技术探究光/电催化反应机理、开发高效催化反应设备是今后光/电催化废塑料升级再造高附加值化学品研究的主要方向。

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关键词: 废塑料光催化电催化升级再造高值化学品

Abstract: The recycling and utilization ofplastic wastes is one of the effective ways to reduce environmental pollution and resource waste. Compared to the traditional mechanical cycle and chemical cycle recycling, the newly emerging photocatalytic and electrocatalytic waste plastic upcycling high value-added chemical technologies have aroused widespread attention due to their mild reaction conditions, high efficiency, and can use renewable energy to drive the reactions. It is expected to realize the circumvention resources of fossil fuel and chemicals development, which is in line with the carbon peaking and carbon neutrality goals. Herein, the latest research progress on photocatalytic and electrocatalytic upcycling of high value-added chemicals from waste plastics in recent years was reviewed, with emphasis on the effects of catalyst types on product types and yields, as well as the reaction paths and mechanisms of different catalysts. Ultimately, in view of the problems with these current technologies, points out the main research directions in future, including the development of efficient photo-/electrocatalytic catalysts to improve the selectivity and yield of high value-added products, theoretical simulation combined with in-situ characterization technologies to explore the mechanisms of catalytic reactions, and the development of efficient catalytic reaction equipment.

Key words: plastic wastes photocatalysis electrocatalysis upcycling high value-added chemicals

出版日期: 2024-10-25 发布日期: 2024-11-05

ZTFLH:

TQ320.9

基金资助: 国家自然科学基金(22205169)

通讯作者: * 孙善富,西安电子科技大学空间科学与技术学院华山准聘副教授、硕士研究生导师。2021年哈尔滨工业大学化学工程与技术学科博士毕业后到西安电子科技大学工作至今。目前主要从事光/电催化、载人航天再生生命保障技术等方面的研究工作。发表SCI论文30余篇,包括ACS Catalysis、Journal of Catalysis、Materials Today Energy、Journal of Colloid and Interface Science等。sunshanfu@xidian.edu.cn

作者简介: 刘睿琦,2022年6月于陕西师范大学获得理学学士学位,现为西安电子科技大学空间科学与技术学院研究生。目前主要研究领域为电催化合成有机化学品。

引用本文:

刘睿琦, 孙善富, 程鹏飞, 王莹麟, 郝熙冬. 光/电催化废塑料升级再造高附加值化学品研究进展[J]. 材料导报, 2024, 38(20): 23060226-7.
LIU Ruiqi, SUN Shanfu, CHENG Pengfei, WANG Yinglin, HAO Xidong. Recent Progresses in Photocatalytic and Electrocatalytic Upcycling of Plastic Wastes to High Value-added Chemicals. Materials Reports, 2024, 38(20): 23060226-7.

链接本文:

http://www.mater-rep.com/CN/10.11896/cldb.23060226 或 http://www.mater-rep.com/CN/Y2024/V38/I20/23060226

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