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材料导报  2023, Vol. 37 Issue (8): 21050145-10    https://doi.org/10.11896/cldb.21050145
  高分子与聚合物基复合材料 |
基于缓蚀剂微/纳米容器的智能自修复涂层研究进展
卫元坤1,2, 张优1,*, 张政1, 王菊萍1, 陈飞1,3
1 北京石油化工学院新材料与化工学院,北京 102617
2 北京石油化工学院安全工程学院,北京 102617
3 特种弹性体复合材料北京市重点实验室,北京 102617
Smart Self-healing Coatings Based on Corrosion Inhibitor Micro-/Nano-containers: a Review
WEI Yuankun1,2, ZHANG You1,*, ZHANG Zheng1, WANG Juping1, CHEN Fei1,3
1 College of New Materials and Chemical Engineering, Beijing Institute of Petrochemical Technology, Beijing 102617, China
2 Department of Safety Engineering, Beijing Institute of Petrochemical Technology, Beijing 102617, China
3 Beijing Key Laboratory of Special Elastomeric Composite Materials, Beijing 102617, China
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摘要 涂层技术是常用的金属腐蚀防护手段。随着材料的服役环境日益严苛,采用传统的涂覆方法只能起到被动防护的作用,一旦涂层受损则会失效。近年来发展起来的智能自修复防腐涂层可根据环境变化自主修复涂层受损处,增强涂层的防护能力,延长金属基体(钢、镁、铝及其合金)的使用寿命。本文综述了国内外基于负载缓蚀剂的微/纳米容器的自修复涂层在金属腐蚀防护方面取得的最新成果,介绍了不同类型的微/纳米容器的特点及对缓蚀剂的负载与控制释放行为,包括介孔纳米颗粒(二氧化硅、二氧化钛等)、无机粘土(多水高岭石、类水滑石、沸石)等无机纳米容器,聚合物微胶囊、纳米纤维、壳聚糖、环糊精等有机纳米容器,碳纳米管、石墨烯等碳材料,以及多种微/纳米容器的复合应用,并对不同微/纳米容器的优点及缺点进行总结。最后,提出了基于缓蚀剂微/纳米容器自修复防腐涂层研究中存在的问题,并对其未来发展方向进行了展望。
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卫元坤
张优
张政
王菊萍
陈飞
关键词:  自修复涂层  微/纳米容器  缓蚀剂  腐蚀防护    
Abstract: Surface coating technologies are essential for corrosion protection. However, the application of passive protection coatings is limited under severe service conditions. Therefore, self-healing corrosion protection coatings are developed to meet specific industrial requirements, owing to their ability to independently, intelligently repair coating defects in response to changing environmental conditions. Self-healing coatings possess both active and passive protective abilities that effectively contribute to prolonging the service life of metal substrates (steel, magnesium, aluminum, and their alloys). This article covers the recent achievements in developing micro-/nano-containers for application in self-healing corrosion protection coatings. A wide variety of micro-/nano-containers with storage or release abilities for corrosion inhibitors has been employed in self-healing corrosion protection coatings. Micro-/nano-containers include inorganic ones, such as mesoporous nanoparticles (e.g., silica and titanium dioxide), inorganic clays (e.g., kaolinite, hydrotalcite, and zeolite), organic ones (e.g., polymer microcapsule, nanofiber, chitosan, and cyclodextrin), and carbon materials (e.g., carbon nanotube and graphene), as well as their diverse combinations. This article comprehensively summarizes the performance advantages and drawbacks of micro-/nano-containers. Finally, the existing problems and future developments of the smart self-healing coatings based on corrosion inhibitor micro-/nano-containers are also reviewed.
Key words:  self-healing coating    micro-/nano-container    corrosion inhibitor    corrosion protection
出版日期:  2023-04-25      发布日期:  2023-04-24
ZTFLH:  TG146  
  TG178.2  
基金资助: 北京市自然科学基金(2182017;2202017);北京市教委科技计划项目(KM201910017004);国家留学基金委公派访问学者项目(201908110124);北京石油化工学院大学生研究训练计划(2021J00134;2021J00135)
通讯作者:  *张优,北京石油化工学院副教授、硕士研究生导师。2010年7月本科毕业于中南大学,2015年7月在北京航空航天大学材料物理与化学专业取得博士学位,2019—2020年任德国亥姆霍兹吉斯达赫特材料与海洋研究中心访问学者、北京市腐蚀与防护学会理事。主要从事材料与装备的腐蚀及先进涂层制造技术研究工作,先后主持并参与国家自然科学基金、北京市自然科学基金、国防重点研发计划、航空基金、国内外企业横向课题10余项。近五年在ACS Applied Materials & Interfaces、Applied Surface Science等国内外高水平期刊发表论文30篇,获授权国家发明专利5项。youzhang@bipt.edu.cn   
作者简介:  卫元坤,2018年6月毕业于河南工程学院,获得学士学位。现为北京石油化工学院安全工程专业硕士研究生,在张优副教授的指导下进行研究。目前主要研究领域为金属的腐蚀监测与智能防腐涂层的制备及性能。
引用本文:    
卫元坤, 张优, 张政, 王菊萍, 陈飞. 基于缓蚀剂微/纳米容器的智能自修复涂层研究进展[J]. 材料导报, 2023, 37(8): 21050145-10.
WEI Yuankun, ZHANG You, ZHANG Zheng, WANG Juping, CHEN Fei. Smart Self-healing Coatings Based on Corrosion Inhibitor Micro-/Nano-containers: a Review. Materials Reports, 2023, 37(8): 21050145-10.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.21050145  或          http://www.mater-rep.com/CN/Y2023/V37/I8/21050145
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