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材料导报  2026, Vol. 40 Issue (6): 25020167-9    https://doi.org/10.11896/cldb.25020167
  高分子与聚合物基复合材料 |
溶解性有机质介导和屏蔽生物炭降解有机污染物的研究进展
张开洋1,2, 管友森1,2, 易鹏1,2, 黄宇1,2,*, 陈全1,2, 吴敏1,2
1 昆明理工大学环境科学与工程学院,昆明 650500;
2 云南省土壤固碳与污染控制重点实验室,昆明 650500
Recent Advancements in the Mediating and Shielding Effects of Dissolved Organic Matter During the Degradation of Organic Pollutants by Biochar
ZHANG Kaiyang1,2, GUAN Yousen1,2, YI Peng1,2, HUANG Yu1,2,*, CHEN Quan1,2, WU Min1,2
1 Faculty of Environmental Science and Engineering, Kunming University of Science and Technology, Kunming 650500, China;
2 Yunnan Provincial Key Laboratory of Soil Carbon Sequestration and Pollution Control, Kunming 650500, China
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摘要 溶解性有机质(Dissolved organic matter,DOM)是自然环境中广泛且普遍存在的物质,由于其复杂的化学物质结构,显著影响着环境中污染物的环境行为和效应。生物炭由于其丰富的孔隙结构和表面官能团组成,可通过物理化学吸附、直接电子传导、诱导产生自由基等过程去除有机污染物,从而实现可持续的有机污染物治理。然而,当生物炭施加到实际环境中时,生物炭会不可避免地与各环境介质中广泛存在的DOM发生相互作用,其环境功能和效应将会受到不同程度的影响。因此,明确DOM对生物炭降解有机污染物的影响及作用机制对于调控生物炭降解有机污染物有着重要意义。本文通过系统分析已报道文献,阐述了DOM介导和屏蔽生物炭降解有机污染物的行为及作用机制。从介导角度来说,DOM可以促进生物炭产生自由基,利于生物炭对有机污染物的降解,还可作为电子穿梭体促进降解。从屏蔽角度来说,DOM会堵塞生物炭孔道,淬灭生物炭上的自由基,或是占据生物炭表面活性位点,从而屏蔽其对有机污染物的降解。通过系统总结上述DOM在生物炭降解有机污染物中的双面效应,本文深入总结了DOM化学结构对上述正反两个过程的控制机制,为后续生物炭结构调控及其在实际环境中的应用奠定了理论基础。
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张开洋
管友森
易鹏
黄宇
陈全
吴敏
关键词:  生物炭  溶解性有机质  有机污染物  自由基  降解  电子穿梭体    
Abstract: Dissolved organic matter(DOM) with complex chemical structures is present universally in natural environments and significantly influences the environmental behaviors and fates of co-presence contaminants. Biochar rich in pore structures and surface functional groups highlighted a promising solution towards sustainable organic pollutant remediation through physicochemical adsorption, direct electron transfer, and free radical induction. However, the environmental functions and effects of biochar may be altered by the inevitable interaction with DOM in actual water and soil environments. Understanding the impact of DOM on the biochar-based degradation of organic pollutants enhances insights into the precise biochar application in such mitigation schemes. In this concept, we elucidated the behaviors and mechanisms of the DOM-mediated or -inhibited organic degradation in biochar systems by recruiting the available literature base. Our analysis confirmed that DOM exhibits a dual role during the biochar-based degradation of organic pollutants. On the one hand, DOM can facilitate the generation of free radicals by interacting with biochar and acting as an electron shuttle, thus enhancing the organic degradation. On the other hand, DOM can clog biochar's pore structures, quenc-hing free radicals and occupying active sites on the biochar surface, thereby hindering the pollutant degradation. We end up by summarizing the acquired evidence related to the regulation strategy of organic degradation by biochar with particular DOM structures. This review extends the theoretical foundation for structural regulation of biochar-based organic pollutant remediation and its potential application in actual environments.
Key words:  biochar    dissolved organic matter    organic pollutants    free radicals    degradation    electron shuttle
出版日期:  2026-03-25      发布日期:  2026-04-03
ZTFLH:  X52  
  X53  
  X131  
基金资助: 国家自然科学基金青年基金(42307499);国家自然科学基金面上基金(42377250)
通讯作者:  *黄宇,博士,昆明理工大学环境科学与工程学院讲师、助理研究员、硕士研究生导师。主要从事溶解性有机质的环境效应及厌氧膜生物反应器研究。yuzhehy@qq.com   
作者简介:  张开洋,昆明理工大学环境科学与工程学院硕士研究生,在陈全教授的指导下研究溶解性有机质介导下生物炭降解酚类污染物的作用及其机理。
引用本文:    
张开洋, 管友森, 易鹏, 黄宇, 陈全, 吴敏. 溶解性有机质介导和屏蔽生物炭降解有机污染物的研究进展[J]. 材料导报, 2026, 40(6): 25020167-9.
ZHANG Kaiyang, GUAN Yousen, YI Peng, HUANG Yu, CHEN Quan, WU Min. Recent Advancements in the Mediating and Shielding Effects of Dissolved Organic Matter During the Degradation of Organic Pollutants by Biochar. Materials Reports, 2026, 40(6): 25020167-9.
链接本文:  
https://www.mater-rep.com/CN/10.11896/cldb.25020167  或          https://www.mater-rep.com/CN/Y2026/V40/I6/25020167
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