Please wait a minute...
材料导报  2024, Vol. 38 Issue (2): 22040368-5    https://doi.org/10.11896/cldb.22040368
  高分子与聚合物基复合材料 |
不同种类道路沥青材料异味特征及析源分析
王超, 任正阳, 周波超*, 宫官雨, 季晓斌
北京工业大学城市建设学部,北京 100124
Odor Characteristics and Source Analysis of Different Kinds of Road Asphalt Materials
WANG Chao, REN Zhengyang, ZHOU Bochao*, GONG Guanyu, JI Xiaobin
Faculty of Architecture, Civil and Transportation Engineering, Beijing University of Technology, Beijing 100124, China
下载:  全 文 ( PDF ) ( 3716KB ) 
输出:  BibTeX | EndNote (RIS)      
摘要 随着我国社会经济逐渐向绿色可持续转型,沥青路面铺筑过程中的异味污染成为不可忽视的环境问题。本研究针对八种不同的道路沥青材料使用过程中产生的挥发性物质,通过气相色谱-质谱联用仪(GC-MS)和气体检测仪进行定性与定量分析。在此基础上,结合异味阈值计算各物质异味活度值 (OAV),通过异味活度值加和 (SOAV) 的方法对沥青异味进行分析,并对异味污染物中各组分及其异味贡献进行进一步的析源工作。研究结果表明,沥青挥发物的浓度与异味活度值加和并没有完全的正相关关系,胶粉改性沥青挥发物浓度及异味活度值加和相较于其他沥青均有显著提高。对八种不同种类道路沥青材料异味特征进行分析得出:六种组分对沥青异味的产生有贡献,其中,苯系物、醛类以及硫化氢对沥青异味的贡献较大,烯烃类以及酮类是胶粉改性沥青挥发物中特有的异味贡献组分。
服务
把本文推荐给朋友
加入引用管理器
E-mail Alert
RSS
作者相关文章
王超
任正阳
周波超
宫官雨
季晓斌
关键词:  道路工程  沥青材料  定性定量  异味活度值  异味活度值加和  异味贡献    
Abstract: With the social economy gradual transformating to green and sustainable, the odor pollution in the process of road asphalt paving has become an environmental problem that cannot be ignored. In this study, gas chromatography-mass spectrometry(GC-MS) and gas detector were used for qualitative and quantitative analysis of volatile substances produced by eight asphalt materials. On this basis, combined with the odor threshold, the odor activity value (OAV) of each substance was calculated, and odor emissions of road asphalt was analyzed by the method of the sum of the odor activity value (SOAV), and the odor contribution of each component and its odor pollutants was further analyzed. The results show that there is no positive correlation between the volatile concentration of asphalt and the sum of the odor activity values, and the volatile concentration and the sum of the odor activity values of asphalt modified by rubber powder are significantly higher than those of other asphalt. The analysis of the odor characteristics of eight different kinds of road asphalt materials shows that six components contribute to the odor of asphalt, among which benzene series, aldehydes and hydrogen sulfide contribute more to the odor, olefin and ketone are special odor contributing components in the volatile of rubber powder modified asphalt.
Key words:  road engineering    asphalt materials    qualitative and quantitative analysis    odor activity value    sum of odor activity values    odor contribution
出版日期:  2024-01-25      发布日期:  2024-01-26
ZTFLH:  U414  
基金资助: 北京市自然科学基金项目(8174059);河北省交通运输厅科技项目(202206)
通讯作者:  *周波超,北京工业大学城市建设学部讲师,2021年7月获得长安大学道路与铁道工程专业工学博士学位。目前主要从事绿色路面技术与能源路面方向的研究工作。公开发表论文20余篇,包括Applied Energy、Renewable Energy、Journal of Cleaner Production、Transportation Research Part D:Transport and Environment、Construction and Building Materials等。bczhou@bjut.edu.cn   
作者简介:  王超,北京工业大学城市建设学部副教授、博士研究生导师,2010年6月、2015年7月分别于重庆交通大学和北京工业大学获得工学学士学位和博士学位。主要从事沥青路面结构与材料方向的研究工作,先后主持国家及省部级科研项目课题多项,发表学术研究论文30余篇。
引用本文:    
王超, 任正阳, 周波超, 宫官雨, 季晓斌. 不同种类道路沥青材料异味特征及析源分析[J]. 材料导报, 2024, 38(2): 22040368-5.
WANG Chao, REN Zhengyang, ZHOU Bochao, GONG Guanyu, JI Xiaobin. Odor Characteristics and Source Analysis of Different Kinds of Road Asphalt Materials. Materials Reports, 2024, 38(2): 22040368-5.
链接本文:  
https://www.mater-rep.com/CN/10.11896/cldb.22040368  或          https://www.mater-rep.com/CN/Y2024/V38/I2/22040368
1 Hawko Charbel, Verriele Maria, Hucher Nicolas, et al. Science of the Total Environment, 2021, 795, 148862.
2 Autelitano F, Garilli E, Giuliani F. Transportation Research Procedia, 2019, 40, 4.
3 Autelitano F, Giuliani F. Construction and Building Materials, 2018, 183, 485.
4 Li A. Deodorization mechanism and performance evaluation of rubber asphalt. Master’s Thesis, Harbin Institute of Technology, China, 2020 (in Chinese).
李澳. 橡胶沥青净味机理及性能评价. 硕士学位论文. 哈尔滨工业大学, 2020.
5 Shi F Q. Study on preparation and performance of environmentally friendly rubber modified asphalt and asphalt mixture. Master’s Thesis, Shandong Jianzhu University, China, 2020 (in Chinese).
史福泉. 环保橡胶改性沥青及其沥青混合料的制备与性能研究. 硕士学位论文, 山东建筑大学, 2020.
6 Wu C D. Odour activity value coefficient method and its application on evaluating the odour pollution of landfill and waste disposal plant. Ph.D. Thesis, University of Science and Technology Beijing, China, 2017 (in Chinese).
吴传东. 异味活度值系数法及其在垃圾场异味评价中应用研究. 博士学位论文, 北京科技大学, 2017.
7 Liu Y, Lu W, Wang H, et al. Journal of Environmental Management, 2018, 220, 136.
8 Wang Y, Li L, Qiu Z, et al. Chemosphere, 2021, 272, 129582.
9 Winiewska M, Kulig A, Lelicińska-Serafin K. Applied Sciences, 2021, 11(9), 3916.
10 Rincón C A, De Guardia A, Couvert A, et al. Atmospheric Environment, 2019, 201, 1.
11 Zhao Z, Pei Y, Zhao P, et al. Molecules, 2022, 27(3), 1125.
12 Ravina M, Panepinto D, Estrada J M, et al. Environmental Science and Pollution Research, 2020, 27, 3992.
13 Wang C M, Yu J W, Guo Q Y, et al. Environmental Pollution, 2019, 249, 305.
14 Jo Sang-Hee, Kim Ki-Hyun, Jeon Byong-Hun, et al. Atmospheric Environment, 2015, 119, 339.
15 Hansen M J, Adamsen A, Wu C, et al. Atmosphere, 2021, 12(8), 1008.
16 Guo Q, Yu J, Li X, et al. Journal of Hazardous Materials, 2020, 393(2003), 122404.
17 Li L P. Research on emission characteristic and the emission inhibition method of the volatile organic compounds of rubber asphalt. Master’s Thesis, Wuhan University of Technology, China, 2017 (in Chinese).
李立平. 橡胶沥青 VOCs 的释放特性及抑制方法研究. 硕士学位论文, 武汉理工大学, 2017.
18 Long Y S, Wu S P, Xiao Y, et al. Journal of Wuhan University of Technology (Transportation Science ＆ Engineering), 2018, 42(1), 1 (in Chinese).
龙永双, 吴少鹏, 肖月, 等. 武汉理工大学学报(交通科学与工程版), 2018, 42(1), 1.
19 Xiao Y, Chang X W, Dong Q K, et al. China Journal of Highway and Transport, 2020, 33(10), 276 (in Chinese).
肖月, 常郗文, 董前坤, 等. 中国公路学报, 2020, 33(10), 276.
20 Li N, Jiang Q, Wang F S, et al. Journal of Cleaner Production, 2020, 278, 123479.
21 Espinoza J, Medina C, Calabi-Floody A, et al. Sustainability, 2020, 12(22), 9546 .
22 Wu S P, Yu M, Chen M Z. Petroleum Asphalt, 2011, 25(3), 1 (in Chinese).
吴少鹏, 余嫚, 陈美祝. 石油沥青, 2011, 25(3), 1.
23 Fan C Z. The study of composition of asphalt smoke and its inhibition. Master’s Thesis, China University of Petroleum, China, 2015 (in Chinese).
范成正. 沥青烟气组成及其抑制研究. 硕士学位论文, 中国石油大学(华东), 2015.
24 Qiu Y J, Luo H Y, Zhang J K, et al. Journal of Changan University (Natural Science Edition), 2020, 40(1), 30 (in Chinese).
邱延峻, 罗浩原, 张家康, 等. 长安大学学报(自然科学版), 2020, 40(1), 30.
25 Nagata Y. Odor Measurement Review, 2003, 118, 118.
26 Trabue S, Scoggin K, Tyndall J, et al. Journal of Environmental Ma-nagement, 2018, 233, 12.
27 Gonzalez D, Guerra N, Colon J, et al. Atmosphere, 2020, 11(2), 211.
28 Huffel K V, Hansen M J, Bruneel J, et al. Biosystems Engineering, 2019, 179, 71.
29 Capelli L, Sironi S, Centola P, et al. Atmospheric Environment, 2008, 42(30), 7050.
30 Lu W, Duan Z, Dong L, et al. Waste Management, 2015, 42, 74.
31 Lee H D, Jeon S B, Choi W J, et al. Atmospheric Environment, 2013, 74, 277.
[1] 田威, 云伟, 党可欣, 李腾. 不同钙源EICP溶液改良路基黄土动力特性研究[J]. 材料导报, 2024, 38(9): 22110275-9.
[2] 王超, 宋立昊, 孙彦广, 宫官雨. 道路沥青疲劳与断裂特性研究进展及发展趋势[J]. 材料导报, 2024, 38(9): 22090197-9.
[3] 延西利, 郑涛, 蒋双全, 李卫成. 沥青温拌技术分类及温拌效果的试验评价方法[J]. 材料导报, 2024, 38(4): 22080003-8.
[4] 兰添晖, 刘旭, 贾存兴, 王凌一, 张军朝, 马国伟, 张默. 沥青胶结料应变延迟恢复特性的动态剪切流变试验表征[J]. 材料导报, 2024, 38(4): 22020138-7.
[5] 王黎明, 孙永卓, 庞宏, 许继新, 董明泽. 微波加热对石油沥青的化学、流变及工程特性的影响[J]. 材料导报, 2024, 38(24): 23120216-8.
[6] 牛冬瑜, 黄山, 师伟博, 谢希望, 汪严, 高仰明. 粗集料接触配位参数影响下沥青混合料的抗断裂特性研究[J]. 材料导报, 2024, 38(23): 23050048-10.
[7] 季节, 张梓源, 文龙, 尤鹏超, 马童, 黄昶惟. 粉胶比对煤直接液化残渣复合改性沥青胶浆及混合料低温性能的影响[J]. 材料导报, 2024, 38(22): 23090053-7.
[8] 刘亚敏, 韩旭晖, 高晨光, 钟国亮. 全程老化沥青中温抗疲劳性能及预测模型研究[J]. 材料导报, 2024, 38(21): 23070147-6.
[9] 郑直, 郭乃胜, 金鑫, 房辰泽, 尤占平, 谭忆秋. 水性丙烯酸交通标线涂料研究现状与发展趋势[J]. 材料导报, 2024, 38(21): 22120007-12.
[10] 唐杰, 赵华, 高红成. 碳化硅粉填充沥青混合料微波自愈合性能及合理掺量[J]. 材料导报, 2024, 38(20): 23080070-10.
[11] 张磊, 王鹏, 杨永志, 邢超, 谭忆秋. 基于LCA的不同设计寿命沥青路面能耗排放分析[J]. 材料导报, 2024, 38(20): 23080071-10.
[12] 况栋梁, 马小军, 马晓燕, 袁斌, 侯俊鹏, 蔡军. 废机油残留物再生剂对老化沥青动态力学性能和组分迁移的影响[J]. 材料导报, 2024, 38(2): 22050182-8.
[13] 王志臣, 孙雅珍, 郭乃胜. 基于连续时间谱的沥青混合料黏弹性参数换算[J]. 材料导报, 2024, 38(18): 22120218-6.
[14] 董仕豪, 韩森, 宿金菲, 陈德, 苏会锋. 沥青路面表面纹理三维评价方法及其计算边界条件分析[J]. 材料导报, 2024, 38(18): 23050210-9.
[15] 赵晓康, 张久鹏, 胡勤石, 裴建中, 程科, 张柳. 长余辉水性道面标线涂料的制备与路用性能[J]. 材料导报, 2024, 38(15): 23020088-7.
[1] Yanzhen WANG, Mingming CHEN, Chengyang WANG. Preparation and Electrochemical Properties Characterization of High-rate SiO2/C Composite Materials[J]. Materials Reports, 2018, 32(3): 357 -361 .
[2] Yimeng XIA, Shuai WU, Feng TAN, Wei LI, Qingmao WEI, Chungang MIN, Xikun YANG. Effect of Anionic Groups of Cobalt Salt on the Electrocatalytic Activity of Co-N-C Catalysts[J]. Materials Reports, 2018, 32(3): 362 -367 .
[3] Qingshun GUAN,Jian LI,Ruyuan SONG,Zhaoyang XU,Weibing WU,Yi JING,Hongqi DAI,Guigan FANG. A Survey on Preparation and Application of Aerogels Based on Nanomaterials[J]. Materials Reports, 2018, 32(3): 384 -390 .
[4] Lijing YANG,Zhengxian LI,Chunliang HUANG,Pei WANG,Jianhua YAO. Producing Hard Material Coatings by Laser-assisted Cold Spray:a Technological Review[J]. Materials Reports, 2018, 32(3): 412 -417 .
[5] Zhiqiang QIAN,Zhijian WU,Shidong WANG,Huifang ZHANG,Haining LIU,Xiushen YE,Quan LI. Research Progress in Preparation of Superhydrophobic Coatings on Magnesium Alloys and Its Application[J]. Materials Reports, 2018, 32(1): 102 -109 .
[6] Wen XI,Zheng CHEN,Shi HU. Research Progress of Deformation Induced Localized Solid-state Amorphization in Nanocrystalline Materials[J]. Materials Reports, 2018, 32(1): 116 -121 .
[7] Xing LIANG, Guohua GAO, Guangming WU. Research Development of Vanadium Oxide Serving as Cathode Materials for Lithium Ion Batteries[J]. Materials Reports, 2018, 32(1): 12 -33 .
[8] Hao ZHANG,Yongde HUANG,Yue GUO,Qingsong LU. Technological and Process Advances in Robotic Friction Stir Welding[J]. Materials Reports, 2018, 32(1): 128 -134 .
[9] Laima LUO, Mengyao XU, Xiang ZAN, Xiaoyong ZHU, Ping LI, Jigui CHENG, Yucheng WU. Progress in Irradiation Damage of Tungsten and Tungsten AlloysUnder Different Irradiation Particles[J]. Materials Reports, 2018, 32(1): 41 -46 .
[10] Fengsen MA,Yan YU,Jie ZHANG,Haibo CHEN. A State-of-the-art Review of Cytotoxicity Evaluation of Biomaterials[J]. Materials Reports, 2018, 32(1): 76 -85 .
Viewed
Full text


Abstract

Cited
  Shared   
  Discussed