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材料导报  2024, Vol. 38 Issue (24): 23100004-13    https://doi.org/10.11896/cldb.23100004
  无机非金属及其复合材料 |
低对称性二维层状过渡金属硫族化合物合金及异质结的化学气相沉积法制备研究进展
邢欢欢1,†, 胡萍1,†, 罗政2, 毛丽秋1, 盛丽萍1,*, 王珊珊2,*
1 湖南师范大学化学化工学院,石化新材料与资源精细利用国家地方联合工程实验室,长沙 410081
2 国防科技大学空天科学学院,新型陶瓷纤维及其复合材料国防科技重点实验室,长沙 410073
Research Progress on Chemical Vapor Deposition Synthesis of Two-dimensional Layered Transition Metal Dichalcogenides Alloys and Heterojunctions with Low Symmetry
XING Huanhuan1,†, HU Ping1,†, LUO Zheng2, MAO Liqiu1, SHENG Liping1,*, WANG Shanshan2,*
1 National Local Joint Engineering Laboratory for New Petro-chemical Materials and Fine Utilization of Resources, College of Chemistry and Chemical Engineering, Hunan Normal University, Changsha 410081, China
2 Science and Technology on Advanced Ceramic Fibers and Composites Laboratory, College of Aerospace Science and Engineering, National University of Defense Technology, Changsha 410073, China
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摘要 低对称性二维过渡金属硫族化合物(TMDs)合金及异质结是一类面外为层状结构、面内对称元素少的功能纳米材料。它不仅表现出丰富可调的电子能带结构,且在光学、电学、力学等方面显示出独特的各向异性物理特性,因而在偏振光探测器、各向异性逻辑电路、触觉传感器等领域具有广阔应用前景。低对称性二维TMDs合金及异质结的可控制备是发挥其优异性能、保障其潜在应用的前提。本文首先按照元素种类的不同从二维铼(Re)基低对称合金和二维碲(Te)基低对称合金两方面对低对称性二维TMDs合金的化学气相沉积法制备进行归纳。然后,按照异质结构的不同从垂直异质结和水平异质结两方面梳理了低对称性二维TMDs异质结制备的最新进展。最后,对该领域现阶段存在的问题及挑战进行了总结与展望。
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邢欢欢
胡萍
罗政
毛丽秋
盛丽萍
王珊珊
关键词:  低对称性  二维  合金  异质结  化学气相沉积法    
Abstract: Two-dimensional (2D) transition metal chalcogenide (TMDs) alloys and heterojunctions with low symmetry are a class of functional nanomaterials with layered structure outside the plane and few symmetrical elements inside the plane. It not only shows rich adjustable electronic band structure, but also shows unique anisotropic physical properties in optics, electricity, mechanics, etc. so it has broad application prospects in the fields of polarized light detector, anisotropic logic circuit, tactile sensor and so on. The controllable preparation of low symmetry 2D TMDs alloys and heterojunctions is a prerequisite for their excellent properties. In this work, according to the different types of elements, the chemical vapor deposition of two-dimensional rhenium (Re)-base low-symmetry alloys and two-dimensional tellurium (Te) -base low-symmetry alloys is summarized. Then, according to the difference of heterostructures, the latest progress in the preparation of low symmetry two-dimensional TMDs heterojunctions is reviewed from the aspects of vertical heterojunctions and horizontal heterojunctions. Finally, the problems and challenges in this field are summarized and prospected.
Key words:  low symmetry    two-dimensional    alloy    heterojunctions    chemical vapor deposition
出版日期:  2024-12-25      发布日期:  2024-12-20
ZTFLH:  TB34  
基金资助: 国家自然科学基金(52172032;52222201); 中国科协青年科技精英资助计划 (YESS20200222); 湖南省自然科学基金(2022JJ20044); 国家国防科技工业局(WDZC20195500503); 国防科技大学(ZK18-01-03)
通讯作者:  * 盛丽萍,湖南师范大学化工学院副教授,博士生和硕士研究生导师。本硕博先后就读于湖南师范大学、中南大学、国防科技大学。主讲课程为《结构化学》《化学综合实验》。目前研究方向为耐高温和疏水高分子复合材料。主持过国家自科、省重点研发计划、省自科、军口横向、地方企业项目等,参与其他项目多项。已发表SCI论文30余篇,申请及授权专利共8项。 sleeping1217@126.com;王珊珊,国防科技大学副研究员。牛津大学材料学博士(师从Jamie Warner教授),北京大学化学博士后(师从张锦教授)。致力于低维功能材料的原子级结构与性质研究。以第一/通信作者在Chemical Society Reviews、Chem、Matter、ACS Nano(9篇)、Small等期刊发表论文20余篇。获国家优秀青年科学基金、湖南省优秀青年科学基金、欧洲显微学大会“青年科学家”奖,入选中国科协“青年人才托举”工程。 wangshanshan08@nudt.edu.cn   
作者简介:  邢欢欢,2021年6月在郑州师范学院获得工学学士学位,现为湖南师范大学化学化工学院硕士研究生(国防科技大学联合培养),在王珊珊老师的指导下,硕士期间主要研究低对称性二维硒化铼的化学气相沉积法制备及形貌调控。胡萍,2020年6月和2023年6月于上饶师范学院和湖南师范大学获获得理学学士学位和理学硕士学位,现为中国电子科技集团有限公司研发工程师。硕士期间于国防科技大学进行联合培养,在王珊珊老师的指导下主要研究低对称性二维硫化铼及其异质结的化学气相沉积法制备;以第一作者在Advanced Functional Materials期刊发表论文1篇,授权专利1项。
†共同第一作者
引用本文:    
邢欢欢, 胡萍, 罗政, 毛丽秋, 盛丽萍, 王珊珊. 低对称性二维层状过渡金属硫族化合物合金及异质结的化学气相沉积法制备研究进展[J]. 材料导报, 2024, 38(24): 23100004-13.
XING Huanhuan, HU Ping, LUO Zheng, MAO Liqiu, SHENG Liping, WANG Shanshan. Research Progress on Chemical Vapor Deposition Synthesis of Two-dimensional Layered Transition Metal Dichalcogenides Alloys and Heterojunctions with Low Symmetry. Materials Reports, 2024, 38(24): 23100004-13.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.23100004  或          http://www.mater-rep.com/CN/Y2024/V38/I24/23100004
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