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材料导报  2024, Vol. 38 Issue (14): 22110145-15    https://doi.org/10.11896/cldb.22110145
  无机非金属及其复合材料 |
氧化亚铜基光催化剂的制备及降解性能研究进展
赵强1,2, 李淑英1,3, 郭智楠1, 许琳1, 赵一博1, 吕靖1,3, 尚建鹏1,2, 郭永1,2, 王俊丽1,3,*
1 山西大同大学化学与化工学院, 山西 大同 037009
2 山西大同大学山西省清洁能源材料联合实验室,山西 大同 037009
3 煤基生态碳汇技术教育部工程研究中心,山西 大同 037009
Progress in the Preparation and Degradation Performance of Cuprous Oxide-based Photocatalysts
ZHAO Qiang1,2, LI Shuying1,3, GUO Zhinan1, XU Lin1, ZHAO Yibo1, LYU Jing1,3, SHANG Jianpeng1,2, GUO Yong1,2, WANG Junli1,3,*
1 School of Chemistry and Chemical Engineering, Shanxi Datong University, Datong 037009, Shanxi, China
2 Shanxi Province Union Laboratory of Clean Energy Materials, Shanxi Datong University, Datong 037009, Shanxi, China
3 Engineering Research Center of Coal-based Ecological Carbon Sequestration Technology of the Ministry of Education, Datong 037009, Shanxi, China
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摘要 Cu2O是一种p型半导体,在光催化领域有着广阔的应用前景。研究者通过调控Cu2O形貌和尺寸、构建异质结结构、设计复合材料增大比表面积和导电性等手段,提高其光利用率,降低了光生电子-空穴对复合率,从而提高了Cu2O 的光催化活性和光稳定性,促进了其在光催化降解染料领域的应用。本文重点综述了通过元素掺杂、半导体异质结构建及与其他材料复合的途径增强Cu2O光催化性能的方法,归纳了其在光催化降解有机污染物方面的应用及异质结增强机理,指出了目前研究存在的短板, 并对氧化亚铜基复合光催化的发展及应用前景进行了展望。
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赵强
李淑英
郭智楠
许琳
赵一博
吕靖
尚建鹏
郭永
王俊丽
关键词:  氧化亚铜  掺杂  半导体  异质结  光降解性能    
Abstract: Cu2O is a kind of p-type semiconductor, which has a wide application prospect in the field of photocatalysis. By adjusting the morphology and size of Cu2O, constructing the heterojunction structure, designing the composite material to increase the specific surface area and electrical conductivity, the light utilization rate of Cu2O was improved and the photogenerated electron-hole pair recombination rate was reduced, thus improving the photocatalytic activity and photostability of Cu2O, and promoting its application in the field of photocatalytic degradation of pollutant. In this paper, the methods to enhance the photocatalytic performance of Cu2O, including metal doping, semiconductor heterostructure construction and composites synthesis, were reviewed. Its application in photocatalytic degradation of organic pollutants and the enhancement mechanism of heterojunction were summarized. In addition, the shortcomings of current research were pointed out. The development and application prospect of cuprous oxide based photocatalysis were also prospected.
Key words:  cuprous oxide    doping    semiconductor    heterojunction    photodegradation performance
出版日期:  2024-07-25      发布日期:  2024-08-12
ZTFLH:  O643  
基金资助: 国家自然科学基金(21908135);山西省自然科学基金 (201901D111308;201901D211435;201801D221057);山西省留学回国人员科技活动项目择优资助(2019-20;20240027); 山西大同大学博士科研启动基金(2018-B-01; 2020-B-02);山西大同大学研究生创新基金(21CX22;22CX17);山西省大学生创新创业训练计划项目(20220807;2016172)
通讯作者:  * 王俊丽,山西大同大学化学与化工学院正高级实验师、硕士研究生导师。2005年太原师范学院化学系化学教育专业本科毕业,2008年太原理工大学物理化学专业硕士毕业后到山西大同大学工作至今,2017年太原理工大学化学工程与技术专业博士毕业。目前主要从事低阶煤及生物质热解和光催化降解等方面的研究工作。发表论文20余篇,包括Energy Conversion and Management、Fuel、Energy &Fuels、《燃料化学学报》等。出版专著1部。wangjunlitylg@126.com   
作者简介:  赵强,山西大同大学化学与化工学院教授、硕士研究生导师。2003年雁北师范学院化学系化学教育专业本科毕业,2007年太原理工大学高分子化学与物理专业硕士毕业后到山西大同大学工作至今,2021年日本弘前大学安全系统工程专业博士毕业。目前主要从事光催化等方面的研究工作。发表论文20余篇,包括Separation and Purification Technology、ACS Applied Nano Materials、Journal of Photochemistry & Photobiology A: Chemistry等。出版专著1部。
引用本文:    
赵强, 李淑英, 郭智楠, 许琳, 赵一博, 吕靖, 尚建鹏, 郭永, 王俊丽. 氧化亚铜基光催化剂的制备及降解性能研究进展[J]. 材料导报, 2024, 38(14): 22110145-15.
ZHAO Qiang, LI Shuying, GUO Zhinan, XU Lin, ZHAO Yibo, LYU Jing, SHANG Jianpeng, GUO Yong, WANG Junli. Progress in the Preparation and Degradation Performance of Cuprous Oxide-based Photocatalysts. Materials Reports, 2024, 38(14): 22110145-15.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.22110145  或          http://www.mater-rep.com/CN/Y2024/V38/I14/22110145
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