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材料导报  2025, Vol. 39 Issue (3): 23080074-18    https://doi.org/10.11896/cldb.23080074
  无机非金属及其复合材料 |
富锂锰基正极材料研究进展
童汇1,2, 谢建龙1,3, 张志谋1, 郭忻3, 喻万景1,2,*, 郭学益1,2, 黄承焕1,3,*
1 中南大学冶金与环境学院,长沙 410083
2 有色金属资源循环利用国家地方联合工程研究中心,长沙 410083
3 湖南长远锂科新能源有限公司,长沙 410205
Research Progress of Li-rich Mn-based Cathode Materials
TONG Hui1,2, XIE Jianlong1,3, ZHANG Zhimou1, GUO Xin3, YU Wanjing1,2,*, GUO Xueyi1,2, HUANG Chenghuan1,3,*
1 School of Metallurgy and Environment, Central South University, Changsha 410083, China
2 National & Regional Joint Engineering Research Center of Nonferrous Metal Resource Recycling, Changsha 410083, China
3 Hunan Changyuan Lico New Energy Co., Ltd., Changsha 410205, China
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摘要 富锂锰基材料(LRMOs)因具有能量密度高、成本低和环境友好等优点而备受青睐。然而,LRMOs存在首次库仑效率低、循环性能和倍率性能差等固有缺陷,限制了其商业化应用。为了应对这些局限,研究者们对LRMOs的制备方法不断进行改进,并且提出了多种改性措施,使得 LRMOs 的性能显著提高。本文介绍了LRMOs的组成与结构、充放电机理,总结了LRMOs的最新研究进展,包括制备方法、面临的挑战和常见改性策略,并指明了未来LRMOs的研究重点,为今后LRMOs的研究及开发提供了重要参考。
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童汇
谢建龙
张志谋
郭忻
喻万景
郭学益
黄承焕
关键词:  富锂锰基材料  锂离子电池  改性  电化学性能    
Abstract: Li-rich Mn-based materials (LRMOs) are highly favored due to their high energy density, cost-effectiveness, and eco-friendliness. However, LRMOs have inherent defects such as low initial Coulombic efficiency, poor cycling and rate performance, which limit their commercial application. In order to address these limitations, researchers have been working on enhancing the preparation techniques of LRMOs and proposing various modification strategies, which have significantly improved the performance of LRMOs. This summary introduces the composition, structure, charging and discharging mechanisms of LRMOs. It summarizes the latest research progress of LRMOs, including preparation methods, challenges faced, and common modification strategies. Moreover, it highlights the future research focus of LRMOs. This work provides valuable references for the research and development of LRMOs in the future.
Key words:  Li-rich Mn-based material    lithium ion battery    modification    electrochemical performance
出版日期:  2025-02-10      发布日期:  2025-02-05
ZTFLH:  TM912  
基金资助: 国家自然科学基金(52227806);长沙市重大科技攻关项目(kh2301024);中南大学前沿交叉项目(2023QYJC027)
通讯作者:  *喻万景,博士,中南大学冶金与环境学院副教授、硕士研究生导师。主要研究方向为低维碳基纳米复合电极材料与新型储能器件、有色金属资源的综合利用等。yuwj2005@163.com; 黄承焕,博士,湖南长远锂科股份有限公司正高级工程师,中南大学硕、博士研究生校外兼职指导老师。主要从事锂离子电池正极材料开发、锂离子电池失效机理研究。chhuang@minmetals.com   
作者简介:  童汇,日本九州大学博士,美国纽约大学博士后。现为中南大学冶金与环境学院教授、博士研究生导师。主要研究方向为新型储能电池材料的设计与开发、失效动力电池清洁回收与循环利用、有色金属资源综合利用等。
引用本文:    
童汇, 谢建龙, 张志谋, 郭忻, 喻万景, 郭学益, 黄承焕. 富锂锰基正极材料研究进展[J]. 材料导报, 2025, 39(3): 23080074-18.
TONG Hui, XIE Jianlong, ZHANG Zhimou, GUO Xin, YU Wanjing, GUO Xueyi, HUANG Chenghuan. Research Progress of Li-rich Mn-based Cathode Materials. Materials Reports, 2025, 39(3): 23080074-18.
链接本文:  
http://www.mater-rep.com/CN/10.11896/cldb.23080074  或          http://www.mater-rep.com/CN/Y2025/V39/I3/23080074
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