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材料导报  2026, Vol. 40 Issue (8): 25040273-18    https://doi.org/10.11896/cldb.25040273
  无机非金属及其复合材料 |
含氟温室气体的捕集及转化研究进展
李阿婷, 赵文波, 徐志勇*
昆明理工大学化学工程学院,昆明 650000
Research Progress on Capture and Conversion of Fluorinated Greenhouse Gases
LI Ating, ZHAO Wenbo, XU Zhiyong*
College of Chemical Engineering, Kunming University of Science and Technology, Kunming 650000, China
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输出:  BibTeX | EndNote (RIS)      
摘要 含氟温室气体(F-gases)在电子半导体工业和制冷与绝缘领域中具有重要的应用,然而这些气体通常具有较高的全球变暖潜能值(GWP),即使排放少量F-gases也会对气候产生长期且严重的影响。因此,F-gases的捕集对于实现半导体产业的可持续发展具有重要意义。传统的捕集方法,如低温冷凝和膜分离,存在效率低和能耗高等问题。近年来,多孔材料(如金属有机框架(MOFs)、共价有机框架(COFs)、氢键有机框架(HOFs)、多孔有机笼(POCs)等)和离子液体(ILs)等新型材料在F-gases捕集方面展现出巨大潜力。此外,催化转化法也为F-gases的后续处理提供了新的思路。本文综合阐述了F-gases的分离捕集与催化转化技术的研究进展,从基于孔隙工程、复合材料设计等方面出发,总结了功能化MOFs的优势;剖析了氟化离子液体吸收F-gases的机理及面临的挑战;同时探讨了催化转化法在处理F-gases中的潜力以及存在的问题。
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李阿婷
赵文波
徐志勇
关键词:  含氟温室气体  金属有机框架  离子液体  催化转化  吸附分离    
Abstract: Fluorinated greenhouse gases (F-gases) play a critical role in the electronics and semiconductor industry as well as in refrigeration and electrical insulation applications. However, these gases typically exhibit high global warming potentials (GWPs), meaning even small emissions can cause severe long-term climatic impacts. Therefore, the capture of F-gases is essential for achieving sustainable development in the semiconductor industry. Conventional capture methods, such as cryogenic condensation and membrane separation, face challenges including low efficiency and high energy consumption. In recent years, novel porous materials, such as metal-organic frameworks (MOFs), covalent organic frameworks (COFs), hydrogen-bonded organic frameworks (HOFs), porous organic cages (POCs) and ionic liquids (ILs) have demonstrated significant potential for F-gases capture. Additionally, catalytic conversion methods are new approaches for the subsequent treatment of F-gases. This review comprehensively summarizes recent advances in the separation, capture, and catalytic conversion technologies for F-gases. It highlights the advantages of functionalized MOFs based on pore engineering and composite material design, analyzes the mechanisms and challenges in the absorption of F-gases using fluorinated ionic liquids, and explores the potential and existing issues of catalytic conversion methods for treating F-gases.
Key words:  F-gases    MOFs    ionic liquids (ILs)    catalytic conversion    adsorption separation
出版日期:  2026-04-25      发布日期:  2026-05-06
ZTFLH:  TQ11  
基金资助: 云南省基础研究计划(202501CF070138)
通讯作者:  * 徐志勇,昆明理工大学特聘教授/硕士研究生导师。近年来主要从事酸性、电子特种气体的捕集和复杂体系的分子模拟研究。ZYXu@kust.edu.cn   
作者简介:  李阿婷,昆明理工大学化学工程学院硕士研究生,主要研究领域为新型多孔碳材料的制备及含氟温室气体的吸附分离。
引用本文:    
李阿婷, 赵文波, 徐志勇. 含氟温室气体的捕集及转化研究进展[J]. 材料导报, 2026, 40(8): 25040273-18.
LI Ating, ZHAO Wenbo, XU Zhiyong. Research Progress on Capture and Conversion of Fluorinated Greenhouse Gases. Materials Reports, 2026, 40(8): 25040273-18.
链接本文:  
https://www.mater-rep.com/CN/10.11896/cldb.25040273  或          https://www.mater-rep.com/CN/Y2026/V40/I8/25040273
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