煤气化渣胶凝活性激发及机理研究进展

doi:10.11896/cldb.24030152

材料导报

2025, Vol. 39

Issue (12): 24030152-9 https://doi.org/10.11896/cldb.24030152

无机非金属及其复合材料

煤气化渣胶凝活性激发及机理研究进展

吴平川^1,2, 刘治兵^1,2, 黄天勇^1,*, 郑永超¹, 张凯帆³, 王长龙^1,2,4,*, 康旺¹, 付兴帅², 白云翼², 翟玉新⁵, 刘枫⁶

1 北京建筑材料科学研究总院有限公司,固废资源化利用与节能建材国家重点实验室,北京 100041
2 河北工程大学土木工程学院,河北省建筑工程低碳建造与韧性提升重点实验室,河北邯郸 056038
3 江西理工大学资源与环境工程学院,江西赣州 341000
4 武汉科技大学,国家环境保护矿冶资源利用与污染控制重点实验室,武汉 430081
5 中铁建设集团有限公司,北京 100040
6 中铁建设集团建筑发展有限公司,北京 100070

Research Progress on Excitation and Mechanism of Coal Gasification Slag Cementitious Reactivity

WU Pingchuan^1,2, LIU Zhibing^1,2, HUANG Tianyong^1,*, ZHENG Yongchao¹, ZHANG Kaifan³,WANG Changlong^1,2,4,*, KANG Wang¹, FU Xingshuai², BAI Yunyi², ZHAI Yuxin⁵, LIU Feng⁶

1 State Key Laboratory of Solid Waste Reuse for Building Materials, Beijing Building Materials Academy of Sciences Research, Beijing 100041, China
2 Hebei Province Key Laboratory for Low-Carbon Construction and Resilience Enhancement of Construction Engineering, School of Civil Engineering, Hebei University of Engineering, Handan 056038, Hebei, China
3 School of Resources and Environmental Engineering, Jiangxi University of Science and Technology, Ganzhou 341000,Jiangxi, China
4 State Environmental Protection Key Laboratory of Mineral Metallurgical Resources Utilization and Pollution Control, Wuhan University of Science and Technology, Wuhan 430081, China
5 China Railway Construction Group Co., Ltd., Beijing 100040, China
6 Construction Development Co., Ltd., China Railway Construction Group, Beijing 100070, China

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摘要煤气化渣作为煤化工产业的主要固体废弃物,具有堆存量大、含碳量高、胶凝活性弱及重金属赋存等特点,其规模化无害化利用面临挑战。本文系统综述了煤气化渣的矿物学特性及其胶凝活性提升的影响机制,研究表明,煤气化渣中高聚合度的铝硅酸盐玻璃体及残碳是限制其活性的核心因素,物理活化通过机械研磨破坏晶体结构并增大比表面积,但作用效果有限;化学活化主要通过酸、碱、盐、有机溶剂,解聚铝硅酸盐玻璃体网络结构,释放活性Al³⁺、Si⁴⁺、Ca²⁺离子提升活性,但需精确控制水化反应;热活化可通过高温消除残碳与重构煤气化渣的晶相,但能耗较高;复合活化及生物矿化展现出协同增效的潜力,但目前研究较少。未来需从煤气化渣矿物学特性出发,开发低碳高效的多技术联用路径,突破高掺量应用瓶颈,为煤气化渣建材化高值化利用提供理论支撑。

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	吴平川
	刘治兵
	黄天勇
	郑永超
	张凯帆
	王长龙
	康旺
	付兴帅
	白云翼
	翟玉新
	刘枫

关键词: 煤气化渣矿物学特性胶凝活性激发机理资源化利用

Abstract: Coal Gasification slag, a solid waste produced during the process of coal gasification, has some characteristics such as a large storage vo-lume, high carbon content, weak cementitious reactivity, and heavy metal enrichment, and its large-scale and harmless utilization faces significant challenges. This paper systematically reviews the mineralogical properties of coal gasification slag and the mechanisms influencing its cementitious reactivity enhancement. The study shows that the highly polymerized aluminosilicate glass phase and residual carbon in coal gasification slag are the core factors limiting its reactivity. physical activation through mechanical grinding to destroy the crystal structure and increase the specific surface area, but the role of the effect is limited. chemical activation is mainly through the acid, alkali, salt, organic solvents to depolymerize the aluminosilicate network to release active ions (Al³⁺, Si⁴⁺, Ca²⁺), but requires precise control of hydration reaction pathways. Thermal activation removes residual carbon and reconstructs crystalline phases through high-temperature treatment, yet faces high energy consumption. Composite activation and bio-mineralization techniques demonstrate synergistic potential, but the current research is insufficient. In the future, it is necessary to develop low-carbon and high-efficiency multi-technology paths from the mineralogical properties of coal gasification slag, overcome bottlenecks in high-dosage applications, and provide theoretical foundations for high-value utilization of coal gasification slag as building mate-rials.

Key words: coal gasification slag mineralogy characteristics cementitious reactivity excitation mechanism resource utilization

出版日期: 2025-06-25 发布日期: 2025-06-19

ZTFLH:

TU526

基金资助: 国家重点研发计划(2021YFC1910605);河北省自然科学基金(E2020402079);河北省科技重大专项项目(21283804Z);固废资源化利用与节能国家重点实验室开放基金( SWR-2023-007);国家环境保护矿冶资源利用与污染控制重点实验室开放基金(HB202306);河北省建筑工程低碳建造与韧性提升重点实验室基金资助(HKL-LRC-2024-2)

通讯作者: ^*黄天勇,博士,北京建筑材料科学研究总院有限公司正高级工程师,博士研究生导师。长期从事预拌砂浆、混凝土及固体废弃物资源化利用研究。hatty555@163.com
王长龙,博士,河北工程大学教授,博士研究生导师。长期从事固废高值利用理论及关键技术研究。baistuwong@139.com

作者简介: 吴平川,博士,河北工程大学教授,硕士研究生导师。长期从事新型低碳环境生态材料、绿色混凝土研究。

引用本文:

吴平川, 刘治兵, 黄天勇, 郑永超, 张凯帆, 王长龙, 康旺, 付兴帅, 白云翼, 翟玉新, 刘枫. 煤气化渣胶凝活性激发及机理研究进展[J]. 材料导报, 2025, 39(12): 24030152-9.
WU Pingchuan, LIU Zhibing, HUANG Tianyong, ZHENG Yongchao, ZHANG Kaifan,WANG Changlong, KANG Wang, FU Xingshuai, BAI Yunyi, ZHAI Yuxin, LIU Feng. Research Progress on Excitation and Mechanism of Coal Gasification Slag Cementitious Reactivity. Materials Reports, 2025, 39(12): 24030152-9.

链接本文:

https://www.mater-rep.com/CN/10.11896/cldb.24030152 或 https://www.mater-rep.com/CN/Y2025/V39/I12/24030152

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