氧化物固体电解质的三维框架结构设计及在全固态锂离子电池中的应用

doi:10.11896/cldb.22020093

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Abstract Due to the advantages of all-solid-state lithium batteries in safety, energy density and working temperature range, the development of solid electrolytes is a crucial step to breaking through the technical bottleneck of lithium batteries and further industrialization. Because of the problems of filler particle agglomeration in composite electrolytes and electrolyte/electrode interfaces, several innovative inorganic electrolyte designs have recently been proposed. This review paper begins with a brief discussion of ion transport pathways in a composite electrolyte based on a three-dimensional oxide solid electrolyte framework, describing the effects that the electrolyte structure may have on ion transport. The designs and application of different types of 3D framework structures of oxide solid electrolyte reported in recent years, together with their preparation methods are then highlighted. We also detail the optimization strategies of the different designs of the structure for the electrochemical perfor-mance of the batteries and make a comparison between them. The 3D oxide solid electrolyte framework can not only be used as the matrix of composite electrolyte but also be filled with electrode materials to form a composite electrode, which provides a new contact form between the electrode and the electrolyte, aiming to solve the problems of volume change and lithium dendrite growth. At the end of this review, the design ideas and ongoing challenges are summarized.

Key words： composite solid electrolyte three-dimensional framework Li⁺ conductivity all-solid-state lithium battery porous material

Published: 10 October 2023 Online: 2023-09-28

CLC number:

TM912

Fund:Guangdong Major Project of Basic and Applied Basic Research (2021B0301030001), Shenzhen Science and Technology Project (JCYJ20190809153405505), the National Natural Science Foundation of China (51972246, 51521001), the National Key Research and Deve-lopment Program of China (2018YFB0905600), Fundamental Research Funds for the Central Universities in China and the ‘111' Project (B13035).

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	Articles by authors
	CHEN Fei
	Rannalter Leana Ziwen
	SONG Shangbin
	CAO Shiyu
	SHEN Qiang

Cite this article:

CHEN Fei,Rannalter Leana Ziwen,SONG Shangbin, et al. Three-dimensional Structural Design in Oxide Solid Electrolytes and Its Application in All-Solid-State Lithium-ion Batteries[J]. Materials Reports, 2023, 37(19): 22020093-15.

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http://www.mater-rep.com/EN/10.11896/cldb.22020093 OR http://www.mater-rep.com/EN/Y2023/V37/I19/22020093

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