3D打印石墨烯增强复合材料研究进展

doi:10.11896/cldb.19040048

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Abstract In recent years, graphene has become a research hotspot on account of its outstanding mechanical and thermal properties and the feasibility of mass production. If it used as a reinforcing phase in materials such as metals, polymers, and ceramics that is promising for enhancing the comprehensive performance of the composites. To meet the ever-increasing demand for composites performance optimization, widely varieties of manufacturing methods for the preparing graphene-based composites have emerged, in which 3D printing technology can achieve the perfect combination of process flexibility and high performance products.
However, graphene has a low density and is easily agglomerated due to its large specific surface area, which will affect the mechanical properties of the composites. In addition, poor wettability of graphene with ceramic or metal matrix cannot ensure a good interfacial bonding between graphene and the matrix. Therefore, how to uniformly disperse graphene in composites has been the research direction of researchers. Currently, the commonly used disperse graphene methods include solution mixing method, melt mixing method, in-situ mixing method and mechanical ball mil-ling method, they are widely used in the preparation of metal, polymer and ceramic composites. Among them, mechanical properties of metal or ceramic composites with uniform dispersion graphene were improved, and they got a good incorporation at the interface. In addition, the more researched graphene-reinforced polymer composites’mechanical properties, thermal and electrical characteristics have been significantly enhanced, and they were used in biomedical or energy storage fields,showing better biological or electrical properties.
This paper reviews the research progress of 3D-printed graphene-based composites from three aspects: metal materials, polymers and ceramic matrix composites. The application of graphene-reinforced composites are elaborated in 3D printing from milling and forming. In the future, graphene-reinforced composites are expected to widely used in energy devices, biological scaffolds and aerospace fields, which will extend a broader space for material research.

Key words： 3D printing graphene-reinforced composites metal polymer ceramic

Published: 27 April 2020

CLC number:

TB333

Fund:This work was financially supported by the National Natural Science Foundation of China (51804280), the Natural Science Foundation of Shanxi Province, China (201701D221086, 201801D221146), the Major Science and Technology Projects of Shanxi Province, China (20181101009), Department of Scientific and Technologial Innovation Programs of Higher Education Institutions in Shanxi (201802076), Returned Overseas Students Research Funding Project of Shanxi Province (2017-095), International Cooperation Project of Shanxi Province (201603D421024), the Support Program for Young Academic Leaders of North University of China, China (QX201802).

About author:: Denghao Yi received his B.S. degree in applied chemistry from North University of China in 2017. He is currently pursuing master’s degree at the School of Material Science and Engineering, North University of China under the supervision of A/Prof. Li Xiaofeng. His research has focused on the preparation of graphene reinforced nickel matrix composites by selective laser melting (SLM).
Xiaofeng Li received his B.E. degree in material from Central South University in 2009 and received his Ph.D. degree in State Key Laboratory for Powder Metallurgy from Central South University, in 2016. He is currently an associate professor and master’s supervisor in North University of China. His research interests are powder metallurgy, additive manufacturing, design and deve-lopment of metal matrix composites.

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	YI Denghao
	FENG Yinghao
	ZHANG Jinfang
	LI Xiaofeng
	LIU Bin
	LIANG Minjie
	BAI Peikang

Cite this article:

YI Denghao,FENG Yinghao,ZHANG Jinfang, et al. Research Progress of 3D-printed Graphene-reinforced Composites[J]. Materials Reports, 2020, 34(9): 9086-9094.

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http://www.mater-rep.com/EN/10.11896/cldb.19040048 OR http://www.mater-rep.com/EN/Y2020/V34/I9/9086

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