气相臭氧分解催化材料的研究进展

doi:10.11896/cldb.21060087

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Abstract Advanced oxidation technology involving strong oxidizing ozone has been applied in the fields of water treatment, air purification and sterilization. But the excessive discharge of ozone causes substantial air pollution and represents a major hazard to human health. Compared to typical ozone treatment procedures, such as adsorption, thermal decomposition, absorption and so on, catalytic ozone decomposition has garnered a lot of attention since it is very efficient, safe and environmentally benign. Up to now, great progress has been made on catalysts for ozone decomposition. The types of catalysts have become more abundant, including activated carbon, noble metals, transition metal oxides, metal-organic framework materials, etc., and their application forms have evolved from powder-based materials to monolithic materials.
Nevertheless, two major difficulties severely limit the practical application of catalysts: on the one hand, catalyst deactivation is unavoidable due to the accumulation of intermediate oxygen species at surface active sites, which is the rate-limiting phase of the reaction. On the other hand, due to the intense competing adsorption between water molecules and ozone at active sites, catalysts are rapidly poisoned in moist conditions. As a result, catalysts with high catalytic activity and water resistance are highly desirable.
To enhance the catalytic property, some effective strategies, including enlarging the surface area, fabricating oxygen vacancy, regulating lattice plane, doping and surface modification, are used to increase the concentration of active sites and accelerate the electron transfer. While hydrophobic treatment is a common approach to improve water resistance. Furthermore, researchers have shown in recent years that water can ope-rate as a promoter at some specific active sites, which not only boosts catalytic activity but also prevents unstable performance caused by water adsorption competition.
This overview covers the research progress of catalytic ozone decomposition materials, as well as the gas ozone decomposition reaction process and mechanism. Especially, the advantages and challenges of various catalysts are summarized and the strategies for improving the activity and stability are highlighted. This review serves as a good reference for the preparation of stable and efficient catalytic ozone decomposition materials and the large-scale application of ozone oxidation technology in the chemical industry.

Key words： environmental pollution ozone decomposition catalyst activity stability

Published: 30 November 2021

CLC number:

TB34

Fund:National Natural Science Foundation of China (U1862111) and Sichuan Science and Technology Program (2020ZDZX0008).

About author:: Ruiyang Zhang received his B.C from Henan Polytechnic University in 2012 and his Ph.D. at Southwest Petroleum University in 2020. Currently he is a lecturer at Southwest Petroleum University. His main research interest is the development and application of environmental functional materials.
Ying Zhou received his B.C and MSc from Central South University and Chinese Academy of Sciences, respectively. In 2010, he received his Ph.D. at the University of Zurich (UZH) under the supervision of Prof. Greta R. Patzke. He then continued his work with a postdoctoral Forschungskredit grant from UZH. He was also awarded a fellowship by the Alexander von Humboldt Foundation at Karlsruhe Institute of Technology with Prof. Jan-Dierk Grunwaldt and was a visiting professor at Kyoto University. He currently holds a professorship at Southwest Petroleum University. His research interest is in the clean utilization of oil and gas and environmental remediation materials as well as the related in situ characterization techniques.

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	ZHANG Ruiyang
	WANG Shuyan
	LI Bangxin
	ZHANG Aili
	ZHANG Qian
	ZHOU Ying

Cite this article:

ZHANG Ruiyang,WANG Shuyan,LI Bangxin, et al. Research Progress of Gaseous Ozone Decomposition Catalysts[J]. Materials Reports, 2021, 35(21): 21037-21049.

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http://www.mater-rep.com/EN/10.11896/cldb.21060087 OR http://www.mater-rep.com/EN/Y2021/V35/I21/21037

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