电化学方法制备MOF膜的研究进展

doi:10.11896/cldb.19070010

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Abstract Metal-organic frameworks (MOFs) are highly-ordered porous network frameworks constructed from metallic nodes and organic ligands linked together with coordination bonds. MOFs have significant potential applications in gas adsorption, storage, catalysis, sensing, magnetism, optics, electrochemistry, drug delivery, etc. because of their large surface area, designable and tunable structures and nature and strength of host-guest interactions. They have become one of the highest-growing types of functional nanostructured porous solids in the past two decades.
MOFs as thin films are much more desirable than MOFs as bulk crystals in the development of MOFs-based components and devices. But the synthesis of defect-free MOF films is still a challenge. The methods for MOF film preparation mainly include hydrothermal synthesis, microwave synthesis, ultrasonic synthesis, mechanical ball milling and electrochemical synthesis. Electrochemical synthesis, usually fast, under environmental temperature and pressure, and with less chemical reagents, has obvious advantages over other methods, which are generally considered as time-consuming and under strict conditions.
This paper reviews the relative progress in MOF film electrochemical synthesis techniques, anodic synthesis, cathode deposition, indirect bipolar electrodeposition (IBED), galvanic displacement, and electrophoretic deposition (EDP) and their applications over the last decade and highlight advantages and disadvantages of electrochemical synthesis methods above as well as the differences in their techniques and mechanisms.

Key words： metal-organic frameworks electrochemical synthesis films nanoporous materials

Published: 05 November 2020

CLC number:

TQ035

Fund:This work was financially supported by State Key Laboratories Development Program of China (2011DA105287-MS201402), Scientific Research Foundation for the Returned Overseas Chinese Scholars State Education Ministry((2010)609-1), and Scientific and Technological Research Program of Chongqing Municipal Education Commission(KJ08A02).

About author:: Jie Zhou, currently pursuing a master’s degree in environmental science and engineering in the School of Resources and Safety of Chongqing University, focusing on the electrochemical preparation of MOF membrane materials.
Mingli Yang, Ph.D., associate professor of Chongqing University, mainly engaged in teaching and scientific research in physical chemistry, biochemistry and related fields.

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Cite this article:

ZHOU Jie,YANG Mingli. Recent Research Progress in Electrochemical Preparation of MOF Films[J]. Materials Reports, 2020, 34(19): 19043-19049.

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http://www.mater-rep.com/EN/10.11896/cldb.19070010 OR http://www.mater-rep.com/EN/Y2020/V34/I19/19043

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