固态锂离子电池电解质材料应用性能的研究进展

doi:10.11896/cldb.24060166

材料导报

2025, Vol. 39

Issue (13): 24060166-20 https://doi.org/10.11896/cldb.24060166

无机非金属及其复合材料

固态锂离子电池电解质材料应用性能的研究进展

张笑儒^1,2, 宋静^2,*, 罗来马^1,3,*, 孙宏骞², 赵聪聪², 田硕², 田亮亮⁴, 吴玉程^1,3

1 合肥工业大学材料科学与工程学院,合肥 230009
2 中国科学院过程工程研究所,战略金属资源绿色循环利用国家工程研究中心,北京 100190
3 高性能铜合金材料及成形加工教育部工程研究中心,合肥 230009
4 重庆文理学院电子信息与电气工程学院,重庆 402160

Research Progress on Applicative Performance of Electrolyte Materials for Solid-state Lithium-ion Batteries

ZHANG Xiaoru^1,2, SONG Jing^2,*, LUO Laima^1,3,*, SUN Hongqian², ZHAO Congcong², TIAN Shuo², TIAN Liangliang⁴, WU Yucheng^1,3

1 School of Materials Science and Engineering, Hefei University of Technology, Hefei 230009, China
2 National Engineering Research Center for Green Recycling of Strategic Metal Resources, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, China
3 Engineering Research Center of High Performance Copper Alloy Materials and Processing, Ministry of Education, Hefei 230009, China
4 School of Electronic Information and Electrical Engineering, Chongqing University of Arts and Sciences, Chongqing 402160, China

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摘要随着新能源汽车和5G通信技术的快速发展,对锂离子电池作为动力源的综合性能提出了更高的要求。在众多锂离子电池技术的研发中,固态锂离子电池因其卓越的能量密度和安全性而受到广泛关注。固态电解质是锂离子电池的关键组成部分,其性能直接影响着电池的整体性能,设计和制造具有优良性能的固态电解质是推动锂离子电池实际应用的关键。本文分别对无机固态电解质、聚合物固态电解质和复合固态电解质中Li⁺传输机制进行了介绍,结合近年发表的文献,全面综述了研究人员利用离子掺杂和引入新的制备技术等方法对固态电解质性能进行改善的研究进展,总结了不同类型固态电解质在国内外各企业中的应用情况,最后对固态电解质存在的挑战和未来的发展趋势进行了展望。本文旨在为开发综合性能优异的新型固态电解质材料提供参考,促进固态电解质的产业化快速发展。

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	张笑儒
	宋静
	罗来马
	孙宏骞
	赵聪聪
	田硕
	田亮亮
	吴玉程

关键词: 固态锂离子电池固态电解质 Li⁺传输机制离子电导率电化学稳定性循环性能

Abstract: With the rapid development of new energy vehicles and 5G communication technology, higher requirements have been put forward for the comprehensive performance of lithium-ion as a power source. In the research and development of many lithium-ion battery technologies, so-lid-state lithium-ion batteries have attracted extensive attention due to their excellent energy density and safety. As a key component of lithium batteries, the performance of solid-state electrolytes directly affects the overall performance of the battery, and the design and manufacture of so-lid-state electrolytes with excellent performance is crucial for promoting the practical application of lithium-ion batteries. In this paper, the Li⁺ transport mechanism in inorganic solid-state electrolytes, polymer solid-state electrolytes and composite solid-state electrolytes is introduced, combined with the literature in recent years, the research progress of researchers using ion doping and the introduction of new preparation techniques to improve the performance of solid-state electrolytes is comprehensively reviewed, the application of different types of solid-state electrolytes in domestic and foreign enterprises is summarized, and finally the challenges and future development trends of solid-state electrolytes are prospected. The aim of this review is to provide useful information for developing new solid-state electrolyte materials with excellent comprehensive perfor-mance, so as to promote the rapid industrialization of solid-state electrolytes.

Key words: solid-state lithium-ion battery solid-state electrolyte Li⁺ transport mechanism ionic conductivity electrochemical stability cyclic performance

出版日期: 2025-07-10 发布日期: 2025-07-21

ZTFLH:

TM911.3

基金资助: 在渝高校与中科院所属院所合作项目(HZ2021013);重庆市自然科学基金创新发展联合基金(CSTB2023NSCQ-LZX0045)

通讯作者: *宋静,博士,副研究员,硕士研究生导师。2008年取得天津大学博士学位后进入中国科学院过程工程研究所进行博士后研究,出站后留所工作。主要研究方向:(1)锆资源清洁高效综合利用;(2)二氧化锆粉体材料的可控制备;(3)绿色制造系统集成。jsong@ipe.ac.cn
罗来马,浙江大学博士,合肥工业大学教授、博士研究生导师,主要从事核聚变材料、粉末冶金与高导热铜基材料研究。luolaima@126.com

作者简介: 张笑儒,2021年6月毕业于大连海事大学,获得专业硕士学位。现为合肥工业大学材料科学与工程学院能源动力专业博士研究生,在中国科学院过程工程研究所联合培养,并在罗来马教授和宋静副研究员的指导下进行研究,主要研究领域为固态电解质。

引用本文:

张笑儒, 宋静, 罗来马, 孙宏骞, 赵聪聪, 田硕, 田亮亮, 吴玉程. 固态锂离子电池电解质材料应用性能的研究进展[J]. 材料导报, 2025, 39(13): 24060166-20.
ZHANG Xiaoru, SONG Jing, LUO Laima, SUN Hongqian, ZHAO Congcong, TIAN Shuo, TIAN Liangliang, WU Yucheng. Research Progress on Applicative Performance of Electrolyte Materials for Solid-state Lithium-ion Batteries. Materials Reports, 2025, 39(13): 24060166-20.

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https://www.mater-rep.com/CN/10.11896/cldb.24060166 或 https://www.mater-rep.com/CN/Y2025/V39/I13/24060166

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