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材料导报  2025, Vol. 39 Issue (5): 24010256-13    https://doi.org/10.11896/cldb.24010256
  高分子与聚合物基复合材料 |
人工模拟酶的构建策略、分类及应用
李兆周1,2,†, 张孝冲1,2,†, 韦玉花1,2, 郭津瑞1,2, 赵明辉1,2, 王耀1,2,*, 万宁波1,2, 古绍彬1,2, 康怀彬1,2, 罗磊1,2
1 河南科技大学食品与生物工程学院,河南 洛阳 471000
2 河南省食品绿色加工与质量安全控制国际联合实验室,河南 洛阳 471000
Construction Strategies,Classifications and Applications of Artificial Enzyme Mimics
LI Zhaozhou1,2,†, ZHANG Xiaochong1,2,†, WEI Yuhua1,2, GUO Jinrui1,2, ZHAO Minghui1,2, WANG Yao1,2,*, WAN Ningbo1,2, GU Shaobin1,2, KANG Huaibin1,2, LUO Lei1,2
1 College of Food and Bioengineering, Henan University of Science and Technology, Luoyang 471000, Henan, China
2 Henan International Joint Laboratory of Food Green Processing and Quality Safety Control, Luoyang 471000, Henan, China
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摘要 人工模拟酶与天然酶具有相似的催化活性,兼有可调节性、稳定性、再生性和易于大规模制备等优点,在催化、分析检测、药物生产和能源开发等领域具有广阔的应用前景。本文根据天然酶结构、催化机制以及现有模拟酶的特点,阐述了模拟酶构建的基本策略,包括底物结合位点的构建以及催化基团的引入,分析了不同构建策略的特点,论述了相关的技术途径。根据模拟酶载体的不同,分别介绍了多肽模拟酶、纳米材料模拟酶和超分子模拟酶,并对各类模拟酶的催化机制和未来发展趋势进行了分析和展望,简述了它们在痕量物质分析、生物医学以及环境保护等方面的应用。本文为模拟酶的研制提供了理论参考,也为模拟酶的推广应用提供了技术支撑。
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作者相关文章
李兆周
张孝冲
韦玉花
郭津瑞
赵明辉
王耀
万宁波
古绍彬
康怀彬
罗磊
关键词:  模拟酶  构建策略  催化机制    
Abstract: Artificial enzyme mimics possess similar catalytic activities to natural enzymes and advantages of tunability, stability, reproducibility, and ease of large-scale production. They have broad application prospects in the fields of catalysis, sensing detection, drug production and energy exploitation. Based on the structures and catalytic mechanisms of natural enzymes and the characteristics of existing enzyme mimics, this paper expounds the basic strategies for the construction of enzyme mimics, including the construction of substrate binding sites and the introduction of ca-talytic groups. The characteristics of different construction strategies are investigated, and the related technical approaches are discussed. According to the different carriers of enzyme mimics, polypeptide enzyme mimics, nanomaterial enzyme mimics, and supramolecular enzyme mi-mics are introduced. Furthermore, the catalytic mechanisms and future development trends of various enzyme mimics are proposed and prospected, and their applications in trace matter analysis, biomedicine and environmental protection are also briefly summarized. The related contents provide theoretical references for the development of enzyme mimics and technical supports for their widespread applications.
Key words:  enzyme mimics    construction strategy    catalyst mechanism
出版日期:  2025-03-10      发布日期:  2025-03-18
ZTFLH:  O643.3  
基金资助: 洛阳市公益性行业科研专项(2202021A);河南省科技攻关计划(242102411001);河南省优秀青年科学基金(202300410121);国家自然科学基金(31701694;U1504330;31702218);河南省青年人才托举工程项目(2020HYTP029);河南省研究生教育改革与质量提升工程项目(HNYJS2020JD06)
通讯作者:  *王耀,博士,河南科技大学食品与生物工程学院副教授、硕士研究生导师,主要从事人工模拟酶及其应用研究。tiger861215@163.com   
作者简介:  李兆周,博士,河南科技大学食品与生物工程学院教授、硕士研究生导师,主要从事人工模拟酶及其应用研究。
张孝冲,河南科技大学硕士研究生,研究方向为分子印迹模拟酶及其应用。†共同第一作者
引用本文:    
李兆周, 张孝冲, 韦玉花, 郭津瑞, 赵明辉, 王耀, 万宁波, 古绍彬, 康怀彬, 罗磊. 人工模拟酶的构建策略、分类及应用[J]. 材料导报, 2025, 39(5): 24010256-13.
LI Zhaozhou, ZHANG Xiaochong, WEI Yuhua, GUO Jinrui, ZHAO Minghui, WANG Yao, WAN Ningbo, GU Shaobin, KANG Huaibin, LUO Lei. Construction Strategies,Classifications and Applications of Artificial Enzyme Mimics. Materials Reports, 2025, 39(5): 24010256-13.
链接本文:  
https://www.mater-rep.com/CN/10.11896/cldb.24010256  或          https://www.mater-rep.com/CN/Y2025/V39/I5/24010256
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