MOFs衍生物在尿素氧化中的研究进展

doi:10.11896/cldb.23020193

材料导报

2024, Vol. 38

Issue (6): 23020193-10 https://doi.org/10.11896/cldb.23020193

电化学能源材料与器件

MOFs衍生物在尿素氧化中的研究进展

张霞^1,2, 吴瑛^1,*, 袁牧锋³, 王春栋^2,*

1 塔里木大学化学化工学院,新疆阿拉尔 843300
2 华中科技大学集成电路学院,武汉 430074
3 香港中文大学(深圳)理工学院,广东深圳 518172

Recent Research Progress of MOFs Derivatives for Urea Oxidation

ZHANG Xia^1,2, WU Ying^1,*, YUEN Mufung³, WANG Chundong^2,*

1 School of Chemistry and Chemical Engineering, Tarim University, Alar 843300, Xinjiang, China
2 School of Integrated Circuits, Huazhong University of Science and Technology, Wuhan 430074, China
3 School of Science and Technology, The Chinese University of Hong Kong (Shenzhen), Shenzhen 518172, Guangdong, China

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摘要尿素氧化反应(UOR)在缓解现代氢能源制备和废水处理等压力中起着关键作用,引入性能优异的电催化剂有助于降低电化学能耗。金属-有机骨架(MOFs)衍生物因能克服MOFs原有导电性及稳定性差的固有缺陷备受关注,被认为是一种很有前途的电催化剂。本文回顾和总结了基于MOFs衍生物的设计和构建的相关研究:(i)基于镍基/非镍基的UOR的机理分析;(ii)概括了利用结构调控、形貌控制、界面工程和缺陷工程的手段提高电子电导率的策略,同时概括了材料物理特性改变与催化活性的相关性;(iii) MOFs衍生物基于UOR的应用研究。最后,对UOR的后期研究挑战和发展提出了合理的建议。

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	张霞
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	袁牧锋
	王春栋

关键词: MOFs衍生物尿素氧化反应结构调控形貌控制界面工程缺陷工程

Abstract: Urea oxidation reaction (UOR) plays an essential role in reducing the strain of contemporary hydrogen energy production and wastewater treatment, and the development of electrocatalysts with superior performance can aid in lowering the amount of energy required. Derivatives of metal-organic frameworks (MOFs) materials have garnered a lot of attention for their potential as electrocatalysts, by addressing the inherent flaws of poor conductivity and stability. With reference to the design and construction of MOF-derivatives, we review and summarize some studies based on: (i) the reaction mechanism of nickel-based/non-nickel-based UOR; (ii) strategies to improve the electronic conductivity by means of structural modulation, morphology control, interfacial engineering, and defect engineering, outlining the change in physical properties of the materials with respect to the catalytic activity correlation;(iii) analyses of the applications of UOR-based MOFs derivatives. Finally, we give some perspectives on the most recent research challenges and developments in UOR.

Key words: MOFs derivatives urea oxidation reactions structure modulation morphology control interface engineering defect engineering

出版日期: 2024-03-25 发布日期: 2024-04-07

ZTFLH:

TQ150

基金资助: 新疆建设兵团南疆重点产业创新发展支撑计划项目(2020DB002;2022DB009);深圳市自然科学基金面上项目(JCYJ20190813172609404)

通讯作者: ^*吴瑛,塔里木大学化学化工学院教授、硕士研究生导师。新疆师范大学化学系专业毕业,目前主要从事于光电催化等方面的研究工作。发表论文50余篇,包括Coordination Chemistry Reviews、Chinese Physics B等。
王春栋,华中科技大学集成电路学院/武汉光电国家研究中心的双聘教授、博士研究生导师。2013 年于香港城市大学获博士学位;2013年—2015年先后在中国香港城市大学、中国香港科技大学、比利时荷语鲁汶大学从事博士后工作。目前主要从事包括单原子催化、自旋催化及燃料电池等方面的研究工作。发表SCI论文160 余篇,包括J.Am.Chem.Soc.、Energy Environ.Sci.、Angew.Chem.Int.Ed.、Adv.Energy Mater.、ACS Nano等,主持国家重点研发计划(政府间国际合作重点专项)、国家自然科学基金(3项)等多项项目。

作者简介: 张霞,塔里木大学化学化工学院硕士研究生,在吴瑛教授和王春栋教授的指导下进行研究。目前主要研究领域为尿素氧化反应中镍基MOFs及其衍生物的电催化剂设计。

引用本文:

张霞, 吴瑛, 袁牧锋, 王春栋. MOFs衍生物在尿素氧化中的研究进展[J]. 材料导报, 2024, 38(6): 23020193-10.
ZHANG Xia, WU Ying, YUEN Mufung, WANG Chundong. Recent Research Progress of MOFs Derivatives for Urea Oxidation. Materials Reports, 2024, 38(6): 23020193-10.

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https://www.mater-rep.com/CN/10.11896/cldb.23020193 或 https://www.mater-rep.com/CN/Y2024/V38/I6/23020193

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