地下水低渗透区重非水相液体(DNAPL)的增渗增移技术综述

doi:10.11896/cldb.22120129

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Abstract Dense non-aqueous phase liquids (DNAPL) is a kind of organic pollutant with stable physicochemical properties and strong toxicity, which poses a great threat to human health and the ecological environment. Due to its high density and strong penetration, DNAPL tends to accumulate in low-permeability zones, forming a long-term source of pollution. The slow flow rate and difficult mass transfer in low-permeability zones make frequently-used remediation methods ineffective, whereas the systematic research focusing on this issue is insufficient. Therefore, it is urgent to summarize the methods of enhancing permeability and migration of DNAPL which are aimed to promote pollutant remediation in low-permeability zones, so that it can serve as the reference for subsequent research. In this paper, firstly, the principle of aforementioned enhancement was delineated through the governing equation. Secondly, mechanisms underlying two methods of enhancing permeability and migration of DNAPL respectively based on surfactants and electrokinetics were summarized: surfactants enhance permeability and migration by micelle solubilizing and reducing adsorption, while electrokinetics enhances migration by electroosmotic flow and electromigration. Additionally, cases using coupling methodologies in practical applications and their effectiveness and feasibility were described. Finally, the future development direction was prospected.

Key words： dense non-aqueous phase liquids (DNAPL) low-permeability zones enhancing permeability and migration surfactant electrokinetics

Published: 25 March 2024 Online: 2024-04-07

CLC number:

X523

Fund:National Key R & D Program of China (2019YFE0114900),Shanghai Sailing Program (22YF1450200),and the National Natural Science Foundation of China (42077175, 52270164).

Corresponding Authors: ^*daichaomeng@tongji.edu.cn

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	HUANG Xiaoyi
	DAI Chaomeng
	YOU Xueji
	LI Si
	TONG Wangkai
	LI Jixiang

Cite this article:

HUANG Xiaoyi,DAI Chaomeng,YOU Xueji, et al. Enhancing the Permeability and Migration of DNAPL in Low-permeability Zones of Groundwater: a Technological Review[J]. Materials Reports, 2024, 38(6): 22120129-8.

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http://www.mater-rep.com/EN/10.11896/cldb.22120129 OR http://www.mater-rep.com/EN/Y2024/V38/I6/22120129

1 Fu Y F. Study on solubilization and mobilization based remediation of DNAPL contaminated aquifer by surfactants and their compounding systems. Master's Thesis, Jilin University, China, 2020 (in Chinese).
付玉丰. 表面活性剂及其复配体系对DNAPL污染含水层的增溶增流修复研究. 硕士学位论文, 吉林大学, 2020.
2 Zheng F. investigation on the migration and mediation of typical DNAPLs in saturated porous media. Ph. D. Thesis, Nanjing University, China, 2015 (in Chinese).
郑菲. 典型DNAPLs在饱和多孔介质中的运移及修复研究. 博士学位论文, 南京大学, 2015.
3 Maire J, Coyer A, Fatin-Rouge N. Journal of Hazardous Materials, 2015, 299, 630.
4 You X J, Liu S G, Dai C M, et al. Environmental Science and Pollution Research, 2020, 27(33), 41623.
5 Chowdhury A I A, Gerhard J I, Reynolds D, et al. Water Research, 2017, 113, 215.
6 Chen X L. Experimental study and numerical modeling on one-dimension solute transport in low permeability media. Master's Thesis, China University of Geosciences, China, 2015 (in Chinese).
陈晓恋. 低渗透介质中-维溶质运移实验与模拟研究. 硕士学位论文, 中国地质大学, 2015.
7 Dominguez C M, Romero A, Santos A. Chemical Engineering Journal, 2019, 376, 9.
8 Liang C J, Weng C Y. Journal of Hazardous Materials, 2022, 439, 8.
9 Fernandez J, Arjol M A, Cacho C. Environmental Science and Pollution Research, 2013, 20(4), 1937.
10 Moccia E, Intiso A, Cicatelli A, et al. Environmental Science and Pollution Research, 2017, 24(12), 11053.
11 Gao Y B, Zhang S B, Li T, et al. Journal of Tongji University(Natural Science), 2020, 48(1), 24 (in Chinese).
高彦斌, 张松波, 李韬, 等. 同济大学学报(自然科学版), 2020, 48(1), 24.
12 Schwille F. In: Pollutants in porous media, Yaron B, Dagan G, Goldshmid J, ed. , Springer, Berlin, 1984, pp. 27.
13 Tatti F, Papini P M, Torretta V, et al. Journal of Contaminant Hydrology, 2019, 222, 89.
14 Choong C E, Wong K T, Jang S B, et al. Journal of Environmental Chemical Engineering, 2022, 10(1), 107075.
15 Zhang J L. Research of the remediation of TCE-polluted low permeability media by using hydraulic fracturing. Master's Thesis, Jilin University, China, 2018 (in Chinese).
张久麟. 水力压裂法修复TCE污染低渗介质的研究. 硕士学位论文, 吉林大学, 2018.
16 Atkinson G M, Eaton D W, Igonin N. Nature Reviews Earth & Environment, 2020, 1(5), 264.
17 Miller C T, Weber W J. Ground Water, 1984, 22(5), 584.
18 Wei Y F. Influential factors of surfactant-enhanced remediation of PAHs contaminated soils and its mechanisms. Ph. D. Thesis, South China University of Technology, China, 2015 (in Chinese).
魏燕富. 表面活性剂增效修复PAHs污染土壤的影响因素及机制. 博士学位论文, 华南理工大学, 2015.
19 Li S. The washing remediation of the contaminated soil by PAHs with surfactants. Master's Thesis, Shenyang University, China, 2017(in Chinese).
李爽. 表面活性剂对多环芳烃污染土壤的淋洗修复研究. 硕士学位论文, 沈阳大学, 2017.
20 Liang X J. Co-solubilization of mixed polycyclic aromatic hydrocarbons (PAHs) in surfactant micelle systems. Ph. D. Thesis, South China University of Technology, China, 2017(in Chinese).
梁旭军. 多环芳烃混合物在表面活性剂胶束体系中的增溶机制研究. 博士学位论文, 华南理工大学, 2017.
21 Zhang J Y. Enhanced flushing remediation of tetrachloroethylene contaminated aquifers by in situ microemulsions. Master's Thesis, Jilin University, China, 2021 (in Chinese).
张婧懿. 原位微乳液对四氯乙烯污染含水层的强化冲洗修复研究. 硕士学位论文, 吉林大学, 2021.
22 Colombano S, Davarzani H, Van Hullebusch E D, et al. Science of the Total Environment, 2021, 760, 143958.
23 Su Y, Zhao Y S, Li L L, et al. China Environmental Science, 2015, 35(3), 817 (in Chinese).
苏燕, 赵勇胜, 李璐璐, 等. 中国环境科学, 2015, 35(3), 817.
24 Zhong L, Szecsody J, Oostrom M, et al. Journal of Hazardous Materials, 2011, 191(1-3), 249.
25 Mulligan C N, Wang S. Engineering Geology, 2006, 85(1-2), 75.
26 Maire J, Fatin-Rouge N. Journal of Hazardous Materials, 2017, 321, 247.
27 Couto H J, Massarani G, Biscaia E C, et al. Journal of Hazardous Materials, 2009, 164, 1325.
28 Fleifel H, Izadi M, Park S, et al. Transport in Porous Media, 2020, 134(3), 565.
29 Roothmel R K, Peters R W, Stmartin E, et al. Environmental Science & Technology, 1998, 32(11), 1667.
30 Gao K N. Study on removal of typical organic matter-heavy metal complex pollutants in soil by microbubble coupling detergent and its mechanism. Master's Thesis, Donghua University, China, 2022 (in Chinese).
高康宁. 微气泡耦合洗涤剂脱除土壤中典型有机物-重金属复合污染物及机理研究. 硕士学位论文, 东华大学, 2022.
31 Boonamnuayvitaya V, Jutaporn P, Sae-ung S, et al. Separation and Purification Technology, 2009, 68(3), 411.
32 Yan Y L, Deng Q, He F, et al. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2011, 385(1-3), 219.
33 Dai C, Tong W K, Zou J J, et al. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2022, 644.
34 Maire J, Brunol E, Fatin-Rouge N. Chemosphere, 2018, 197, 661.
35 Boufadel M C, Jj W, Jayalakshmamma M P, et al. Journal of Environmental Engineering, 2021, 147(3), 03120011.
36 Silva J A K, Liberatore M, Mccray J E. Journal of Environmental Engineering, 2013, 139(2), 149.
37 Martel R, Hebert A, Lefebvre R, et al. Journal of Contaminant Hydrology, 2004, 75(1-2), 1.
38 Robert T, Martel R, Conrad S H, et al. Journal of Contaminant Hydrology, 2006, 86(1-2), 3.
39 Attela O, Del Campo Estrada E, Bertin H. Reviews in Environmental Science and Bio/Technology, 2013, 12(4), 379.
40 Hauswirth S C, Miller C T. Journal of Contaminant Hydrology, 2014, 167, 44.
41 Martel K E, Martel R, Lefebvre R, et al. Groundwater Monitoring & Remediation, 1998, 18(3), 103.
42 Lian J R. Application of KMnO₄ for remediation of TCE-contaminated heterogeneous aquifer under viscosity control: mechanisms and effectiveness. Master's Thesis, Jilin University, China, 2018 (in Chinese).
廉静茹. 流体粘度调控下KMnO₄对TCE非均质含水层污染的强化修复机理与效能. 硕士学位论文, 吉林大学, 2018.
43 Wang H, Chen J. Environmental Technology, 2014, 35(5-8), 993.
44 Hirasaki G J, Miller C A, Szafranski R, et al. In: the SPE Annual Technical Conference and Exhibition. Texas, 1997, pp. 1836.
45 Mulligan C N, Eftekhari F. Engineering Geology, 2003, 70(3-4), 269.
46 Bouzid I, Fatin-Rouge N. Journal of Hazardous Materials, 2022, 432, 128703.
47 Zhong L, Oostrom M, Wietsma T W, et al. Journal of Contaminant Hydrology, 2008, 101(1-4), 29.
48 Rodrigo M A, Rodrigo M A, Dos Santos E V, et al. Electrochemically assisted remediation of contaminated soils: fundamentals, technologies, combined processes and pre-pilot and scale-up applications, Springer, Switzerland, 2021, pp. 30.
49 Koliyabandara S M P A, Siriwardhana C, De Silva S M, et al. In: Electrokinetic remediation for environmental security and sustainability, Wiley, US, 2021, pp. 453.
50 Wang X, Ren L, Long T, et al. Environmental Chemistry Letters, DOI: 10. 1007/s10311-022-01506-w.
51 Pazos M, Rosales E, Alcantara T, et al. Journal of Hazardous Materials, 2010, 177(1-3), 1.
52 Kebria D Y, Taghizadeh M, Camacho J V, et al. Environmental Earth Sciences, 2016, 75, 699.
53 Du W, Zou H, Yu C S, et al. Environmental Engineering Science, 2017, 34(12), 908.
54 Qiao W, Ye S, Wu J, et al. Ground Water, 2018, 56(4), 673.
55 Maturi K, Reddy K R. Water, Air, and Soil Pollution, 2008, 189(1), 199.
56 Alcántara T, Pazos M, Cameselle C, et al. Environmental Geochemistry and Health, 2008, 30(2), 89.
57 Yeung A T, Gu Y Y. Journal of Hazardous Materials, 2011, 195, 11.
58 Yuan S, Tian M, Lu X. Journal of Hazardous Materials, 2006, 137(2), 1218.
59 Li T, Yuan S, Wan J, et al. Journal of Hazardous Materials, 2010, 176(1-3), 306.
60 Chang J H, Qiang Z, Huang C P. Colloids and Surfaces A: Physicoche-mical and Engineering Aspects, 2006, 287(1), 86.
61 Zou H, Du W, Ji M, et al. Environmental Engineering Science, 2016, 33(7), 507.
62 Reddy K R, Darko-Kagya K, Al-Hamdan A Z. Water, Air, & Soil Pollution, 2011, 221(1-4), 35.
63 Ik Chung H, Kamon M. Engineering Geology, 2005, 77(3-4), 233.
64 Pham T D, Sillanpää M. Advanced Water Treatment, 2020, 227, 1403.
65 Zheng D, Geng Z, Huang W, et al. Journal of Hazardous Materials, 2022, 439, 129633.
66 Geng Z, Liu B, Li G, et al. Journal of Hazardous Materials, 2021, 413, 125455.
67 Mumford K G, Martin E J, Kueper B H. Journal of Contaminant Hydro-logy, 2021, 243, 103892.
68 Reddy K R, Darko-Kagya K, Al-Hamdan A Z. Environmental Enginee-ring Science, 2011, 28(6), 405.
69 Liu B, Li G, Mumford K G, et al. Chemosphere, 2020, 250, 126209.
70 Jiradecha C, Urgun-Demirtas M, Pagilla K. Journal of Hazardous Mate-rials, 2006, 136(1), 61.
71 Pham T D, Shrestha R A, Virkutyte J, et al. Electrochimica Acta, 2009, 54(5), 1403.