| ELECTROCHEMICAL ENERGY MATERIALS AND DEVICES |
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| Recent Research Progress of MOFs Derivatives for Urea Oxidation |
| ZHANG Xia1,2, WU Ying1,*, YUEN Mufung3, WANG Chundong2,*
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1 School of Chemistry and Chemical Engineering, Tarim University, Alar 843300, Xinjiang, China
2 School of Integrated Circuits, Huazhong University of Science and Technology, Wuhan 430074, China
3 School of Science and Technology, The Chinese University of Hong Kong (Shenzhen), Shenzhen 518172, Guangdong, China |
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Abstract Urea oxidation reaction (UOR) plays an essential role in reducing the strain of contemporary hydrogen energy production and wastewater treatment, and the development of electrocatalysts with superior performance can aid in lowering the amount of energy required. Derivatives of metal-organic frameworks (MOFs) materials have garnered a lot of attention for their potential as electrocatalysts, by addressing the inherent flaws of poor conductivity and stability. With reference to the design and construction of MOF-derivatives, we review and summarize some studies based on: (i) the reaction mechanism of nickel-based/non-nickel-based UOR; (ii) strategies to improve the electronic conductivity by means of structural modulation, morphology control, interfacial engineering, and defect engineering, outlining the change in physical properties of the materials with respect to the catalytic activity correlation;(iii) analyses of the applications of UOR-based MOFs derivatives. Finally, we give some perspectives on the most recent research challenges and developments in UOR.
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Published: 25 March 2024
Online: 2024-04-07
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| Fund:South Xinjiang Innovation and Development Program of Key Industries of Xinjiang Production and Construction Corps(2020DB002, 2022DB009), and Shenzhen Natural Science Foundation of China (General Program) (JCYJ20190813172609404). |
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Corresponding Authors:
*wuyingjuyuan@163.com;apcdwang@hust.edu.cn
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